Doped Tin Oxide Thin Film Coating for Low-E Glass Durability

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Solution Overview

Problem

Low-E coatings incorporating silver layers face challenges such as limited durability, susceptibility to corrosion, and degradation during heat treatment, tempering, and bending, which affects their infrared reflecting properties and aesthetic appeal.

Innovation Solution

The introduction of an oxidizing chemical additive during pyrolytic deposition of doped tin oxide thin films enhances the optical and infrared reflecting properties, improving durability and resistance to heat treatment, and allowing for online deposition on heated glass ribbons, thus overcoming the limitations of silver-based coatings.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If silver layers are used in low-E coatings, then high infrared reflectance is achieved, but chemical and mechanical durability deteriorates

Engineering Contradiction:
Improvechemical and mechanical durabilityVSAvoidsusceptibility to corrosion and degradation
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent uses a composite structure with multiple thin film layers including metal oxide layers (such as tin oxide, zinc oxide, or indium oxide) combined with dielectric layers. This composite material approach replaces the single silver layer with a multi-layer system that provides both infrared reflectance and enhanced durability, eliminating the corrosion and degradation issues associated with pure silver coatings.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the material parameters by transitioning from metallic silver to metal oxide materials with specific optical and mechanical properties. By adjusting the composition, thickness, and stacking sequence of the metal oxide and dielectric layers, the coating achieves comparable infrared reflectance to silver while providing superior chemical stability and mechanical strength.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If sputter deposited silver layers are used, then high performance solar control is achieved, but production time increases due to offline deposition requirement

Engineering Contradiction:
Improveproduction timeVSAvoidonline deposition capability
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The patent replaces the sputtering deposition process with a pyrolytic deposition process. Pyrolytic deposition allows for online coating application directly on the glass ribbon during the float glass manufacturing process, eliminating the need for separate offline sputtering equipment and operations. This substitution of the deposition mechanism enables continuous production and significantly reduces manufacturing time.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Reliability

If silver layers are used in low-E coatings, then neutral color appearance is achieved, but aesthetic appeal deteriorates due to oxidation and reaction during heat treatment

Engineering Contradiction:
Improveaesthetic appeal and durabilityVSAvoidoxidation and reaction during heat treatment
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical composition parameters by using metal oxides (tin oxide, zinc oxide, indium oxide) instead of metallic silver. These metal oxide materials have inherent resistance to oxidation and chemical reactions, maintaining their optical properties and neutral appearance even after exposure to high temperatures during heat treatment processes. The material parameter change from metal to metal oxide eliminates the aesthetic degradation problem.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method results in low-E thin film optical stacks with improved infrared reflecting properties, increased durability, and reduced production time, making them competitive with silver-based coatings in terms of performance and cost.

Implementation Method 1

pyrolytic deposition of doped tin oxide thin films

Methodology Applied
Scientific EffectPyrolytic deposition: Pyrolysis

Implementation Method 2

pyrolytic deposition

Methodology Applied
Scientific EffectChemical vapor deposition: Chemical Vapour Deposition

Implementation Method 3

introduction of an oxidizing chemical additive during pyrolytic deposition

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 4

reflecting and blocking emission of infrared (IR) radiation

Methodology Applied
Scientific EffectInfrared reflection: Reflection

Implementation Method 5

permit the passage of visible light

Methodology Applied
Scientific EffectVisible light transmission: Refraction

Data Source

PatentEP2408618B1Method of making a thin film coating
Publication Date: 2020.05.06 AGC FLAT GLASS NORTH AMERICA INC
  • EP2408618B1 patent drawingFigure 1
  • EP2408618B1 patent drawingFigure 2
  • EP2408618B1 patent drawingFigure 3

AI summary

The present invention provides low-E thin film optical stacks with improved optical and infrared reflecting properties and methods of making the same. More specifically, the present invention provides for a metal oxide thin film coating that exhibits lower emissivity values than its predecessor due to the inclusion of an oxidizer in the metal oxide deposition process, such as a strong acid such as nitric acid. The present invention also provides for a method that increases the coating efficiencies of the thin films described herein.