Embolization Particles with Metal Oxide Nanoparticles for Deep Tumor Treatment

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Solution Overview

Problem

Current cancer treatment methods, such as radiotherapy and photodynamic therapy, face limitations in penetrating deep tissues and are ineffective against hypoxic tumor cells, while embolization techniques struggle to simultaneously occlude blood vessels and deliver radiotherapeutic agents effectively.

Innovation Solution

Development of multimodal embolization particles coated with metal oxide nanoparticles doped with rare earth elements, specifically titanium dioxide, zinc oxide, or cerium dioxide, which can be excited by X-ray or proton beam radiation to generate reactive oxygen species (ROS) under both normoxic and hypoxic conditions, allowing for simultaneous embolization and radiotherapeutic treatment of tumors.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If photodynamic therapy is used to treat cancer, then superficial cancers can be treated with photosensitizing agents and light exposure, but the treatment cannot penetrate deep into the body and is limited to superficial cancers

Engineering Contradiction:
Improvelight penetration depthVSAvoidtreatment applicability to deep tumors
Core Design Contradiction:
Illumination intensityVSAdaptability or versatility

Solution Approach 1:

The patent combines embolization particles with metal oxide nanoparticles into a single multimodal particle system. The embolization component occludes blood vessels while the metal oxide nanoparticles generate ROS under X-ray or proton beam radiation, integrating two therapeutic functions into one particle that can treat deep-seated tumors effectively

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent replaces the light-based activation mechanism of photodynamic therapy with X-ray or proton beam radiation activation. This substitution enables deeper tissue penetration since ionizing radiation can reach deep tumors, and the metal oxide nanoparticles convert this radiation energy into ROS for therapeutic effect

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Reliability

If radiotherapy is used to treat radioresistant cancers such as renal cell cancer, then high doses of radiation are required to destroy the cancer, but these high doses increase the risk of causing cancer and are too high to be safe in clinical practice

Engineering Contradiction:
Improvecancer destruction efficacyVSAvoidradiation safety and secondary cancer risk
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent creates localized ROS generation at the tumor site through metal oxide nanoparticles that are selectively delivered via embolization. The ROS are generated only where the nanoparticles accumulate in the tumor vasculature and are activated by targeted X-ray or proton beam radiation, concentrating the therapeutic effect locally while minimizing exposure to healthy tissues

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The metal oxide nanoparticles act as intermediaries that convert X-ray or proton beam radiation energy into reactive oxygen species. This intermediary mechanism allows the use of lower doses of ionizing radiation compared to conventional radiotherapy, as the nanoparticles amplify the biological effect through ROS generation, thereby reducing the harmful effects of high-dose radiation

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If conventional embolization particles are used to occlude blood vessels, then blood flow to the tumor is restricted, but the particles cannot simultaneously generate radiotherapeutic effects under hypoxic conditions

Engineering Contradiction:
Improveembolization efficacyVSAvoidradiotherapeutic functionality
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent merges embolization particles with metal oxide nanoparticles to create a single multimodal particle that performs both embolization and radiotherapeutic functions. The embolization component occludes tumor blood vessels while the metal oxide nanoparticles provide ROS generation capability under X-ray or proton beam radiation, including under hypoxic conditions where conventional radiotherapy fails

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The multimodal embolization particle with metal oxide nanoparticles serves multiple functions: it embolizes tumor vasculature to restrict blood flow, delivers metal oxide nanoparticles to the tumor site, and generates ROS under X-ray or proton beam radiation even under hypoxic conditions. This multi-functionality overcomes the limitations of conventional single-function embolization particles

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The embolization particles effectively occlude tumor vasculature and generate ROS to treat cancer cells under hypoxic conditions, enhancing the efficacy of radiotherapy and improving treatment outcomes by combining embolization with radiotherapeutic effects.

Implementation Method 1

nanoparticles which comprise a metal oxide doped with one or more rare earth elements, wherein the metal oxide is titanium dioxide, zinc oxide or cerium dioxide... can be excited by X-ray or proton beam radiation to generate reactive oxygen species (ROS)

Methodology Applied
Scientific EffectRadiation-induced ROS generation: Radiation

Implementation Method 2

The agent is absorbed by cells all over the body, but it generally accumulates in the tumour due to abnormalities or defects in the tumour vasculature. It is also rapidly absorbed by cancer cells, which tend to grow and divide much more quickly than healthy cells and hence have a higher metabolic activity.

Methodology Applied
Scientific EffectAccumulation in tumour tissue: Absorption (physical)

Implementation Method 3

The photosensitizing agent that has accumulated in the tumour is excited by exposure to this light and reacts with nearby oxygen or water molecules in the tissue to produce reactive oxygen species (ROS), such as singlet oxygen... a superoxide radical... or a hydroxyl radical

Methodology Applied
Scientific EffectPhotoexcitation and ROS production: Photo-oxidation

Implementation Method 4

It is believed that the titanium dioxide particles produce hydroxyl radicals that oxidize the membrane lipids of the cells to produce peroxidants, which then set up a series of peroxidant chain reactions. The oxidatively stressed malignant cells progress to a necrotic state that results in their destruction.

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP3283134B1Embolization particle
Publication Date: 2019.07.03 OXFORD UNIVERSITY INNOVATION LTD
  • EP3283134B1 patent drawingFigure 1
  • EP3283134B1 patent drawingFigure 2~3
  • EP3283134B1 patent drawingFigure 4

AI summary

The present invention relates to an embolization particle comprising a microparticle coated with a plurality of nanoparticles, which nanoparticles comprise a metal oxide doped with one or more rare earth elements, wherein the metal oxide is titanium dioxide, zinc oxide or cerium dioxide. An embolization particle of the invention for use in the treatment of cancer in combination with X-ray radiation or proton beam radiation, or use in embolization, is also described. The invention also relates to a process for producing an embolization particle comprising a microparticle coated with a plurality of nanoparticles, which nanoparticles comprise a metal oxide doped with one or more rare earth elements, wherein the metal oxide is titanium dioxide, zinc oxide or cerium dioxide, which process comprises: (i) providing a microparticle; (ii) contacting the microparticle with a plurality of the nanoparticles; and (iii) heating the microparticle and the nanoparticles to form the embolization particle.