Integrated Electrolytic Device for Gas Recombination

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Solution Overview

Problem

Existing electrolytic devices for ion chromatography struggle with simultaneous electrolysis and catalytic gas elimination, requiring external columns and platinum catalysts, which increase operational resistance, wattage, and noise, and can damage ion exchange components due to hydrogen peroxide formation.

Innovation Solution

An electrolytic device with at least two flow-through channels separated by charged ion-exchange membranes, incorporating a catalyst in two channels to recombine hydrogen and oxygen gases into water, reducing the need for external columns and lowering operational resistance by using alternating current to constantly reverse electrolytic water splitting reactions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If external columns and platinum catalysts are used for catalytic gas elimination, then hydrogen and oxygen recombination is achieved, but operational resistance and wattage increase

Engineering Contradiction:
Improvecatalytic gas eliminationVSAvoidoperational wattage
Core Design Contradiction:
ReliabilityVSUse of energy by stationary object

Solution Approach 1:

The patent combines the electrolytic device and catalytic gas elimination function into a single integrated device. The electrolytic cell generates hydrogen and oxygen gases through water splitting, while the same device incorporates a catalyst (such as platinum-coated porous material or ion-exchange resin with platinum) that catalytically recombines these gases back into water. This merging eliminates the need for separate external columns and reduces operational resistance and energy consumption.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent uses an intermediary substance (catalyst such as platinum-coated porous material or ion-exchange resin impregnated with platinum) that facilitates the catalytic recombination of hydrogen and oxygen gases. This intermediary enables the gas elimination function without requiring high energy input, as the catalyst lowers the activation energy barrier for the recombination reaction.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Reliability

If external columns and platinum catalysts are used for catalytic gas elimination, then hydrogen and oxygen recombination is achieved, but device complexity increases

Engineering Contradiction:
Improvecatalytic gas eliminationVSAvoiddevice structure
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent merges the electrolytic cell structure with the catalytic gas elimination function into a single integrated device. The electrolytic cell contains electrodes for water splitting and also incorporates catalyst-containing porous material or ion-exchange resin that performs catalytic recombination. This integration eliminates the need for separate external columns and reduces structural complexity.

Inventive Principle:
Principle #5Merging (Combining)

3Reliability

If catalyst is used for gas recombination, then hydrogen and oxygen are converted to water, but hydrogen peroxide formation can damage ion exchange components

Engineering Contradiction:
Improvegas recombination efficiencyVSAvoidhydrogen peroxide damage
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent optimizes catalytic reaction parameters (such as catalyst composition, surface area, and reaction conditions) to favor the formation of water over hydrogen peroxide. By controlling the catalytic recombination process, the device minimizes the formation of harmful hydrogen peroxide while maintaining efficient gas conversion.

Inventive Principle:
Principle #35Parameter changes

4Use of energy by stationary object

If alternating current is used to reverse electrolytic reactions, then operational resistance is lowered, but control complexity increases

Engineering Contradiction:
Improveoperational resistanceVSAvoidcontrol system
Core Design Contradiction:
Use of energy by stationary objectVSDevice complexity

Solution Approach 1:

The patent employs alternating current to periodically reverse the electrolytic water splitting reactions. During one half-cycle, water is split into hydrogen and oxygen; during the reverse half-cycle, the catalyst facilitates recombination back into water. This periodic action prevents gas accumulation, lowers operational resistance, and reduces energy consumption without requiring complex control systems beyond standard AC power supply.

Inventive Principle:
Principle #19Periodic action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables efficient simultaneous electrolysis and catalytic gas elimination, reducing operational wattage, noise, and minimizing hydrogen peroxide concentration, thereby protecting ion exchange components and improving suppression efficiency.

Implementation Method 1

separated by a first charged barrier having exchangeable ions capable of passing ions of only one charge, positive or negative, and of blocking bulk liquid flow

Methodology Applied
Scientific EffectIon exchange: Ion Exchange

Implementation Method 2

A catalyst is packed in the first and third channels for combining hydrogen and oxygen gas and removing hydrogen peroxide

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

The catalyst can remove hydrogen peroxide by the decomposition of hydrogen peroxide into water and oxygen

Methodology Applied
Scientific EffectCatalytic decomposition: Catalysis

Implementation Method 4

Electrolytic devices generate electrolytic gases from the water splitting reactions when a DC potential in excess of about 1.5 volts is applied

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Data Source

PatentEP2881496B1Gas-less electrolytic device and method
Publication Date: 2020.08.19 DIONEX CORP
  • EP2881496B1 patent drawingFigure 1
  • EP2881496B1 patent drawingFigure 2
  • EP2881496B1 patent drawingFigure 3

AI summary

An electrolytic device, e.g. a suppressor, including at least two flow-through channels separated by a charged membrane barrier, and a catalyst, for combining hydrogen and oxygen gas, together with ion exchange material, disposed in one of the channels. Also, a method for simultaneous electrolysis and catalytic gas elimination in a channel of the device is described.