Electrochemical device and method for adjusting carbon dioxide concentration in indoor atmospheres

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Solution Overview

Problem

Current methods for reducing carbon dioxide concentrations in indoor air are energy-intensive and inefficient, with high energy costs associated with frequent ventilation and existing regenerative CO2 removal systems, which also generate heat and have limitations in continuous processing.

Innovation Solution

An electrochemical device with a cathode and anode chamber separated by a solid electrolyte membrane, using a polymerized ionic liquid membrane to transport ionic carrier species, allowing for continuous and efficient CO2 removal or addition to indoor air at low temperatures and power consumption.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If regenerative CO2 removal systems using absorbents are used, then CO2 can be removed from indoor air, but the system becomes heavy and requires high temperature heating for regeneration

Engineering Contradiction:
ImproveCO2 removal capacityVSAvoidabsorbent volume
Core Design Contradiction:
Quantity of substanceVSWeight of stationary object

Solution Approach 1:

The patent replaces the thermal regeneration mechanism with an electrochemical mechanism. Instead of heating absorbents to high temperatures to release CO2, the invention uses electrochemical reactions at electrodes to continuously remove CO2 through a membrane, substituting mechanical/thermal processes with electrochemical ones.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The invention changes the operating parameters from high temperature (above 150°C) to ambient or low temperatures by using electrochemical potentials. The electrochemical cell operates at much lower temperatures than thermal regeneration systems, fundamentally changing the temperature parameter of the CO2 removal process.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If regenerative absorbent systems are used, then CO2 can be removed, but continuous processing is limited and large heat is generated

Engineering Contradiction:
ImproveCO2 removalVSAvoidheat generation
Core Design Contradiction:
Quantity of substanceVSLoss of energy

Solution Approach 1:

The patent replaces the thermal cycle of absorbent regeneration with a continuous electrochemical process. The electrochemical cell continuously converts CO2 to carbonate ions at the cathode and regenerates the carrier at the anode without requiring thermal input, eliminating the heat generation problem of regenerative systems.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The electrochemical system enables continuous CO2 removal through uninterrupted electrochemical reactions. Unlike batch regenerative systems that require periodic heating cycles, the electrochemical cell operates continuously with constant ion transport through the membrane, maintaining steady-state CO2 removal without interruption.

Inventive Principle:
Principle #20Continuity of useful action

3Reliability

If frequent ventilation is used to maintain CO2 levels, then indoor air quality can be maintained, but energy cost becomes quite high

Engineering Contradiction:
Improveindoor air qualityVSAvoidventilation energy cost
Core Design Contradiction:
ReliabilityVSUse of energy by stationary object

Solution Approach 1:

The patent extracts and removes only the CO2 component from indoor air using the electrochemical cell, rather than replacing all indoor air through ventilation. The system selectively removes CO2 through electrochemical reactions while recirculating the bulk air, extracting the harmful component without the energy cost of full air replacement.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the approach from bulk air exchange to selective component removal. Instead of changing the entire air composition through ventilation, the electrochemical system specifically targets and removes CO2 molecules through electrochemical conversion to carbonate ions, fundamentally changing the parameter of what is being treated.

Inventive Principle:
Principle #35Parameter changes

4Quantity of substance

If electrochemical methods with quinone carriers are used, then CO2 removal can be achieved, but oxygen stability is poor and CO2 removal flux is low

Engineering Contradiction:
ImproveCO2 removal fluxVSAvoidoxygen stability
Core Design Contradiction:
Quantity of substanceVSStability of the object's composition

Solution Approach 1:

The patent uses a composite membrane system combining a polymer matrix with ionic liquid or ion-exchange functional groups. This composite structure provides both the mechanical integrity needed for stability and the ionic conductivity required for high CO2 flux, while the polymer backbone offers oxygen stability that simple quinone carriers lack.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The electrochemical device enables continuous, energy-efficient CO2 removal or addition, reducing energy consumption and thermal load, while maintaining indoor air quality, and can be integrated into HVAC systems for widespread application.

Implementation Method 1

A reduction catalyst layer in the cathode chamber reduces carbon dioxide in the gas to form an ionic carrier species

Methodology Applied
Scientific EffectElectrochemical reduction: Electrolysis

Implementation Method 2

The membrane includes a polymerized ionic liquid. The membrane transports the ionic carrier species between the cathode chamber and the anode chamber when a voltage difference is applied across the membrane

Methodology Applied
Scientific EffectIonic transport: Ion Exchange

Implementation Method 3

An oxidation catalyst layer in the anode chamber oxidizes the ionic carrier species to form carbon dioxide

Methodology Applied
Scientific EffectElectrochemical oxidation: Oxidation

Data Source

PatentEP3372298B1Electrochemical device and method for adjusting carbon dioxide concentration in indoor atmospheres
Publication Date: 2021.08.25 PALO ALTO RESEARCH CENTER INC
  • EP3372298B1 patent drawingFigure 1
  • EP3372298B1 patent drawingFigure 2
  • EP3372298B1 patent drawingFigure 3

AI summary

An electrochemical device suited to modifying a carbon dioxide concentration in an interior space includes a cathode chamber with an inlet which receives a feed gas containing carbon dioxide. A reduction catalyst layer in the cathode chamber reduces carbon dioxide in the gas to form an ionic carrier species. An anode chamber with an outlet outputs a gas comprising carbon dioxide. A solid electrolyte membrane spaces the anode chamber from the cathode chamber and transports the ionic carrier species between the cathode chamber and the anode chamber. The membrane includes an ionic liquid. An oxidation catalyst layer in the anode chamber oxidizes the ionic carrier species to form carbon dioxide. A voltage source provides a voltage difference across the membrane.