Dehydrogenation Reactor Volume Reduction via Partial Reaction

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Solution Overview

Problem

Existing methods for providing hydrogen gas in mobile applications, such as hydrogen-powered vehicles, require large installation spaces due to the need for extensive dehydrogenation reactors and storage containers, leading to inefficiencies and increased space requirements.

Innovation Solution

The method involves optimizing the dehydrogenation reaction by focusing on zones with high reaction rates within the dehydrogenation reactor, reducing the overall installation space by minimizing the length of the flow tube and using multiple reactors in parallel or series configurations to maintain efficient hydrogen release, while adjusting the dehydrogenation stroke for optimal space utilization.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If complete dehydrogenation reaction is used to release hydrogen gas from hydrogen carrier medium, then hydrogen release efficiency is improved, but overall installation space increases significantly

Engineering Contradiction:
Improvehydrogen release efficiencyVSAvoidoverall installation space
Core Design Contradiction:
ProductivityVSVolume of stationary object

Solution Approach 1:

The patent applies partial action by deliberately stopping the dehydrogenation reaction before complete hydrogen release (at 5-15% residual hydrogen instead of 0%). This partial dehydrogenation approach reduces the required reactor volume and flow tube length while still providing sufficient hydrogen for mobile applications, thereby resolving the contradiction between hydrogen release efficiency and installation space requirements

Inventive Principle:
Principle #16Partial or excessive action

Solution Approach 2:

The patent changes the dehydrogenation stroke parameter from the conventional near-complete conversion to a controlled partial conversion (stopping at 5-15% residual hydrogen). This parameter change optimizes the balance between hydrogen release productivity and reactor volume, reducing installation space while maintaining adequate hydrogen supply for mobile applications

Inventive Principle:
Principle #35Parameter changes

2Volume of stationary object

If dehydrogenation reactor volume is reduced to minimize installation space, then overall device compactness is improved, but hydrogen release rate decreases

Engineering Contradiction:
Improvereactor volumeVSAvoidhydrogen release rate
Core Design Contradiction:
Volume of stationary objectVSProductivity

Solution Approach 1:

By implementing partial dehydrogenation (stopping at 5-15% residual hydrogen), the patent reduces the effective dehydrogenation stroke required in the reactor. This allows for a smaller reactor volume while maintaining adequate hydrogen release rates for mobile applications, as the reaction is stopped in the high-rate zone before catalyst deactivation and side reactions occur

Inventive Principle:
Principle #16Partial or excessive action

Solution Approach 2:

The patent skips the low-productivity zone of the dehydrogenation reaction by deliberately stopping the process at 5-15% residual hydrogen. This avoids the extended residence time and larger reactor volume that would be required to achieve complete dehydrogenation, thereby reducing installation space while maintaining sufficient hydrogen release rates

Inventive Principle:
Principle #21Skipping (Rushing through)

3Volume of stationary object

If flow tube length is minimized to reduce installation space, then device compactness is improved, but reaction completeness deteriorates

Engineering Contradiction:
Improveflow tube lengthVSAvoidreaction completeness
Core Design Contradiction:
Volume of stationary objectVSManufacturing precision

Solution Approach 1:

The patent applies partial action by intentionally limiting the flow tube length to achieve only partial dehydrogenation (5-15% residual hydrogen). This shorter flow tube length reduces installation space while the controlled partial reaction completeness is sufficient for mobile hydrogen applications, avoiding the need for excessively long flow tubes that would increase device size

Inventive Principle:
Principle #16Partial or excessive action

4Reliability

If multiple reactors are used in parallel or series to maintain hydrogen release efficiency, then hydrogen release stability is improved, but device complexity increases

Engineering Contradiction:
Improvehydrogen release stabilityVSAvoidreactor configuration complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

By implementing partial dehydrogenation in a single reactor, the patent simplifies the overall device configuration compared to multiple-reactor systems. The partial reaction approach maintains adequate hydrogen release stability for mobile applications without requiring complex parallel or series reactor arrangements, thereby reducing device complexity while preserving sufficient reliability

Inventive Principle:
Principle #16Partial or excessive action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly reduces the overall installation space required for hydrogen gas provision, improves the efficiency of hydrogen storage and release, and enhances the purity of the hydrogen stream by minimizing catalyst material and residence time, thus optimizing the hydrogen storage process for mobile applications.

Implementation Method 1

The hydrogen is released by a material conversion of the loaded hydrogen carrier medium (LOHC-H) by discharging in the at least one dehydrogenation reactor of the discharging unit by means of a catalytic dehydrogenation reaction

Methodology Applied
Scientific EffectCatalytic dehydrogenation reaction: Catalysis

Implementation Method 2

A heating circuit with at least one hydrogen burner serves to provide heat for the dehydrogenation reactor

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 3

A heating circuit with at least one hydrogen burner serves to provide heat for the dehydrogenation reactor

Methodology Applied
Scientific EffectCombustion: Combustion

Data Source

PatentEP3837209B1Process and device for providing hydrogen gas
Publication Date: 2025.01.01 HYDROGENIOUS TECH GMBH
  • EP3837209B1 patent drawingFigure 1
  • EP3837209B1 patent drawingFigure 2
  • EP3837209B1 patent drawingFigure 3

AI summary

The invention relates to a process for providing hydrogen gas, comprising the steps of supplying a hydrogen carrier medium of a first hydrogenation degree from a storage reservoir (15, 35) to a dehydrogenation reactor (17) and of dehydrogenating the hydrogen carrier medium to a second hydrogenation degree which is lower than the first hydrogenation degree, thereby releasing hydrogen gas, the difference between the first hydrogenation degree and the second hydrogenation degree being in the range of an optimum dehydrogenation capacity.