Battery Electrode Binder Composition for Stable Slurry Viscosity

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Solution Overview

Problem

Conventional binder compositions for non-aqueous secondary battery electrodes face challenges in maintaining viscosity stability and achieving high peel strength, particularly during long-term storage and electrode formation.

Innovation Solution

A binder composition incorporating a particulate polymer with specific chemical composition and particle properties, including aromatic vinyl, conjugated diene, and acidic group-containing monomer units, with acidic groups partially in the form of salts, and controlled particle diameters, is used to enhance viscosity stability and peel strength.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If a conventional binder composition is used, then the slurry composition can be produced, but the viscosity stability deteriorates during long-term storage

Engineering Contradiction:
Improveviscosity stabilityVSAvoidstorage time
Core Design Contradiction:
Stability of the object's compositionVSDuration of action of stationary object

Solution Approach 1:

The invention changes the particle size parameters of the particulate polymer (average particle diameter X: 140-300 nm, particle diameter ratio X/Y: 1.05-2.00) to achieve optimal viscosity stability. By controlling these physical parameters within specific ranges, the binder composition maintains stable viscosity during long-term storage while ensuring proper adhesion and processing characteristics.

Inventive Principle:
Principle #35Parameter changes

2Strength

If a binder composition with strong adhesion is used, then peel strength increases, but viscosity stability may deteriorate

Engineering Contradiction:
Improvepeel strengthVSAvoidviscosity stability
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The invention optimizes the chemical composition parameters of the particulate polymer, specifically controlling the content of aromatic vinyl monomer units (5-40 mass%), conjugated diene monomer units (20-70 mass%), and acidic group-containing monomer units (0.1-10 mass%). This parameter optimization achieves a balance between adhesion strength and viscosity stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite particulate polymer structure combining multiple monomer units with different functions: aromatic vinyl units for structural backbone, conjugated diene units for flexibility and adhesion, and acidic group-containing units for polarity and bonding. This composite structure enables simultaneous achievement of high peel strength and viscosity stability.

Inventive Principle:
Principle #40Composite materials

3Strength

If the particle size of the particulate polymer is reduced, then the adhesion improves, but the viscosity control becomes difficult

Engineering Contradiction:
ImproveadhesionVSAvoidviscosity control
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The invention precisely controls the particle size parameters (average diameter X: 140-300 nm, ratio X/Y: 1.05-2.00) to achieve optimal balance between adhesion and viscosity control. This specific particle size range provides sufficient surface area for adhesion while maintaining appropriate flow characteristics.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The proposed binder composition achieves excellent viscosity stability and peel strength for non-aqueous secondary battery electrodes, ensuring effective adhesion and performance over time.

Implementation Method 1

a binder composition containing a binder does not cause the viscosity of a slurry composition produced used the binder composition to significantly increase or decrease from designed viscosity straight after production even in a situation in which the slurry composition is stored for a long time

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 2

it is desirable that a binder composition containing a binder does not cause the viscosity of a slurry composition produced used the binder composition to significantly increase or decrease from designed viscosity straight after production even in a situation in which the slurry composition is stored for a long time

Methodology Applied
Scientific EffectViscosity stability:

Data Source

PatentUS20250006936A1Binder composition for non-aqueous secondary battery electrode, slurry composition for non-aqueous secondary battery electrode, electrode for non-aqueous secondary battery, and non-aqueous secondary battery
Publication Date: 2025.01.02 ZEON CORP

AI summary

Provided is a binder composition for a non-aqueous secondary battery electrode with which it is possible to produce a slurry composition that has excellent viscosity stability and is capable of producing an electrode having excellent peel strength. The binder composition contains a particulate polymer and water. The particulate polymer includes an aromatic vinyl monomer unit, a conjugated diene monomer unit, and an acidic group-containing monomer unit, wherein an acidic group of the acidic group-containing monomer unit is at least partially in a form of a salt. The particulate polymer has an average particle diameter X according to cumulant method analysis as measured by dynamic light scattering of 140 nm to 300 nm. A particle diameter ratio X/Y calculated as a ratio of the average particle diameter X relative to a volume-average particle diameter Y of the particulate polymer measured by laser diffraction/scattering is 1.05 to 2.00.