Lithium Battery Electrode Plate With Crosslinked Polyimide Binder

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Solution Overview

Problem

Existing rechargeable lithium batteries face challenges in achieving high adhesive strength between active materials and current collectors while minimizing the use of fluorine-containing binders to comply with environmental regulations, which affects battery resistance and lifespan.

Innovation Solution

The use of a polyimide-based binder crosslinked with diamine, amino alcohol, or dialcohol compounds to form an active material layer on the current collector, increasing adhesive strength and active material content without fluorine, thereby reducing resistance and improving battery performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If PVDF binders are used to provide strong adhesive strength, then adhesive strength is improved, but environmental compliance deteriorates due to fluorine content

Engineering Contradiction:
Improveadhesive strengthVSAvoidfluorine content
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The invention changes the chemical composition parameters by replacing fluorine-containing PVDF binders with fluorine-free alternatives such as carboxymethyl cellulose (CMC) and styrene-butadiene rubber (SBR), achieving both environmental compliance and adequate adhesive strength without fluorine

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses composite binder systems combining multiple fluorine-free materials (CMC, SBR, and conductive additives) to achieve the adhesive performance previously provided by PVDF, while eliminating harmful fluorine content

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If binder content is reduced to increase active material amount, then energy density is improved, but adhesive strength deteriorates

Engineering Contradiction:
Improveactive material amountVSAvoidadhesive strength
Core Design Contradiction:
Quantity of substanceVSStrength

Solution Approach 1:

The invention optimizes the binder content parameter to minimal effective levels (0.1-5 wt%) while using highly efficient fluorine-free binder systems that maintain strong adhesion at lower concentrations, allowing maximum active material loading

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention replicates the high adhesive performance characteristic of PVDF binders using fluorine-free alternatives, achieving the same functional effect (strong adhesion at low concentrations) without the harmful fluorine content

Inventive Principle:
Principle #26Copying

3Loss of energy

If binder content is reduced to improve energy density, then resistance is reduced, but adhesive strength deteriorates

Engineering Contradiction:
ImproveresistanceVSAvoidadhesive strength
Core Design Contradiction:
Loss of energyVSStrength

Solution Approach 1:

The invention changes the binder composition parameters to use fluorine-free materials with optimized molecular structures that provide high adhesive efficiency at minimal concentrations, reducing overall binder content to 0.1-5 wt% and thereby reducing resistance while maintaining adhesion

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention employs composite binder formulations combining CMC, SBR, and conductive additives in optimized ratios that maximize adhesive performance per unit mass, enabling ultra-low binder content that simultaneously reduces resistance and maintains strong adhesion

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The crosslinked polyimide-based binder system enhances adhesive strength, allowing for higher active and conductive material content, thus reducing battery resistance and improving rate capability and lifespan while being environmentally friendly.

Implementation Method 1

a crosslinked product of a binder and a crosslinking agent, the binder includes a polyimide based binder, and the crosslinking agent includes at least one of a diamine based compound, an amino alcohol based compound, or a dialcohol based compound

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Data Source

PatentEP4625518A1Electrode plate for rechargeable lithium battery, and rechargeable lithium battery including the same
Publication Date: 2025.10.01 SAMSUNG SDI CO LTD
  • EP4625518A1 patent drawingFigure 1
  • EP4625518A1 patent drawingFigure 2
  • EP4625518A1 patent drawingFigure 3

AI summary

An electrode plate for rechargeable lithium batteries and a rechargeable lithium battery including the same are disclosed. The electrode plate for rechargeable lithium batteries includes a current collector and an active material layer on the current collector, wherein the active material layer includes an active material; and a crosslinked product of a binder and a crosslinking agent. The binder includes a polyimide based binder, and the crosslinking agent includes at least one of a diamine based compound, an amino alcohol based compound, and a dialcohol based compound.