FCC Additive Composition for Gasoline Octane and Yield

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Solution Overview

Problem

Conventional ZSM-5 additives used in fluid catalytic cracking (FCC) operations increase gasoline octane but result in significant gasoline yield loss, as they crack gasoline range molecules into lighter olefins, thereby reducing overall gasoline yield.

Innovation Solution

A customized additive composition incorporating medium pore pentasil zeolites with variable SiO2/Al2O3 mole ratios, combined with kaolin clay, alumina, phosphate, and bivalent metals from Group-IIA or Group-IB, which enhances gasoline octane without appreciable cracking, thereby minimizing yield loss.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If conventional ZSM-5 additives are used to enhance gasoline octane, then gasoline octane increases, but gasoline yield decreases due to cracking of gasoline range molecules into lighter olefins

Engineering Contradiction:
Improvegasoline octaneVSAvoidgasoline yield
Core Design Contradiction:
Measurement precisionVSQuantity of substance

Solution Approach 1:

The patent modifies the SiO2/Al2O3 mole ratio parameter of ZSM-5 zeolite from conventional values to specifically 18-35, and controls crystal size at 0.5-5.0 microns. These parameter changes optimize the catalyst's selectivity to enhance octane through aromatic formation rather than cracking, thereby improving octane while preserving gasoline yield

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite additive system combining modified ZSM-5 zeolite with a matrix containing alumina, silica, and phosphate. This composite structure allows the ZSM-5 component to selectively enhance octane while the matrix provides structural support and controls overall cracking activity, resolving the contradiction between octane enhancement and yield preservation

Inventive Principle:
Principle #40Composite materials

2Measurement precision

If ZSM-5 additives crack gasoline range molecules to increase octane, then gasoline octane improves, but lighter olefin yield increases at the expense of gasoline

Engineering Contradiction:
Improvegasoline octaneVSAvoidgasoline loss
Core Design Contradiction:
Measurement precisionVSLoss of substance

Solution Approach 1:

By optimizing the SiO2/Al2O3 ratio to 18-35 and crystal size to 0.5-5.0 microns, the patent changes the reaction pathway selectivity of ZSM-5. This causes the catalyst to favor aromatic formation (which increases octane) over cracking to lighter olefins, thereby improving octane while minimizing gasoline loss

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The additive increases gasoline octane by 2-3 units with minimal loss, improving light olefin and aromatics selectivity while maintaining gasoline yield, outperforming conventional ZSM-5 additives.

Implementation Method 1

Catalytic cracking catalyst includes a ZSM-5 type catalytic component contacted in the reaction zone with metal containing hydrocarbon feedstock. The hydrocarbon feedstock is cracked at high temperature by cracking catalyst resulting in increased gasoline octane

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

said additive further comprises bivalent metal selected from Group-IIA or Group-IB in an amount of 0.1 to 5.0 wt. %

Methodology Applied
Scientific EffectIon Exchange: Ion Exchange

Data Source

PatentUS11465132B2Fluid catalytic cracking additive composition for enhancing gasoline octane barrel and a process of preparation thereof
Publication Date: 2022.10.11 INDIAN OIL CORP LTD

AI summary

This invention relates to an additive capable of increasing the gasoline octane (by 2-3 units) with minimum loss of gasoline. More specifically, the present invention discloses a fluid catalytic cracking additive composition capable of enhancing gasoline octane, said composition comprising 5-50 wt. % zeolite component, 0-15 wt % alumina, 5-20 wt % colloidal silica, 10-60 wt % kaolin clay, 5-15 wt % phosphate, and 0.1 to 5.0 wt. % of bivalent metal selected from Group-IIA or Group-IB, wherein the zeolite component comprises of medium pore pentasil zeolite in an amount of 1 to 50 wt. % and said zeolite consists of one or more MFI topology zeolite having SiO2/Al2O3 mole ratio in the range of 10-280. The present invention also discloses a process for preparation of the additive.