Flash Column for CO2 Recovery Contaminant Removal

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Solution Overview

Problem

Conventional methods for recovering high purity carbon dioxide from gaseous sources, such as flue gases, face challenges with contaminants like nitrogen oxides, sulphurous compounds, and volatile organic compounds, which require costly and hazardous oxidation steps and result in inefficient energy consumption and product yield.

Innovation Solution

Incorporating a flash column between the absorption and stripper columns to remove contaminants, allowing for the reduction of oxygen and nitrogen oxides, thereby eliminating the need for oxidation steps and enhancing the overall efficiency of the carbon dioxide recovery process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If conventional absorption method using amine-based agent is used to recover carbon dioxide, then carbon dioxide can be absorbed from gaseous source, but contaminants such as nitrogen oxides, sulphurous compounds and volatile organic compounds are also absorbed together with carbon dioxide

Engineering Contradiction:
Improvecarbon dioxide absorptionVSAvoidcontaminant absorption
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The absorption process is divided into two separate stages: first absorbing carbon dioxide with the amine-based agent, then selectively stripping contaminants in a separate step. This segmentation allows the system to achieve both carbon dioxide recovery and contaminant removal without compromising either function.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

An intermediary stripping step is introduced between absorption and final separation. This intermediary process uses controlled heating to selectively release contaminants from the absorbing agent while retaining carbon dioxide, thereby mediating between the absorption of both substances and enabling their separate handling.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Object-generated harmful factors

If oxidation step is used to remove contaminants from stripper off gas, then contaminant levels can be reduced, but hazardous chemicals are required and energy consumption increases

Engineering Contradiction:
Improvecontaminant removalVSAvoidhazardous chemicals and energy consumption
Core Design Contradiction:
Object-generated harmful factorsVSObject-affected harmful factors

Solution Approach 1:

The patent converts the harmful effect of contaminants being absorbed into a benefit by utilizing the selective stripping process. The same absorbing agent that inadvertently absorbs contaminants is used to selectively release them through controlled heating, transforming the contamination problem into a separable feature.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

Temperature is used as a controlling parameter to change the absorption characteristics of the amine-based agent. By adjusting temperature during the stripping step, contaminants are selectively released while carbon dioxide remains absorbed, enabling separation without oxidation or hazardous chemicals.

Inventive Principle:
Principle #35Parameter changes

3Quantity of substance

If oxygen is present in the gaseous source and alkanolamine is used as absorbing agent, then carbon dioxide absorption proceeds, but oxygen causes degradation of alkanolamine and corrosion problems

Engineering Contradiction:
Improvecarbon dioxide absorptionVSAvoidabsorbing agent stability
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

A preliminary stripping step is performed before the main carbon dioxide release step. This preliminary action removes oxygen and other contaminants from the absorbing agent solution, preventing their harmful effects during subsequent processing while maintaining the agent's stability and effectiveness.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly reduces contaminant levels in the stripper off-gas, eliminates the need for hazardous chemicals, decreases energy consumption, and increases product yield by minimizing the loss of carbon dioxide during condensation.

Implementation Method 1

a gas comprising carbon dioxide, oxygen, N2, nitrogen oxides and optionally sulphurous compounds and volatile organic contaminants is fed into an absorption column and absorbed in a chemical absorbing agent, by which the gas is separated into a carbon dioxide-lean gas and a carbon dioxide-rich liquid

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Implementation Method 2

The liquid is separated by means of flashing in a flash column into a N2-, NOx- and oxygen-rich gas and a N2-, NOx- and oxygen-depleted liquid

Methodology Applied
Scientific EffectFlashing: Flash Evaporation

Implementation Method 3

The liquid is separated into a carbon dioxide-rich stripper off gas and a carbon dioxide-depleted liquid by means of stripping in a stripper column

Methodology Applied
Scientific EffectStripping: Desorption

Implementation Method 4

The gas is cooled in a condenser with a temperature as low as the dew point temperature of the gas

Methodology Applied
Scientific EffectCondensation: Condensation

Data Source

PatentEP2121520B1A method for recovery of high purity carbon dioxide
Publication Date: 2016.09.28 UNION ENGINERING A/S
  • EP2121520B1 patent drawingFigure 1
  • EP2121520B1 patent drawingFigure 2

AI summary

The present invention describes a method for recovery of high purity carbon dioxide, which is substantially free of nitrogen oxides. This high purity carbon dioxide is obtained by introducing into the method a step in which carbon dioxide absorbed in an absorbing agent is flashed. The present invention also discloses a plant for recovery of said high purity carbon dioxide comprising an absorption column, a flash column, a stripper column, and a down stream purification unit comprising a washing column, a dehydrator, a condenser and a distillation unit.