Dynamically Crosslinked Thermoplastic Elastomer Recycling

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Solution Overview

Problem

Existing crosslinked rubbers and thermoset materials are difficult to recycle, leading to increased manufacturing costs due to scrap materials generated during production, and there is a need for recyclable products after their useful life.

Innovation Solution

A method of creating dynamically crosslinked thermoplastic materials by partially crosslinking an elastomer composition and then mixing it with a thermoplastic polymer composition at a higher temperature to form a dispersed phase of crosslinked elastomer domains within a thermoplastic matrix, preventing the transfer of non-polymeric components and allowing for further shaping and recycling.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If crosslinked rubbers and thermoset materials are used to achieve excellent physical properties, then resilience and durability are improved, but recyclability deteriorates

Engineering Contradiction:
ImproveresilienceVSAvoidrecyclability
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes the chemical state of the elastomer from fully crosslinked (thermoset) to dynamically crosslinked (thermoplastic), allowing the material to transition between solid and melt states. This parameter change enables both excellent physical properties when solid and recyclability when melted, resolving the contradiction between resilience and recyclability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system combining thermoplastic resin matrix with dynamically crosslinked elastomer domains. This composite structure allows the material to exhibit both the resilience of crosslinked rubbers and the recyclability of thermoplastics, as the thermoplastic matrix can be remelted and reprocessed

Inventive Principle:
Principle #40Composite materials

2Reliability

If crosslinked rubbers and thermoset materials are used to achieve excellent physical properties, then durability is improved, but manufacturing cost increases due to scrap materials

Engineering Contradiction:
ImprovedurabilityVSAvoidscrap material
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

By changing the material from thermoset to dynamically crosslinked thermoplastic, the patent enables scrap material to be remelted and reprocessed multiple times without degradation, eliminating waste and reducing manufacturing costs while maintaining durability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent enables recovery and reuse of scrap material through remelting and reprocessing, converting what would be discarded waste into reusable feedstock, thereby reducing loss of substance and manufacturing cost

Inventive Principle:
Principle #34Discarding and recovering

3Ease of manufacture

If thermoplastic resin and rubber are melt mixed and cured to form dynamically crosslinked materials, then recyclability is improved, but component transfer between phases occurs

Engineering Contradiction:
ImproverecyclabilityVSAvoidcomponent transfer
Core Design Contradiction:
Ease of manufactureVSStability of the object's composition

Solution Approach 1:

The patent applies preliminary crosslinking to the elastomer before mixing with thermoplastic resin, creating stable elastomer domains that resist component transfer during subsequent processing and recycling, thus maintaining compositional stability while enabling recyclability

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent uses the crosslinked elastomer domains as intermediaries that prevent direct contact and transfer between thermoplastic components, acting as a barrier that maintains compositional stability during recycling processes

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting dynamically crosslinked thermoplastic materials exhibit excellent physical properties, including resilience, thermal properties, and sound dampening, with the ability to be recycled, reducing waste and manufacturing costs.

Implementation Method 1

partially crosslinking an elastomer composition at a first crosslinking temperature to form a thermoplastic, partially crosslinked elastomer composition

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

heating the thermoplastic polymer composition and the thermoplastic, partially crosslinked elastomer composition to a second crosslinking temperature higher than the first crosslinking temperature

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 3

wherein the thermoplastic polymer composition is liquid at the second crosslinking temperature

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 4

continuously mixing the mixture while further crosslinking the elastomer composition to form a thermoplastic material having a dispersed phase of crosslinked elastomer composition in the thermoplastic polymer composition

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Data Source

PatentEP3046951B8Dynamically crosslinked thermoplastic material process
Publication Date: 2017.12.06 FENG TAY ENTERPRISE CO LTD

AI summary

A method for making a thermoplastic material includes: (a) partially crosslinking an elastomer composition at a first crosslinking temperature to form a thermoplastic, partially crosslinked elastomer composition; (b) mixing a thermoplastic polymer composition with the thermoplastic, partially crosslinked elastomer composition and heating the mixture to a second crosslinking temperature higher than the first crosslinking temperature, wherein the thermoplastic polymer composition is liquid at the second crosslinking temperature; and (c) continuously mixing the mixture while further crosslinking the elastomer composition to form a thermoplastic material having a dispersed phase of crosslinked elastomer composition in the thermoplastic polymer composition. The elastomer composition may include an elastomer compounded with a curing agent and optionally additional components. A thermoplastic material resulting from this process may be molded or shaped by any method used for forming thermoplastic materials into articles, such as molding, extrusion, or thermoforming.