Epsilon-Phase Magnetic Powder With Controlled Coercivity Distribution

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Magnetic powders containing ε-Fe2O3 used in magnetic recording media suffer from signal decay due to the presence of superparamagnetic components, which affect durability and magnetic properties, despite efforts to control particle size and magnetic properties through ultrafiltration and crystal structure management.

Innovation Solution

Development of magnetic powders with epsilon-phase iron oxide-based compounds, specifically ε-AaFe2-aO3, with controlled particle diameters and magnetic field ratios, and a manufacturing method involving trivalent iron ions, alkali agents, polyvalent carboxylic acids, and heat treatment to minimize amorphous components and enhance magnetic properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If particle size distribution is narrowed and magnetic properties are adjusted to meet specifications, then magnetic properties are improved, but signal decay occurs and durability deteriorates

Engineering Contradiction:
Improveparticle size distribution controlVSAvoidsignal decay resistance
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the physical and chemical parameters of the magnetic powder by controlling the crystal phase composition (specifically the ratio of epsilon-phase to other phases), particle size distribution (average diameter 8-25 nm with controlled fine particle content), and magnetic field ratios (Hc/Hc' between 0.6-1.0). These parameter changes achieve both improved magnetic properties and resistance to signal decay, resolving the contradiction between manufacturing precision and reliability.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If ultrafiltration is used to remove unnecessary ions, then purity is improved, but amorphous components increase and fine particles are generated

Engineering Contradiction:
Improveion purityVSAvoidamorphous component content
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent controls the chemical composition parameters during synthesis to achieve the desired purity while minimizing amorphous content. By optimizing the ratio of crystalline phases and controlling the particle size distribution through controlled synthesis conditions rather than post-synthesis ultrafiltration, the method achieves both ion purity and reduced amorphous component generation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent performs preliminary control of the synthesis conditions to pre-determine the crystal phase composition and particle size distribution before any purification steps. This preliminary action ensures that the magnetic powder achieves the desired properties during formation, avoiding the need for aggressive ultrafiltration that would generate amorphous components.

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If trivalent iron ion compounds are used to form magnetic powder precursor, then magnetic properties are improved, but amorphous portion increases

Engineering Contradiction:
Improvemagnetic property controlVSAvoidamorphous portion content
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent optimizes the chemical composition parameters by controlling the ratio of trivalent iron ions to other metal ions, the pH conditions during precipitation, and the heating temperature range (800-1400°C). These parameter changes enable the formation of desired magnetic properties through epsilon-phase crystal structure while minimizing amorphous content by ensuring complete crystallization.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent utilizes phase transition during heat treatment to convert the precursor material into the desired epsilon-phase crystal structure. By controlling the heating temperature and duration, the method ensures complete phase transformation from amorphous or other crystalline phases to the epsilon-phase, thereby reducing amorphous content while maintaining improved magnetic properties.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively prevents signal decay and improves magnetic properties by reducing superparamagnetic components, ensuring durability and performance in magnetic recording media.

Implementation Method 1

subjecting the magnetic powder precursor to heat treatment at a temperature condition of 800° C. to 1,400° C.

Methodology Applied
Scientific EffectHeat treatment: Heat Treatment

Implementation Method 2

in a case where a crystal structure is focused, the amount of an amorphous portion of metal powder increases, in a magnetic powder precursor formed under the conditions of a step of forming metal powder including iron

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

removing a silicic acid compound in the heat-treated magnetic powder precursor by using an alkali aqueous solution

Methodology Applied
Scientific EffectChemical dissolution:

Implementation Method 4

Magnetic powders containing ε-Fe2O3 used in magnetic recording media suffer from signal decay due to the presence of superparamagnetic components

Methodology Applied
Scientific EffectSuperparamagnetism: Superparamagnetism

Data Source

PatentUS12198841B2Magnetic powder, manufacturing method of magnetic powder, and magnetic recording medium
Publication Date: 2025.01.14 FUJIFILM CORP

AI summary

Magnetic powder includes: an epsilon-phase iron oxide-based compound selected from ε-Fe2O3 or a compound represented by Formula (1). The magnetic powder has an average particle diameter of 8 nm to 25 nm, a ratio of Hc to Hc′ of from 0.6 to 1.0, and Hc′ satisfying Expression (II). Hc′ represents a magnetic field at which a value of Expression (I) becomes zeroin a magnetic field-magnetization curve obtained by performing measurement at a maximum applied magnetic field of 359 kA/m, a temperature of 296 K, and a magnetic field sweeping speed of 1.994 kA/m/s. M represents magnetization and H represents applied magnetic field. Hc represents a magnetic field at which magnetization becomes zero in the magnetic field-magnetization curve. In Formula (1), A represents at least one metal element other than Fe, and a represents a number that satisfies a relationship of 0<a<2.d2M/dH2  Expression (I)119 kA/m<Hc′<2380 kA/m  Expression (II)ε-AxFe2-xO3  (1)