Ethylene-α-olefin-polyene copolymer processability

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Solution Overview

Problem

Conventional ethylene-α-olefin-nonconjugated polyene copolymers do not adequately satisfy both roll kneading processability and extrusion processability, which are essential for producing polymer compositions like rubber hoses.

Innovation Solution

An ethylene-α-olefin-nonconjugated polyene copolymer with specific molecular weight ratios, iodine values, and intrinsic viscosities is developed, incorporating ethylene, α-olefin, and nonconjugated polyene units, optimized for improved roll kneading and extrusion processability through precise polymerization conditions and catalyst composition.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If conventional ethylene-α-olefin-nonconjugated polyene copolymer is used, then basic polymer properties are maintained, but roll kneading processability and extrusion processability are insufficient

Engineering Contradiction:
Improveroll kneading processabilityVSAvoidprocessability consistency
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent applies parameter changes by precisely controlling multiple polymer properties including intrinsic viscosity (0.5-1.8 dl/g), molecular weight ratios (Mz/Mn: 15-25, Mw/Mn: 3-5), iodine value (1-50), and monomer composition ratios. These parameter optimizations resolve the contradiction by enabling both good roll kneading processability and extrusion processability simultaneously, which conventional polymers could not achieve.

Inventive Principle:
Principle #35Parameter changes

2Ease of operation

If polymer composition is optimized for roll kneading processability, then mixing ease improves, but extrusion processability deteriorates

Engineering Contradiction:
Improveroll kneading easeVSAvoidextrusion processability
Core Design Contradiction:
Ease of operationVSEase of manufacture

Solution Approach 1:

The patent resolves this contradiction through coordinated parameter changes: controlling intrinsic viscosity at 0.5-1.8 dl/g for kneading ease, while simultaneously optimizing Mz/Mn (15-25) and Mw/Mn (3-5) ratios for extrusion performance. The specific iodine value range (1-50) and monomer composition further balance these competing requirements.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polymer structure incorporating ethylene units, α-olefin units, and nonconjugated polyene units in specific ratios. This composite composition enables the material to exhibit both good roll kneading characteristics and extrusion processability, resolving the contradiction between these two manufacturing requirements.

Inventive Principle:
Principle #40Composite materials

3Strength

If molecular weight is increased to improve mechanical properties, then strength increases, but processability decreases

Engineering Contradiction:
Improvepolymer strengthVSAvoidprocessability
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The patent resolves this contradiction by changing molecular weight parameters strategically: controlling Mz/Mn ratio (15-25) and Mw/Mn ratio (3-5) to achieve a balanced molecular weight distribution. This enables the polymer to have sufficient strength while maintaining good processability in both roll kneading and extrusion operations.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentUS8962776B2Ethylene-α-olefin-nonconjugated polyene copolymer
Publication Date: 2015.02.24 SUMITOMO CHEM CO LTD

AI summary

Provided is an ethylene-α-olefin-nonconjugated polyene copolymer having ethylene units, α-olefin units and nonconjugated polyene units, wherein the copolymer satisfies the following requirements: (A): the intrinsic viscosity [η] is 0.5 to 1.8 dl/g, (B): the content of ethylene units is 50 to 90 mol % and the content of α-olefin units is 50 to 10 mol % where the sum total of the contents of ethylene units and α-olefin units is taken as 100 mol %, (C): the iodine value is 1 to 50, (D): the ratio of tan δ taken at 100° C. and 2 cpm to tan δ taken at 100° C. and 1000 cpm is from 1.0 to 1.7, and (E): the ratio of the Z-average molecular weight to the number average molecular weight is from 15 to 25 and the weight average molecular weight to the number average molecular weight is from 3 to 5.