2,6-Dimethylnaphthalene Purification via Melt Crystallization

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Solution Overview

Problem

Current methods for separating and purifying 2,6-dimethylnaphthalene from a mixture of dimethylnaphthalene isomers face challenges due to close boiling points, requiring complex and costly processes, and existing methods are not suitable for industrial scale-up, especially those involving crystallization which demand high fixed investment and production costs.

Innovation Solution

A combined process of column melt crystallization and sweating operation, where molten dimethylnaphthalene isomers are cooled to form crystal layers, followed by vacuum filtration and partial melting of impurities, allowing for the separation and recovery of high-purity 2,6-dimethylnaphthalene with reduced energy consumption and simplified apparatus.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If distillation is used to separate dimethylnaphthalene isomers, then separation can be achieved, but the process becomes complex and costly due to very close boiling points

Engineering Contradiction:
Improveseparation purityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention changes the separation parameter from boiling point (distillation) to melting point (crystallization). Since dimethylnaphthalene isomers have very close boiling points making distillation difficult, the method exploits the significant difference in melting points, particularly that 2,6-DMN has the highest melting point (112°C), to achieve separation through selective crystallization.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes the phase transition from liquid to solid through controlled cooling. By cooling the molten mixture to a temperature where 2,6-DMN crystallizes first (exploiting its highest melting point), the method achieves separation without the complexity of distillation equipment and multiple stages.

Inventive Principle:
Principle #36Phase transitions

2Manufacturing precision

If crystallization methods are used to separate 2,6-dimethylnaphthalene, then high purity can be achieved, but fixed investment and production costs increase

Engineering Contradiction:
Improveproduct purityVSAvoidproduction cost
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The invention extracts 2,6-DMN from the isomeric mixture through selective crystallization based on its unique highest melting point. By removing 2,6-DMN in crystalline form while other isomers remain in the mother liquor, the method achieves high purity without requiring expensive solvents or complex extraction systems.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The method uses simple, inexpensive equipment for cooling and filtration rather than expensive, complex crystallization apparatus. The process relies on basic thermal control and vacuum filtration, avoiding high fixed investment in specialized equipment while achieving the desired purification.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Manufacturing precision

If existing crystallization processes are used, then purification can be achieved, but the apparatus becomes complex and energy consumption increases

Engineering Contradiction:
Improvepurification efficiencyVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

Instead of using complex multi-stage crystallization processes that require extensive heating and cooling cycles, the invention inverts the approach by using a single-stage cooling process that exploits the natural crystallization temperature difference. The simple cooling step followed by vacuum filtration reduces energy consumption compared to conventional methods.

Inventive Principle:
Principle #13The other way round (Inversion)

4Manufacturing precision

If multi-stage crystallization is used to achieve high purity, then separation efficiency improves, but productivity decreases due to repeated operations

Engineering Contradiction:
Improveseparation efficiencyVSAvoidthroughput
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The invention performs preliminary selection of 2,6-DMN through its unique highest melting point characteristic in a single cooling step. By designing the process to crystallize 2,6-DMN first at a specific temperature range, the method achieves high purity in one stage without requiring repeated crystallization cycles, thereby maintaining high productivity.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method achieves high-purity 2,6-dimethylnaphthalene with a high yield, reducing production costs and enabling industrial scalability by utilizing a simpler, energy-efficient process that minimizes the need for expensive solvents and complex apparatus.

Implementation Method 1

cooling a molten liquid of a mixture of dimethylnaphthalene (DMN) isomers to perform melt crystallization

Methodology Applied
Scientific EffectMelt crystallization: Crystallisation

Implementation Method 2

separating the thus-produced crystals from a mother liquor by vacuum filtration

Methodology Applied
Scientific EffectVacuum filtration: Filter (physical)

Implementation Method 3

heating the crystal layers to partially melt impurities on surfaces of the crystal layers and between the crystal layers

Methodology Applied
Scientific EffectPartial melting: Melting

Data Source

PatentEP1852409B1Method for separating and purifying 2,6-dimethylnaphthalene
Publication Date: 2009.12.02 HYOSUNG CORP
  • EP1852409B1 patent drawingFigure 1
  • EP1852409B1 patent drawingFigure 2
  • EP1852409B1 patent drawingFigure 3

AI summary

A method for separating and purifying 2,6-dimethylnaphthalene, is provided in which 2,6-dimethylnaphthalene of high purity is obtained from a mixture of dimethylnaphthalene isomers with a high yield, by means of a combined process of column melt crystallization and sweating operation.