Esterification Unit Counter-Current Flow MMA Yield

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Solution Overview

Problem

Current industrial processes for producing methyl methacrylate (MMA) face challenges in achieving high yield and quality, with existing esterification methods resulting in low MMA concentration and high spent acid organic content, as well as reliability issues due to polymer fouling.

Innovation Solution

The proposed solution involves an improved esterification unit with a series of reactors configured for counter-current flow between gaseous and liquid phases, incorporating additional reactors in parallel to enhance reliability and using steam distribution for efficient mixing, along with specific reactor design and material selection to maintain high MMA concentration and reduce fouling.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional esterification methods are used, then the production process is simple, but the MMA concentration is low and spent acid organic content is high

Engineering Contradiction:
ImproveMMA concentrationVSAvoidreactor configuration
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The esterification unit is divided into multiple reactors (first reactor, second reactor, and optional third reactor) arranged in series. Each reactor performs a stage of the esterification process, allowing progressive conversion of methacrylamide to MMA. This segmentation enables higher overall MMA concentration (50-80 wt%) while managing the complexity through modular design with standardized reactor configurations.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent introduces a vertical dimension to the reaction process by implementing counter-current flow between gaseous phase (steam and MMA vapors) rising through the reactor and liquid phase (reactant mixture) flowing downward. This multi-dimensional flow pattern enhances mass and heat transfer efficiency, improving MMA concentration without requiring excessively large horizontal reactor volumes.

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

2Reliability

If conventional esterification units are used, then the process is easy to operate, but unplanned shut-downs due to fouling occur frequently

Engineering Contradiction:
Improveproduction continuityVSAvoidoperational complexity
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

Different reactors in the series are optimized for specific functions: the first reactor is designed to handle the initial esterification with appropriate steam injection, the second reactor continues the reaction with controlled liquid flow, and the optional third reactor provides additional conversion capacity. Each reactor has tailored operating parameters (temperature, steam flow, liquid flow rates) to minimize polymerization and fouling in critical zones, ensuring production continuity.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The series configuration of multiple reactors enables continuous operation without unplanned shut-downs. The counter-current flow system maintains continuous removal of MMA product from the reaction zone, preventing polymer accumulation and fouling. The system is designed for continuous steam injection and liquid flow, ensuring uninterrupted esterification process and reliable MMA production.

Inventive Principle:
Principle #20Continuity of useful action

3Productivity

If steam distribution is not used, then the mixing is simpler, but the esterification efficiency is lower

Engineering Contradiction:
Improveesterification yieldVSAvoidsteam distribution system
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent utilizes steam (gaseous phase) distributed through the liquid reaction mixture in the reactors to achieve efficient mixing and heat transfer. Steam is injected at the bottom of each reactor and rises through the downward-flowing liquid, creating intense turbulence and contact between phases. This pneumatic-hydraulic interaction enhances esterification yield to over 95% while the steam distribution system uses simple nozzles and natural buoyancy-driven flow, avoiding complex mechanical mixers or agitators.

Inventive Principle:
Principle #29Pneumatics and hydraulics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach achieves a yield of over 95% MMA with high concentration (50-80 wt%) and minimizes unplanned shut-downs due to fouling, ensuring reliable and efficient production with low organic content in spent acids.

Implementation Method 1

reactors are set up in a serial way so that there is a counter current flow between gaseous phase and liquid phase, the liquid phase flowing from first reactor (1) to last reactor (N or (N+1)), and the gaseous phase flowing from last reactor to first reactor

Methodology Applied
Scientific EffectCounter-current flow: Convection

Implementation Method 2

using steam distribution for efficient mixing

Methodology Applied
Scientific EffectSteam distribution: Sparging

Implementation Method 3

Gaseous phase distributor (90) located inside the lower part of reactor

Methodology Applied
Scientific EffectGas-liquid mixing: Turbulence

Implementation Method 4

esterification reaction of methacrylamide with at least a reactant to form methyl methacrylate

Methodology Applied
Scientific EffectEsterification reaction: Chemical Bonding

Data Source

PatentEP3057932B1Esterification unit for producing crude methyl methacrylate, esterification process using said unit and plant comprising said unit
Publication Date: 2022.06.22 TRINSEO EURO GMBH
  • EP3057932B1 patent drawingFigure 1
  • EP3057932B1 patent drawingFigure 2
  • EP3057932B1 patent drawingFigure 3

AI summary

The invention relates to an esterification unit (150) and esterification process for producing crude methyl methacrylate (MMA) from methacrylamide (MAM), which enable particularly to improve the yield, meaning that the organics spent acids are low; and at the same time, providing crude MMA with rather good quality, meaning that MMA concentration in crude MMA is rather high and preferably from 50wt% to 80wt%. According to the invention, the esterification unit comprises esterification reactors (1,..., 5 (or 6) set up in a serial way so that there is a counter current flow between gaseous phase and liquid phase, the liquid phase flowing from first reactor (1) of the series to last reactor (5 (or 6)), and the gaseous phase flowing from reactor to first reactor (1).