Degradable Polymer Coatings for Fracturing Proppant

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Solution Overview

Problem

Conventional fracking techniques face issues such as material deficiencies, rheology limitations, and environmental concerns in hydraulic-based recovery systems, particularly in low permeability subsurface formations, which hinder economical extraction of hydrocarbons.

Innovation Solution

A degradable polymer composition that remains solid under dry conditions but depolymerizes into a viscous liquid when exposed to water, allowing for hydraulic fracturing and subsequent breakdown into water-soluble components, enhancing formation permeability and facilitating hydrocarbon extraction.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional fracking materials are used, then hydraulic fracturing can be performed, but material deficiencies and rheology limitations occur that hinder effective treatment of low permeability formations

Engineering Contradiction:
Improvefracturing effectivenessVSAvoidmaterial suitability for low permeability formations
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent applies parameter changes by utilizing the temperature-dependent solubility characteristics of polymers in supercritical CO2. The polymer is selected to be substantially insoluble at reservoir temperature (maintaining solid proppant coating) but soluble at surface temperature (enabling disposal). This parameter change resolves the contradiction by making the same material suitable for both low permeability formation treatment and easy disposal, while maintaining fracturing effectiveness throughout the process

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs composite materials by combining polymer coatings with proppant particles. The polymer-proppant composite provides both the mechanical support needed for fracturing effectiveness and the temperature-responsive solubility characteristics. This composite structure enables the material to function effectively in low permeability formations while remaining dispensable, thus resolving the adaptability contradiction

Inventive Principle:
Principle #40Composite materials

2Reliability

If solid proppant is used to maintain fracture openness, then fracture conductivity is improved, but proppant disposal becomes difficult and costly

Engineering Contradiction:
Improvefracture conductivityVSAvoidproppant disposal ease
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent utilizes parameter changes in polymer solubility with temperature. At reservoir temperature, the polymer is insoluble and maintains solid proppant characteristics for fracture conductivity. At surface temperature, the polymer becomes soluble and can be easily disposed of by flushing with CO2. This resolves the contradiction between maintaining fracture conductivity and enabling easy disposal

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies the disposable principle by using polymer-coated proppant that is designed to be temporary. The polymer coating provides necessary fracture conductivity during production, then becomes soluble and removable via CO2 flushing. This replaces permanent proppant with a disposable alternative, resolving the disposal difficulty while maintaining fracture conductivity during the needed period

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Productivity

If polymer viscosity is increased to improve fluid carrying capacity, then proppant transport capability improves, but fluid rheology becomes more difficult to control

Engineering Contradiction:
Improveproppant transport capabilityVSAvoidfluid rheology control
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent extracts the viscosity-control function from the bulk fracturing fluid and places it solely on the polymer-coated proppant particles. The polymer coating provides the necessary viscosity and carrying capacity at the particle level, while the bulk fluid maintains simple, easily controlled rheology. This separation resolves the contradiction between proppant transport capability and fluid rheology control complexity

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The degradable polymer composition effectively increases formation permeability, enabling efficient hydrocarbon extraction by transforming into a viscous, pumpable form that can be used for fracturing and subsequently breaks down into environmentally benign components, reducing equipment costs and environmental impact.

Implementation Method 1

the polymer chains are slowly 'degrading' due primarily to hydrolytic action, referred to at times herein as 'depolymerization,' which eventually manifests qualitatively as an observable transition of the polymeric material from an essentially solid form to a less and less 'solid' state, then ultimately to dissolved or dispersed state

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Data Source

PatentEP2970754B1Degradable polymers and method for fracking applications
Publication Date: 2020.09.30 DANIMER SCIENTIFIC LLC

AI summary

The present disclosure is directed degradable polymers. The polymers are solid when maintained under substantially dry conditions at a temperature of up to about 90 degrees C. When contacted with water at a temperature of up to about 90 degrees C, however, the polymers initially remain solid for a period of up to about 6 to about 24 hours, then depolymerize to provide a liquid having a viscosity of from about 1 to about 200,000 centipoise after a period of time from about 8 hours to about 3 days and then further depolymerizes to water-soluble components after a period of time at least about 3 days. Also disclosed are sand screen coatings made with the polymers and hydraulic and acid fracturing methods using the polymers.