Flagellin Aerosol Stabilization via Buffer and Surfactant

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Solution Overview

Problem

The challenge lies in developing a stable aerosol composition for pulmonary delivery of flagellin polypeptides that maintains their biological activity and stability during aerosolization, as they are prone to aggregation and degradation due to shear stress and temperature changes, which is crucial for effectively treating lung bacterial infections.

Innovation Solution

Aerosol compositions comprising flagellin polypeptides with acetate or phosphate buffers and polysorbate surfactants, formulated to maintain a pH of 8 or lower, which reduces aggregation and enhances stability during nebulization, ensuring effective delivery and activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If flagellin is formulated in saline phosphate buffer (PBS) for pulmonary delivery, then the protein can be administered to the lungs, but the flagellin undergoes high aggregation and loss of biological activity due to aerosolization stress

Engineering Contradiction:
Improvepulmonary delivery capabilityVSAvoidflagellin stability and activity
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent changes the buffer system from PBS to acetate buffer, adjusts pH to 4.0-6.0 range, and optimizes flagellin concentration to 1-10 mg/mL. These parameter changes fundamentally alter the formulation properties to prevent aggregation during aerosolization while maintaining pulmonary delivery capability and flagellin biological activity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces specific excipients as intermediaries: acetate buffer acts as a pH mediator to maintain stable conditions, and polysorbate 80 serves as a surfactant mediator that prevents protein-protein interactions and aggregation during the aerosolization process, thereby protecting flagellin stability

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If the aerosolization process is performed with standard formulations, then the flagellin can be delivered to the lungs, but the protein experiences shear stress and temperature changes leading to degradation

Engineering Contradiction:
Improvedelivery efficiencyVSAvoidshear stress and temperature sensitivity
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent applies prior cushioning by incorporating polysorbate 80 surfactant and optimizing the buffer system before aerosolization occurs. These pre-formulation protections cushion the flagellin against the impending shear stress and temperature changes during nebulization, preventing degradation while maintaining delivery efficiency

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

3Device complexity

If flagellin is nebulized without optimized formulation, then the administration process is simple, but the protein exhibits decreased stability at the air-liquid interface

Engineering Contradiction:
Improveformulation simplicityVSAvoidflagellin stability at air-liquid interface
Core Design Contradiction:
Device complexityVSStability of the object's composition

Solution Approach 1:

The patent introduces polysorbate 80 as a surfactant intermediary that specifically addresses the air-liquid interface problem. This surfactant reduces surface tension and prevents flagellin aggregation at the interface during nebulization, maintaining stability without significantly complicating the formulation or administration process

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The formulation effectively stabilizes flagellin polypeptides, maintaining their potency and reducing aggregation, thereby ensuring effective pulmonary delivery and treatment of lung bacterial infections.

Implementation Method 1

a surfactant consisting of polysorbate

Methodology Applied
Scientific EffectSurfactant: Surfactant

Implementation Method 2

proteins can be sensitive towards aerosolization-associated shear stress and/or increase in temperature and/or may exhibit decreased stability at the air-liquid interface in an aerosol

Methodology Applied
Scientific EffectSurface tension reduction: Surface Tension

Implementation Method 3

a buffering agent selected from the group consisting of acetate, phosphate and combinations thereof; wherein the liquid formulation has a pH which is equal to or lower than about 8

Methodology Applied
Scientific EffectBuffering:

Data Source

PatentUS20240277801A1Aerosol composition for pulmonary delivery of flagellin
Publication Date: 2024.08.22 INST NAT DE LA SANTE & DE LA RECHERCHE MEDICALE (INSERM)

AI summary

The present invention arises from a formulation study in order to define the best excipients including buffer, surfactant, sugar and amino acid to stabilize Flagellin during mesh-nebulization. One of the key factors in stabilising proteins is determining the optimal pH and buffer system to provide adequate solubility and stability and avoid aggregate formation during the aerosolization process. Different formulation have been assayed in order to obtain a stable and soluble aerosol composition comprising flagellin polypeptide in particular considering the choice of the buffering agent, the surfactant and the pH of the liquid formulation comprising the flagellin polypeptide in order to maintain the activity of the flagellin after the aerosolization process. Accordingly, the present invention relates to an aerosol composition comprising droplets comprising a liquid formulation, wherein the liquid formulation comprises a flagellin polypeptide, a buffer (acetate and/or phosphate) and a surfactant (polysorbate).The aerosol composition of the present invention is suitable for the treatment of lung bacterial infections.