Fluorinated Photopolymer Patterning for OLED Manufacturing

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Solution Overview

Problem

Current patterning methods for organic electronic devices, such as OLEDs, face challenges with fine metal masks that require frequent cleaning and alignment issues due to thermal expansion, leading to increased manufacturing costs and reduced positional accuracy, especially for pattern dimensions less than 100 µm.

Innovation Solution

A method using a fluorinated photopolymer layer with a radiation-absorbing dye and solubility-altering reactive groups, exposed to patterned radiation and developed with a fluorinated solvent to form undercut structures that can be easily lifted off, allowing for cost-effective and accurate patterning of organic electronic devices.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If a fine metal mask is used for patterning OLED devices, then the positional accuracy of mask openings is improved, but the mask requires frequent cleaning and maintenance due to film buildup, increasing manufacturing costs

Engineering Contradiction:
Improvepositional accuracy of mask openingsVSAvoidmask maintenance and cleaning frequency
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent extracts the patterning function from the metal mask and transfers it to a photopolymer layer that is deposited directly on the substrate. The photopolymer layer is then selectively removed through chemical etching or dissolution, eliminating the need for a reusable metal mask and its associated maintenance requirements while maintaining patterning precision

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The photopolymer layer serves as a disposable patterning medium that is applied fresh for each patterning operation and then completely removed after serving its purpose. This replaces the expensive, reusable metal mask with a low-cost, single-use alternative that eliminates cleaning and maintenance costs

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Area of stationary object

If the fine metal mask is increased in size to accommodate larger substrates, then the coverage area is improved, but the positional accuracy becomes more difficult to maintain due to thermal expansion issues

Engineering Contradiction:
Improvesubstrate coverage areaVSAvoidpositional accuracy of mask openings
Core Design Contradiction:
Area of stationary objectVSManufacturing precision

Solution Approach 1:

The patent replaces the mechanical metal mask system with a photopolymer-based optical patterning system. The photopolymer layer is deposited conformally across the entire substrate surface and patterned through photolithography, allowing large substrate areas to be covered without the thermal expansion and alignment issues that plague large metal masks

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Manufacturing precision

If the stiffness of the mask frame is enhanced to improve positional accuracy, then the alignment stability is improved, but the weight of the mask increases causing handling difficulties

Engineering Contradiction:
Improvealignment stability during depositionVSAvoidmask weight
Core Design Contradiction:
Manufacturing precisionVSWeight of moving object

Solution Approach 1:

The patent extracts the patterning function from the heavy metal mask and transfers it to a lightweight photopolymer layer deposited directly on the substrate. This eliminates the need for a stiff, heavy mask frame while maintaining alignment stability through the photopolymer's direct attachment to the substrate and optical patterning methods

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables efficient and precise patterning of organic electronic devices with a wide processing latitude, providing gentle processing conditions compatible with sensitive materials and enabling rapid, low-toxicity processing suitable for both organic and non-organic devices like MEMS.

Implementation Method 1

forming over a device substrate a fluorinated photopolymer layer comprising a radiation-absorbing dye

Methodology Applied
Scientific EffectAbsorption (EM radiation): Absorption (EM radiation)

Implementation Method 2

exposing the photopolymer layer to patterned radiation to form an exposed photopolymer layer having exposed and unexposed areas

Methodology Applied
Scientific EffectPhotopolymerisation: Photopolymerisation

Implementation Method 3

contacting the exposed photopolymer layer with a developing agent to remove the unexposed areas, thereby forming a developed structure having a first pattern of photopolymer

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentEP3238288B1Photolithographic patterning of electronic devices
Publication Date: 2020.07.29 ORTHOGONAL
  • EP3238288B1 patent drawingFigure 1A~1E
  • EP3238288B1 patent drawingFigure 2
  • EP3238288B1 patent drawingFigure 3

AI summary

A method of patterning a device includes forming a fluorinated photopolymer layer over a device substrate. The photopolymer layer has a lower portion proximate the device substrate and an upper portion distal the device substrate. The fluorinated photopolymer layer includes a radiation-absorbing dye and a fluorinated photopolymer having a solubility-altering reactive group. The photopolymer layer is exposed to patterned radiation to form exposed and unexposed areas in accordance with the patterned radiation and a developed structure is formed by removing unexposed areas using a developing agent that includes a first fluorinated solvent. The lower portion of the exposed area of the photopolymer layer has a dissolution rate in the developing agent that is at least 5 times higher than a dissolution rate for the upper portion.