Decorative Sheet With Dual Urethane Acrylates for Crack Resistance

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Solution Overview

Problem

Existing decorative sheets with ionizing radiation-curable resins suffer from curing shrinkage, contamination resistance, alkali resistance, and brittleness, leading to cracks and breakage, and the use of aliphatic isocyanate can destabilize these properties over time.

Innovation Solution

A decorative sheet with a laminate structure comprising a first surface-protecting layer made of two kinds of aliphatic urethane acrylates, one with an isocyanurate skeleton and the other with an alicyclic skeleton, and a second surface-protecting layer with lower hardness, providing a nanoindentation hardness range of 160-240 MPa and 100-240 MPa respectively, enhancing contamination and alkali resistance while reducing cracks and breakage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If an ionizing radiation-curable resin is used for the surface-protecting layer, then contamination resistance and alkali resistance are improved, but the layer becomes brittle and prone to cracks and breakage

Engineering Contradiction:
Improvecontamination resistance and alkali resistanceVSAvoidimpact resistance
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent uses a composite resin system comprising both ionizing radiation-curable resin and two-component curable resin in the surface-protecting layer. This composite structure allows the layer to simultaneously achieve contamination resistance and alkali resistance from the ionizing radiation-curable resin while gaining impact resistance and flexibility from the two-component curable resin, thereby resolving the contradiction between durability and brittleness.

Inventive Principle:
Principle #40Composite materials

2Reliability

If an ionizing radiation-curable resin is used for the surface-protecting layer, then contamination resistance and alkali resistance are improved, but curing shrinkage occurs affecting surface quality

Engineering Contradiction:
Improvecontamination resistance and alkali resistanceVSAvoidsurface quality
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent combines ionizing radiation-curable resin with two-component curable resin in a composite system. The two-component curable resin compensates for the curing shrinkage of the ionizing radiation-curable resin, thereby maintaining surface quality and dimensional stability while preserving the contamination resistance and alkali resistance properties.

Inventive Principle:
Principle #40Composite materials

3Strength

If aliphatic isocyanate is added to the surface-protecting layer, then impact resistance is improved, but physical properties become unstable over time

Engineering Contradiction:
Improveimpact resistanceVSAvoidphysical property stability
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The patent modifies the chemical composition parameters by replacing aliphatic isocyanate with aromatic isocyanate in the two-component curable resin system. This parameter change maintains the impact resistance benefits while improving long-term stability, as aromatic isocyanate provides more stable cured structures that resist degradation over time.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The laminate structure with specific aliphatic urethane acrylates in the surface-protecting layers ensures long-term contamination and alkali resistance, minimizing cracks and breakage, and improves scratch resistance under high loads.

Implementation Method 1

a surface-protecting layer formed from an ionizing radiation-curable resin

Methodology Applied
Scientific EffectCrosslinking polymerization: Photopolymerisation

Implementation Method 2

the first surface-protecting layer comprising an ionizing radiation-curable resin containing two kinds of aliphatic urethane acrylates

Methodology Applied
Scientific EffectCuring reaction: Chemical Bonding

Data Source

PatentEP3848199B1Decorative sheet, decorative panel, and coating agent for forming surface protective layer
Publication Date: 2025.11.05 DAI NIPPON PRINTING CO LTD
  • EP3848199B1 patent drawingFigure 1
  • EP3848199B1 patent drawingFigure 2
  • EP3848199B1 patent drawingFigure 3(a)~3(c)

AI summary

The present invention provides a decorative sheet comprising a surface-protecting layer, the surface-protecting layer having excellent contamination resistance, alkali resistance, etc., for a long period of time, while limiting the occurrence of breakage and cracks when an impact is applied thereto or during processing; and also provides a decorative plate using the decorative sheet. Specifically, the present invention provides a decorative sheet comprising a laminate, the laminate comprising at least a base material sheet and a first surface-protecting layer in sequence in the thickness direction; (1) the first surface-protecting layer comprising an ionizing radiation-curable resin containing two kinds of aliphatic urethane acrylates, i.e., resin A and resin B, wherein resin A is an aliphatic urethane acrylate with an isocyanurate skeleton, and resin B is an aliphatic urethane acrylate with an alicyclic skeleton without an isocyanurate skeleton, and (2) the first surface-protecting layer having a nanoindentation hardness of 160 MPa or more and 240 MPa or less. The present invention also provides a decorative plate using the decorative sheet.