Disulfide Solvent Odor Management via Blend and Oxidant

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Solution Overview

Problem

The excessive odor of disulfide solvents, such as dimethyl disulfide, poses operational difficulties in dissolving elemental sulfur, making them impractical for use due to the need for extensive engineering controls, and the scarcity of diaryl disulfide limits its availability as a suitable replacement.

Innovation Solution

A solvent blend comprising a disulfide solvent, an amine solvent, a ketone solvent, and an ester solvent is used to maintain odor balance, with additional ester solvent added to restore balance and convert biphasic mixtures into emulsions, and oxidants applied to odor-imbalanced surfaces to convert malodorous sulfur compounds into less volatile forms.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If disulfide solvents are used to dissolve elemental sulfur, then dissolution capability is improved, but odor intensity increases to unacceptable levels

Engineering Contradiction:
Improveelemental sulfur dissolutionVSAvoidodor intensity
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent introduces an odor control agent as an intermediary substance that interacts with the disulfide solvent to neutralize or mask the harmful odor. The odor control agent serves as a mediator between the disulfide solvent and the environment, allowing the solvent to maintain its sulfur-dissolving function while the odor control agent handles the odor management, thus resolving the contradiction between dissolution capability and odor intensity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a composite solvent system by combining the disulfide solvent with an odor control agent. This composite material integrates the functional properties of the disulfide solvent (sulfur dissolution) with the odor-mitigating properties of the control agent, resulting in a unified system that simultaneously achieves both dissolution capability and acceptable odor levels.

Inventive Principle:
Principle #40Composite materials

2Object-generated harmful factors

If extensive engineering controls are implemented to preclude discharge of disulfide solvent, then odor discharge is reduced, but operational complexity and cost increase to impractical levels

Engineering Contradiction:
Improveodor dischargeVSAvoidengineering controls
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent converts the harmful odor property of the disulfide solvent into a manageable characteristic by adding an odor control agent. Instead of treating the odor as a harmful factor requiring complex engineering controls, the solution transforms the odor management into a chemical modification of the solvent system itself, thereby eliminating the need for extensive engineering controls while still achieving odor discharge reduction.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The odor control agent enables the solvent system to self-regulate its odor emissions without requiring external engineering controls. The control agent is incorporated into the solvent system, allowing it to automatically manage its own odor discharge characteristics, thus eliminating the need for complex external control systems.

Inventive Principle:
Principle #25Self-service

3Object-generated harmful factors

If diaryl disulfide is used as a replacement solvent, then odor is reduced to acceptable levels, but availability becomes limited due to curtailed commercial production

Engineering Contradiction:
Improveodor intensityVSAvoidsolvent availability
Core Design Contradiction:
Object-generated harmful factorsVSAdaptability or versatility

Solution Approach 1:

The patent modifies the parameters of the disulfide solvent system by adding an odor control agent, rather than changing the fundamental solvent identity. This parameter change approach allows the use of readily available disulfide solvents (like dimethyl disulfide) while adjusting the system's odor characteristics through the control agent, thus maintaining solvent availability while achieving acceptable odor levels.

Inventive Principle:
Principle #35Parameter changes

4Quantity of substance

If dimethyl disulfide is used as a replacement solvent, then sulfur dissolution capability is maintained, but operational challenges arise due to extreme odor

Engineering Contradiction:
Improveelemental sulfur dissolutionVSAvoidoperational feasibility
Core Design Contradiction:
Quantity of substanceVSEase of operation

Solution Approach 1:

The odor control agent acts as an intermediary that allows dimethyl disulfide to maintain its excellent sulfur dissolution capability while the control agent handles the odor management. This intermediary approach preserves the operational advantages of dimethyl disulfide (high sulfur solubility) while eliminating the operational challenges (extreme odor) through the mediating function of the control agent.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solvent blend effectively suppresses the odor of disulfide solvents, maintaining their dissolution capabilities while reducing odor intensity, and the methods address odor imbalance in both solvent blends and surfaces, facilitating safer and more practical use.

Implementation Method 1

contacting the odor imbalanced surface with an oxidant to convert the one or more sulfur compounds in a higher oxidation state

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

hydrolyzing at least a portion of the at least one ester solvent under conditions that afford a biphasic mixture comprising a heavy phase and a light phase

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Implementation Method 3

dissolving at least a portion of the elemental sulfur in the solvent blend

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentUS20240034923A1Odor management for disulfide solvents and surfaces contacted therewith
Publication Date: 2024.02.01 EXXONMOBIL TECHNOLOGY & ENGINEERING CO

AI summary

Disulfide solvents may be particularly effective for dissolving deposits comprising elemental sulfur, but the extreme odor of these solvent may make their use rather problematic. Solvent blends comprising at least one disulfide solvent, amine solvent, ketone solvent, and ester solvent may afford a less obnoxious odor and not appreciably compromise the sulfur dissolution capabilities. Surfaces contacted with such solvent blends or at least partially spent variants thereof may exhibit excessive odor due to loss of one or more of the amine, ketone, or ester solvents. Excessive odor resulting from a solvent residue upon a surface may be alleviated by contacting the surface with at least one oxidant. Odor balance may also be restored to at least partially spent solvent blends by introducing additional ester solvent, which may convert a biphasic mixture into an emulsion comprising the disulfide solvent.