Encapsulated Lithium Particles for Stable Electrochemical Storage

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Solution Overview

Problem

Lithium metal is unstable and reactive, posing safety concerns and limiting its shelf life due to its flammability in oxygen-containing environments and moisture, which complicates its use in electrochemical devices like lithium ion capacitors.

Innovation Solution

Encapsulated lithium particles with a lithium metal core coated in a shell comprising a lithium salt, oil, and optional binder are developed, providing stability against oxygen and moisture, and can be easily integrated into electrodes using a single-step coating method at lower temperatures.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Use of energy by moving object

If lithium metal is used directly in electrochemical devices, then high energy density is achieved, but stability and safety deteriorate due to flammability in oxygen-containing environments and moisture

Engineering Contradiction:
Improveenergy densityVSAvoidstability and safety
Core Design Contradiction:
Use of energy by moving objectVSReliability

Solution Approach 1:

The patent creates a composite structure where lithium metal particles are coated with a shell comprising lithium salt, oil, and optional binder. This composite encapsulation provides both the high energy density of lithium metal and the stability/safety of the protective shell, resolving the contradiction between energy density and reliability

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The shell coating creates an inert protective environment around the lithium metal particles, shielding them from oxygen and moisture in the external environment. This allows the lithium metal to maintain its high energy density while the inert shell ensures stability and safety during storage and handling

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

2Reliability

If lithium metal is stabilized through coating, then stability against oxygen and moisture is improved, but device complexity increases

Engineering Contradiction:
Improvestability against oxygen and moistureVSAvoidstructure complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent employs a thin film shell coating composed of lithium salt, oil, and optional binder that encapsulates the lithium metal particles. This thin film approach provides effective protection against oxygen and moisture while adding minimal structural complexity, maintaining simplicity in the overall device design

Inventive Principle:
Principle #30Flexible shells and thin films

Solution Approach 2:

The shell coating serves multiple functions simultaneously: it provides protection against oxygen and moisture, enables safe handling of lithium metal, and maintains compatibility with electrochemical cell chemistry. This multi-functionality reduces the need for additional separate components, thereby limiting the increase in device complexity

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Ease of operation

If lithium metal is handled without encapsulation, then ease of operation is maintained, but harmful factors increase due to flammability and reactivity

Engineering Contradiction:
Improvehandling easeVSAvoidflammability and reactivity
Core Design Contradiction:
Ease of operationVSObject-generated harmful factors

Solution Approach 1:

The shell coating acts as an intermediary layer between the lithium metal particles and the external environment. This intermediary shell comprises lithium salt, oil, and optional binder, providing a safe interface that allows easy handling of lithium metal while preventing direct contact between the reactive lithium and oxygen/moisture, thereby eliminating flammability and reactivity hazards

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The encapsulated lithium particles enhance the stability and safety of lithium metal, allowing for reliable handling and integration into devices, improving discharge rate performance and extending storage stability, while maintaining compatibility with electrochemical cell chemistry.

Implementation Method 1

Encapsulated lithium particles with a lithium metal core coated in a shell comprising a lithium salt, oil, and optional binder are developed, providing stability against oxygen and moisture

Methodology Applied
Scientific EffectEncapsulation: Physical Containment

Implementation Method 2

can be easily integrated into electrodes using a single-step coating method at lower temperatures

Methodology Applied
Scientific EffectCoating: Coatings

Data Source

PatentEP3198671B1Encapsulated lithium particles and methods of making and use thereof
Publication Date: 2019.10.23 CORNING INC
  • EP3198671B1 patent drawingFigure 1A
  • EP3198671B1 patent drawingFigure 1B
  • EP3198671B1 patent drawingFigure 2A~2B

AI summary

An encapsulated lithium particle (100) including: • a core (110) comprised of at least one of: lithium; a lithium metal alloy; or a combination thereof; and • a shell (120) comprised of a lithium salt, an oil, and optionally a binder, and • the shell encapsulates the core, and the particle size is from 10 to 500 microns. Also, disclosed is a method of making the particle and using the particle in electrical devices such as a capacitor or a battery.