Dry Particulate Geopolymer Composition Reducing Water Demand

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Existing geopolymer dry mixtures require a high amount of water for production, which is inefficient and may lead to incomplete reactions, and often have unsatisfactory mechanical properties due to insufficient amorphous aluminosilicate content and specific surface area.

Innovation Solution

A dry particulate composition comprising at least 45 wt.% amorphous aluminosilicate with a specific surface area product in the range of 7 to 15 m^2/g, combined with alkali metal hydroxide and alkali metal silicate, that can be easily mixed with limited water (less than 50 wt.%) at temperatures between 0°C and 100°C to form geopolymers with improved mechanical properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional liquid alkaline silicate is used to initiate polymerisation, then geopolymer formation occurs, but a very large amount of water is required which must subsequently be removed

Engineering Contradiction:
Improvegeopolymer formationVSAvoidwater demand
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The invention changes the physical state of the activating agent from liquid to dry particulate form. The dry particulate composition comprises alkali metal hydroxide and alkali metal silicate in dry particulate form, which when mixed with water, releases heat (exothermic reaction) to initiate geopolymerisation without requiring the large amounts of water needed for liquid alkaline silicate systems

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase transition by converting the activating agent from liquid phase to solid particulate phase. The dry particulate composition maintains stability in solid form during storage and handling, then transitions to active form upon contact with water, initiating the geopolymerisation reaction through exothermic heat release

Inventive Principle:
Principle #36Phase transitions

2Ease of manufacture

If existing dry mixture formulations are used, then storage and transport are simplified, but a high amount of water is still required for production

Engineering Contradiction:
Improvestorage and handlingVSAvoidwater demand
Core Design Contradiction:
Ease of manufactureVSQuantity of substance

Solution Approach 1:

The invention creates a composite dry particulate composition combining alkali metal hydroxide, alkali metal silicate, and aluminosilicate in specific proportions. This composite formulation ensures that when mixed with limited water (less than 50 wt.%), the components work synergistically to produce complete geopolymerisation with satisfactory mechanical properties

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention optimizes the water content parameter to less than 50 wt.%, which is significantly lower than conventional formulations. This parameter change, combined with the specific composition ratios, enables complete reaction without requiring the high water amounts needed by existing dry mixture technologies

Inventive Principle:
Principle #35Parameter changes

3Device complexity

If insufficient amorphous aluminosilicate content is used, then material composition is simplified, but mechanical properties become unsatisfactory

Engineering Contradiction:
Improvecomposition complexityVSAvoidmechanical properties
Core Design Contradiction:
Device complexityVSStrength

Solution Approach 1:

The invention specifies that at least 45 wt.% of the aluminosilicate must be in amorphous state. This local quality requirement ensures sufficient reactivity and bond formation capability in the geopolymer matrix, directly contributing to satisfactory mechanical properties while maintaining composition simplicity

Inventive Principle:
Principle #3Local quality

4Ease of manufacture

If specific surface area product is outside the optimal range, then material processing is simplified, but geopolymerisation reaction completeness is compromised

Engineering Contradiction:
Improveprocessing simplicityVSAvoidreaction completeness
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The invention defines a specific parameter range for the product of specific surface area (7 to 15 m²/g) that optimizes the reaction surface area available for geopolymerisation. This parameter control ensures complete reaction between components while maintaining practical processing simplicity

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach reduces water demand, simplifies on-site geopolymer production, and enhances mechanical properties by ensuring complete geopolymerization reactions, resulting in geopolymers with satisfactory cohesion and strength.

Implementation Method 1

a dissolution of a solid aluminosilicate by alkaline hydrolysis is the first reaction step and leads to the formation of aluminates and silicates

Methodology Applied
Scientific EffectDissolution: Solvation

Implementation Method 2

a dissolution of a solid aluminosilicate by alkaline hydrolysis is the first reaction step

Methodology Applied
Scientific EffectAlkaline hydrolysis: Hydrolysis

Implementation Method 3

a saturated solution is formed which leads to a network of oligomers that undergo polycondensation to form a three-dimensional network of aluminosilicates

Methodology Applied
Scientific EffectPolycondensation: Chemical Bonding

Implementation Method 4

The geopolymerization reaction releases heat to drive the formation of the geopolymer product

Methodology Applied
Scientific EffectExothermic reaction: Exothermic Reaction

Data Source

PatentEP3262008B1Particulate compositions for the formation of geopolymers, their use and methods for forming geopolymers therewith
Publication Date: 2020.12.16 IMERTECH SAS
  • EP3262008B1 patent drawingFigure 1

AI summary

The present invention relates to dry particulate composition for forming a geopolymer, comprising an alkali metal hydroxide, an alkali metal silicate, and an aluminosilicate. The invention further relates to methods for forming geopolymers and geopolymers formed according to said methods or using the said dry particulate compositions.