Dehydrogenation Catalyst Bed with Heat-Generating Component

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Solution Overview

Problem

Current endothermic hydrocarbon conversion processes require high energy due to high air temperatures and flow rates, leading to increased operating and capital costs, and suffer from lower hydrocarbon conversion yields due to temperature control challenges and coke deposition on catalysts.

Innovation Solution

The process involves a multi-component catalyst bed with a heat-generating component, such as copper or manganese, in the middle section to preheat the catalyst bed, reducing the need for external heating and allowing lower air-to-hydrocarbon ratios and operation at near-atmospheric pressures, thereby improving energy efficiency and conversion yields.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If high air temperatures and flow rates are used in the regeneration step, then the catalyst bed can be effectively regenerated and reheated, but energy consumption increases significantly

Engineering Contradiction:
Improvecatalyst regeneration effectivenessVSAvoidenergy consumption
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

A heat-generating component (such as copper oxide or manganese oxide) is incorporated into the catalyst bed that can generate heat during the reduction step before dehydrogenation. This preliminary heat generation pre-heats the catalyst bed, reducing the amount of heat that needs to be supplied during regeneration and thereby lowering overall energy consumption while maintaining effective catalyst regeneration

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention changes the thermal parameters of the catalyst bed by incorporating materials with specific heat generation and storage properties. The heat-generating component alters the temperature profile and heat distribution within the bed, enabling more efficient heat utilization during the cyclic process and reducing the energy required for regeneration at high temperatures and flow rates

Inventive Principle:
Principle #35Parameter changes

2Reliability

If high air flow rates are used during regeneration, then coke removal is improved, but operating costs increase

Engineering Contradiction:
Improvecoke removal efficiencyVSAvoidoperating costs
Core Design Contradiction:
ReliabilityVSLoss of energy

Solution Approach 1:

The heat-generating component in the catalyst bed provides self-heating during the reduction step, creating a self-sustaining thermal cycle. This internal heat generation reduces the dependency on external high-temperature air flow for coke removal, allowing effective regeneration at lower air flow rates and thereby reducing operating costs while maintaining coke removal efficiency

Inventive Principle:
Principle #25Self-service

3Productivity

If the catalyst bed is reheated between cycles, then dehydrogenation conversion is improved, but additional external heating equipment is required

Engineering Contradiction:
Improvehydrocarbon conversion yieldVSAvoidheating equipment
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The catalyst bed contains heat-generating components that automatically generate heat during the reduction step, providing self-reheating functionality. This eliminates the need for external heating equipment between cycles, as the catalyst bed self-regenerates and self-reheats through the chemical reactions of the incorporated heat-generating materials, thereby improving conversion yield without increasing device complexity

Inventive Principle:
Principle #25Self-service

4Productivity

If the catalyst bed temperature is maintained uniformly, then reaction efficiency is improved, but temperature control becomes more difficult due to coke distribution variations

Engineering Contradiction:
Improvereaction efficiencyVSAvoidtemperature control
Core Design Contradiction:
ProductivityVSEase of operation

Solution Approach 1:

The heat-generating component is distributed throughout the catalyst bed, providing localized heat generation at multiple points. This distributed approach compensates for local variations in coke distribution and heat consumption, maintaining more uniform temperature profiles across the bed and improving reaction efficiency while simplifying temperature control, as the system self-regulates through the distributed heat generation rather than requiring complex external control mechanisms

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach decreases energy costs and maintains or improves hydrocarbon conversion yields while reducing coke deposition and temperature fluctuations within the catalyst bed, enhancing overall process efficiency and cost-effectiveness.

Implementation Method 1

reducing the catalyst bed wherein the heat-generating component of the second catalyst composition generates heat that passes into the first catalyst composition and, if present, the third catalyst composition

Methodology Applied
Scientific EffectHeat generation: Exothermic Reaction

Implementation Method 2

regenerating the catalyst bed by contacting the catalyst bed with air

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

contacting a hydrocarbon feedstock with the catalyst bed to form a dehydrogenated hydrocarbon

Methodology Applied
Scientific EffectEndothermic reaction: Endothermic Reaction

Data Source

PatentEP3116844B1Improved dehydrogenation process with heat generating material
Publication Date: 2019.01.16 CLARIANT CORP
  • EP3116844B1 patent drawingFigure 1~2

AI summary

The disclosure provides an improved endothermic hydrocarbon conversion process that comprises reacting a hydrocarbon with a multi-component catalyst bed, and regenerating the catalyst bed with air, where the air used in regeneration step and hydrocarbon are at low air to hydrocarbon ratios and optionally at near-atmospheric pressures.