Flame retardant compositions with low formaldehyde content

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Solution Overview

Problem

Existing flame-retardant textile treatments using condensates of tetrakis (hydroxyorgano) phosphonium salts and (thio)urea contain high levels of formaldehyde, posing toxicity issues during storage, transportation, and handling.

Innovation Solution

Using tetrakis (hydroxyorgano) phosphonium sulfate (THPS) instead of tetrakis (hydroxyorgano) phosphonium chloride (THPC) to produce a condensate with a formaldehyde content of less than 0.1%, thereby reducing formaldehyde formation and odor during application.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If tetrakis (hydroxyorgano) phosphonium chloride (THPC) is used to produce flame-retardant condensate, then flame-retardant properties are achieved, but formaldehyde content exceeds 0.1% causing toxicity issues

Engineering Contradiction:
Improveflame-retardant propertiesVSAvoidformaldehyde content
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical parameter of the phosphonium salt from chloride form (THPC) to sulfate form (THPS). This parameter change fundamentally alters the formaldehyde generation behavior during alkaline treatment, reducing formaldehyde content from >0.1% to <0.1% while preserving the flame-retardant functionality of the condensate.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If strong base (KOH or NaOH) is added to elevate pH for condensate formation, then condensate is produced, but formaldehyde formation increases

Engineering Contradiction:
Improvecondensate formationVSAvoidformaldehyde formation
Core Design Contradiction:
Ease of manufactureVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical parameter of the phosphonium salt from chloride to sulfate form. This parameter change fundamentally alters the formaldehyde generation behavior during alkaline treatment, reducing formaldehyde content from >0.1% to <0.1% while preserving the flame-retardant functionality of the condensate.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If conventional THP+ chloride condensate is used for textile treatment, then flame-retardant treatment is achieved, but odor increases during application

Engineering Contradiction:
Improveflame-retardant treatmentVSAvoidodor
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the chemical parameter of the phosphonium salt from chloride form (THPC) to sulfate form (THPS). This parameter change fundamentally alters the formaldehyde generation behavior during alkaline treatment, reducing formaldehyde content from >0.1% to <0.1% while preserving the flame-retardant functionality of the condensate.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of THPS in the condensate significantly reduces formaldehyde content to below 0.1%, making the precursor safer for handling and use, while also minimizing odor during textile application.

Implementation Method 1

the fabric is then dried and then cured with ammonia (NH3) whereby a phosphonium-based polymer is produced within the fibers of the fabric

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 2

the obtained polymer is generally oxidized in order to convert at least a part of the trivalent phosphorus (carried by the phosphonium group) into a pentavalent phosphorous (an phosphine oxide group)

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentUS12320062B2Flame retardant compositions with low formaldehyde content
Publication Date: 2025.06.03 ENERGY SOLUTIONS US LLC

AI summary

The instant invention relates to a composition useful as a precursor for imparting flame-retardant properties to textile articles, comprising a condensate of: (a) a tetrakis (hydroxyorgano) phosphonium sulfate THPS; (b) urea, or alternatively thiourea; (c) optionally, and preferably, an aliphatic hydroxyl-reactive compound, such an amine wherein said composition has a very low free formaldehyde content, namely of less than 0.1%.