Exfoliated Graphite Production via Polymer Grafting and Pyrolysis

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Solution Overview

Problem

Conventional methods for producing exfoliated graphite require complex steps and result in powdery materials that are difficult to handle, involving acid treatment and high-temperature processing.

Innovation Solution

A method involving the preparation of a composition with graphite and a polymer, where the polymer is grafted onto the graphite and then pyrolyzed to exfoliate it, increasing the specific surface area and improving handleability by creating a structure with increased interlayer distance and edge exfoliation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional acid treatment and high-temperature processing methods are used to exfoliate graphite, then exfoliated graphite can be obtained, but the production process becomes complex and the product becomes powdery and difficult to handle

Engineering Contradiction:
Improveexfoliation qualityVSAvoidproduction process complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent introduces an organic solvent as an intermediary medium to facilitate polymer grafting onto graphite surfaces. The solvent enables the polymer to interact with graphite in a controlled manner, allowing exfoliation to occur through polymer insertion rather than aggressive acid treatment, thus simplifying the production process while maintaining exfoliation quality

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the chemical parameters of the treatment process by using polymer-solvent systems instead of strong acids. This parameter change allows exfoliation to proceed under milder conditions, reducing process complexity and avoiding the formation of difficult-to-handle powdery products

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If conventional acid treatment methods are used to exfoliate graphite, then exfoliated graphite can be obtained, but the handling difficulty increases due to powdery product formation

Engineering Contradiction:
Improveexfoliation qualityVSAvoidproduct handleability
Core Design Contradiction:
Manufacturing precisionVSEase of operation

Solution Approach 1:

The patent creates a composite material structure where polymer chains are grafted onto graphite surfaces and extend into the solvent. This composite structure allows the exfoliated graphite to maintain structural integrity while being surrounded by polymer-solvent complexes, preventing powdery formation and improving handleability

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The organic solvent acts as a mediator that surrounds the exfoliated graphite structures, preventing them from aggregating into difficult-to-handle powders. The solvent-polymer-graphite complex maintains a structured form that is easier to handle while preserving the exfoliated structure

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method produces exfoliated graphite with a large specific surface area, making it easier to handle and more suitable for applications, such as resin composites with enhanced physical and electrical properties.

Implementation Method 1

pyrolyzing the polymer contained in the composition to exfoliate the graphite or primary exfoliated graphite and remove the polymer by pyrolysis of the polymer

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Data Source

PatentEP2816010B1Method for producing flake graphite, and flake graphite
Publication Date: 2021.06.30 SEKISUI CHEMICAL CO LTD
  • EP2816010B1 patent drawingFigure 1~2
  • EP2816010B1 patent drawingFigure 3~5
  • EP2816010B1 patent drawingFigure 6~7

AI summary

There is provided a method for producing relatively easily handleable exfoliated graphite by exfoliating graphite without complicated steps, and exfoliated graphite obtained by the method. A method for producing exfoliated graphite, comprising steps of preparing a composition which comprises graphite or primary exfoliated graphite and a polymer and in which the polymer is fixed to the graphite or primary exfoliated graphite; and pyrolyzing the polymer contained in the composition to exfoliate the graphite or primary exfoliated graphite and remove the polymer by pyrolysis.