Multi-Stage Filtration Cascade for Hydrothermal Carbonization

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Solution Overview

Problem

In hydrothermal carbonization processes, side reactions produce humic substances and oligomers that contaminate process water, reducing product purity and increasing cleaning efforts in extraction columns, as these impurities are similar to desired products and difficult to separate.

Innovation Solution

A multi-stage filter cascade is employed, where each stage selectively retains or allows through specific impurities and products, using membrane filters to separate humic substances, oligomers, and educts, ensuring only pure products reach the extraction column, with optional further filtration to concentrate and purify the products.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Device complexity

If a single-stage membrane filter is used to remove impurities from process water, then the filtration process is simplified, but impurities such as humic substances and oligomers cannot be effectively separated from products, leading to reduced product purity

Engineering Contradiction:
Improvefiltration process complexityVSAvoidproduct purity
Core Design Contradiction:
Device complexityVSManufacturing precision

Solution Approach 1:

The filtration process is divided into multiple stages with different membrane permeabilities. The first stage uses a membrane with higher permeability to remove larger impurities, while the second stage uses a membrane with lower permeability to separate smaller impurities from products. This segmentation allows each stage to focus on specific separation tasks, achieving high product purity without requiring an overly complex single-stage system.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different regions of the filtration process are assigned different membrane properties. The first filtration stage employs membranes with specific permeability characteristics suited for removing humic substances, while the second stage uses membranes with different permeability optimized for separating oligomers from products. This local differentiation of membrane quality enables effective separation throughout the process.

Inventive Principle:
Principle #3Local quality

2Productivity

If no pre-filtration is performed before extraction, then the extraction column operates continuously without interruption, but cleaning efforts increase significantly due to accumulation of humic substances and oligomers

Engineering Contradiction:
Improveextraction column throughputVSAvoidcleaning effort
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The filter cascade performs preliminary removal of impurities before the process water enters the extraction column. By eliminating humic substances and oligomers in advance, the extraction column receives pre-cleaned water, preventing accumulation of deposits that would require frequent cleaning interruptions. This preliminary action maintains continuous operation while minimizing cleaning requirements.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The filtration system preemptively counteracts the formation of problematic accumulations in the extraction column. By removing impurities that would otherwise deposit on column walls and heat exchangers, the system prevents the harmful effects of contamination before they occur, allowing uninterrupted operation.

Inventive Principle:
Principle #9Preliminary anti-action

3Manufacturing precision

If a two-stage filter cascade is implemented to improve product purity, then cleaning efforts are reduced, but the device complexity and initial investment increase

Engineering Contradiction:
Improveproduct purityVSAvoidfilter cascade structure
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The filtration system is segmented into two functional stages, each with specific separation objectives. The first stage handles bulk removal of humic substances, while the second stage focuses on fine separation of oligomers. This segmentation achieves high product purity through a manageable two-stage structure rather than requiring a single complex stage or multiple unnecessary stages.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The system changes the permeability parameter between stages to optimize separation. The first membrane has higher permeability for removing larger impurities, while the second membrane has lower permeability for separating smaller molecules. This parameter variation enables effective separation at each stage, achieving high purity with a practical device complexity.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method significantly reduces cleaning efforts, improves product purity, and enhances process efficiency by effectively removing impurities and recycling valuable educts, thereby increasing the quality of 5-hydroxymethylfurfural, furfural, and levulinic acid extraction.

Implementation Method 1

the filtration process is carried out by means of ultrafiltration

Methodology Applied
Scientific EffectUltrafiltration: Permeation

Implementation Method 2

the proportions in the process water whose size exceeds the permeability of the respective filtration stage are eliminated

Methodology Applied
Scientific EffectSize-based membrane separation: Semipermeable Membrane

Data Source

PatentEP2990385B1Method for treatment of process water
Publication Date: 2017.10.11 AVA CO2 SCHWEIZ
  • EP2990385B1 patent drawingFigure 1~2

AI summary

In the hydrothermal carbonization of biomass, in addition to the main product, coal, the platform chemical 5-hydroxymethylfurfural, as well as furfural and levulinic acid, are produced. These are extracted from the process water of the carbonization reaction. However, a problem arises: humic substances accumulate on the walls of the extraction column and can only be removed with considerable cleaning effort. Furthermore, oligomers significantly reduce the purity of the product. This problem is solved by a filtration cascade through which the process water passes before extraction. In a first filtration stage, the aforementioned contaminants are removed, and in a second filtration stage, the remaining products and reactants are separated. Only the products are then fed into the extraction process.