Ester Composition for Resin Processability

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Solution Overview

Problem

Existing eco-friendly plasticizers face challenges in processability and physical properties due to limitations in absorption rate and fusion time, particularly in sheet formulation and compound formulation of wires, automobile interior materials, films, sheets, tubes, wallpaper, toys, and floor materials.

Innovation Solution

A method for preparing an ester composition comprising hybrid branched type, non-hybrid unbranched type, and non-hybrid branched type alkyl-substituted terephthalate compounds through esterification reaction, with the hybrid branched type alkyl-substituted terephthalate compound present in specific amounts, using terephthalic acid, unbranched, and branched alcohols with acid catalysts at controlled temperatures and times.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If conventional eco-friendly plasticizers are used, then environmental friendliness is improved, but processability and physical properties deteriorate due to low absorption rate and long fusion time

Engineering Contradiction:
Improveenvironmental friendlinessVSAvoidabsorption rate and fusion time
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The patent applies parameter changes by precisely controlling the content of hybrid branched type alkyl-substituted terephthalate compound (1-70 wt%, preferably 10-50 wt%) in the ester composition. This specific compositional parameter optimization resolves the contradiction by achieving both environmental friendliness and improved processability with high absorption rate and short fusion time

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite plasticizer composition containing three types of ester compounds (hybrid branched type, non-hybrid unbranched type, and non-hybrid branched type alkyl-substituted terephthalates). This composite approach combines the environmental benefits of terephthalate-based plasticizers with improved processability through the specific hybrid branched component, resolving the contradiction between eco-friendliness and productivity

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If esterification reaction conditions are optimized for high conversion, then yield is improved, but reaction time and energy consumption increase

Engineering Contradiction:
Improveester composition yieldVSAvoidreaction time
Core Design Contradiction:
Quantity of substanceVSLoss of time

Solution Approach 1:

The patent optimizes multiple reaction parameters simultaneously: temperature (130-250°C), time (1-10 hours), and acid catalyst amount (0.1-15 parts by weight per 100 parts terephthalic acid). This multi-parameter optimization achieves high yield within reasonable time frames, resolving the contradiction between quantity and time loss

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses acid catalysts (paratoluenesulfonic acid, methanesulfonic acid, ethanesulfonic acid, propanesulfonic acid, or sulfuric acid) as intermediaries to accelerate the esterification reaction. These catalysts enable high conversion yields without requiring excessively long reaction times or extreme conditions, thus resolving the time-yield contradiction

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method enhances processability by achieving high absorption rates and short fusion times, resulting in superior physical properties and improved workability in resin compositions, such as those used in cables, automobile interior materials, films, sheets, tubes, wallpaper, and floor materials.

Implementation Method 1

the esterification reaction is carried out by reacting terephthalic acid, an unbranched alcohol and a branched alcohol using an acid catalyst at 130 to 250°C for 1 to 10 hours

Methodology Applied
Scientific EffectEsterification reaction: Chemical Bonding

Implementation Method 2

using an acid catalyst in the range of 0.1 to 15 parts by weight, with respect to 100 parts by weight of the terephthalic acid, and wherein the acid catalyst comprises at least one selected from the group consisting of paratoluenesulfonic acid, methanesulfonic acid, ethanesulfonic acid, propanesulfonic acid and sulfuric acid

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP2837646B1Method for manufacturing ester composition, and resin composition
Publication Date: 2017.08.30 LG CHEM LTD
  • EP2837646B1 patent drawingFigure 1
  • EP2837646B1 patent drawingFigure 2
  • EP2837646B1 patent drawing

AI summary

Disclosed are a method for preparing an ester composition and a resin composition comprising the ester composition. It is possible to suitably prepare a plasticizer composition which improves processability due to high absorption rate and short fusion time to resins and thus provides superior physical properties when processed with resins.