Synergic EVA Copolymer Additives for Paraffin Crude Oil Pour Point Reduction

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Solution Overview

Problem

Current Pour Point Depressant additives for crude oils are inefficient in significantly lowering the gel point of paraffinic crude oils with high paraffin content, particularly those with a Pour Point above 10° C., due to limitations in co-crystallization with a wide range of paraffins and excessive crystal growth.

Innovation Solution

A synergic composition of ethylene-vinyl acetate (EVA) copolymers with different vinyl acetate comonomer contents, combined with a dispersing agent having a HLB>10, which co-crystallizes with paraffins and alters their crystalline structure, effectively lowering the Pour Point of paraffinic crude oils by widening the range of action and preventing crystal growth.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional single-grade EVA copolymers are used as Pour Point Depressants, then the additive can be dissolved in crude oil at suitable temperatures, but the gel point reduction is insufficient for crude oils with high paraffin content and PP above 10° C.

Engineering Contradiction:
Improvegel point reduction efficiencyVSAvoidrange of action over different paraffin types
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The invention divides the single EVA copolymer into multiple segments with different vinyl acetate contents (15-50% VA). Each segment (copolymer grade) targets specific paraffin crystal types, collectively providing comprehensive coverage across the entire paraffin spectrum, thereby resolving the insufficient gel point reduction for high paraffin content crude oils.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention creates a composite additive system by combining multiple EVA copolymer grades with different vinyl acetate contents and molecular weights. This composite approach synergistically interacts with various paraffin crystal structures, achieving superior gel point reduction compared to single-grade additives while maintaining solubility in crude oil.

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If additives are used at low concentrations to hinder paraffin crystallization, then economic costs are reduced, but the crystal growth is not sufficiently prevented for crude oils with high paraffin content

Engineering Contradiction:
Improveadditive concentrationVSAvoidcrystal growth prevention
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The invention optimizes the vinyl acetate content parameter across different copolymer grades (15-50% VA) to enhance interaction with paraffin crystals. This parameter variation allows the additive to effectively hinder crystal growth at low concentrations by improving the thermodynamic compatibility and interaction strength with paraffin structures.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

Different EVA copolymer grades with specific vinyl acetate contents are selectively effective against specific paraffin crystal types. The local quality of each copolymer grade (its specific VA content and molecular weight) is optimized for targeting particular crystal structures, enabling effective crystal growth prevention at low overall additive concentrations.

Inventive Principle:
Principle #3Local quality

3Ease of operation

If emulsions or suspensions containing dispersed polymers in aqueous/organic solvents are used, then the additives can be conveyed in crude oil, but the system complexity increases and additional solvents are required

Engineering Contradiction:
Improveadditive conveyance in crude oilVSAvoidsystem composition
Core Design Contradiction:
Ease of operationVSDevice complexity

Solution Approach 1:

The EVA copolymer additives are inherently soluble in crude oil without requiring external solvents or emulsifiers. The additive system serves itself by utilizing the crude oil medium directly for dissolution and transport, eliminating the need for complex emulsion or suspension formulations and reducing system complexity.

Inventive Principle:
Principle #25Self-service

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The synergic mixture of EVA copolymers with varying vinyl acetate contents and a surfactant achieves a significant reduction in the Pour Point of paraffinic crude oils, making them suitable for transportation and commercialization, with some achieving Pour Points below 0° C., even at low concentrations.

Implementation Method 1

The main action of these additives consists in co-crystallization with the paraffins present in the oil, altering/weakening their crystalline structure.

Methodology Applied
Scientific EffectCo-crystallization: Crystallisation

Implementation Method 2

a dispersing agent having a HLB>10, which co-crystallizes with paraffins and alters their crystalline structure

Methodology Applied
Scientific EffectDispersion: Dispersion (of waves)

Data Source

PatentUS10370607B2Compositions based on ethylene-vinyl acetate copolymers and their use as anti-gelling additives of paraffinic crude oils
Publication Date: 2019.08.06 VERSALIS OILFILED SOLUTIONS SRL

AI summary

A polymeric composition suitable for lowering the Pour Point of paraffinic crude oils comprising a synergic mixture including at least two ethylene-vinyl acetate copolymers respectively having an average molecular weight Mw lower than 130,000 Dalton (measured via GPC), a content of vinyl acetate monomer ranging from 15 to 50% by weight, with the proviso that the content of vinyl acetate monomer in the respective copolymers differs from one copolymer to another, by over 5%, on a weight basis.