Flexible Solid Polymer Electrolyte for High Conductivity Batteries

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Solution Overview

Problem

Current battery technologies using liquid or gel electrolytes face issues with electrolyte loss and decreased performance over time, requiring protective enclosures that increase size and bulk, while traditional solid polymer electrolytes have low ion transport at room temperature.

Innovation Solution

A flexible solid polymer electrolyte is developed, comprising a diblock copolymer with a polyether block and an acrylate block, incorporating lithium ions within microphase-separated spherical domains, along with a second lithium salt, such as lithium bis(oxalato)borate, to enhance conductivity and reduce crystallinity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If liquid or gel electrolytes are used in batteries, then ease of operation and initial performance are improved, but electrolyte loss over time and need for protective enclosures increase device complexity and reduce reliability

Engineering Contradiction:
Improveease of operationVSAvoidreliability
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent changes the physical state parameter of the electrolyte from liquid/gel to solid polymer form, eliminating electrolyte loss while maintaining ionic conductivity through careful selection of polymer matrix and lithium salt combinations

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite polymer electrolyte materials combining different polymer matrices (such as PEO, PANI, PPy) with lithium salts to achieve both mechanical stability and high ionic conductivity, resolving the contradiction between solid structure and operational performance

Inventive Principle:
Principle #40Composite materials

2Reliability

If traditional solid polymer electrolytes are used, then reliability and stability are improved, but ion transport at room temperature deteriorates

Engineering Contradiction:
ImprovereliabilityVSAvoidion transport
Core Design Contradiction:
ReliabilityVSSpeed

Solution Approach 1:

The patent modifies the chemical composition parameters of the solid polymer electrolyte by incorporating conductive polymers (PANI, PPy) and optimizing lithium salt content to achieve high ionic conductivity at room temperature while maintaining structural stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent utilizes the porous or microstructured morphology of the polymer matrix to facilitate ion transport pathways, allowing rapid ion movement through the solid electrolyte without requiring high temperatures

Inventive Principle:
Principle #31Porous materials

3Reliability

If protective enclosures are added to contain reactive electrolytes, then reliability is improved, but device complexity and bulk increase

Engineering Contradiction:
ImprovereliabilityVSAvoiddevice complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent extracts and eliminates the need for protective enclosures by using inherently stable solid polymer electrolytes that do not require additional containment structures, thereby reducing device complexity while maintaining safety and reliability

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The flexible solid polymer electrolyte exhibits high ion transport at room temperature, minimal capacity fade over 500 cycles, and longer performance life compared to conventional inorganic glass or ceramic electrolytes, enabling the creation of lightweight, shape-conforming batteries for miniature medical devices and other applications.

Implementation Method 1

a first polymer block capable of solvating a second lithium salt

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 2

a second polymer block that has the ability to incorporate lithium ions from a first lithium salt within microphase separated spherical domains

Methodology Applied
Scientific EffectMicrophase separation:

Data Source

PatentUS9252456B2Polymer solid electrolyte for flexible batteries
Publication Date: 2016.02.02 UNIV OF MARYLAND

AI summary

A flexible polymer solid electrolyte material useful in battery technology is described. The flexible solid electrolyte comprises a first block that has the ability to solvate alkali metal salts. The flexible solid electrolyte comprises a second block that has the ability to incorporate lithium ions within microphase separated spherical domains, wherein the lithium ions are from a secondary lithium source. The flexible solid electrolyte further comprises a second lithium salt.