Fluorinated Silicon-Oxide Passivation for Solar Cell Textures

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Solution Overview

Problem

Existing silicon-based photovoltaic device manufacturing processes face challenges in achieving efficient etching and passivation of substrates, particularly for sub-micrometer features, which affects the electrical properties and reflectivity of solar cells, as conventional methods result in low carrier lifetime and surface defects.

Innovation Solution

A dry chemical etching and passivation process using molecular fluorine as the etchant gas at atmospheric pressure, followed by in-situ oxidation to create a stable fluorinated silicon-oxide layer, ensuring the preservation of electrical properties and reducing thermal budget, all performed within a single tool without exposing the substrate to air.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If conventional etching processes are used to create surface texture, then reflectivity is reduced, but surface defects are generated that degrade electrical properties

Engineering Contradiction:
ImprovereflectivityVSAvoidelectrical properties
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent combines the etching step and passivation step into a single integrated process. The fluorinated etchant simultaneously etches the silicon surface to create light-trapping texture and passivates the surface by forming a fluorinated silicon-oxide layer, eliminating the need for separate etching and passivation tools and processes.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent changes the chemical parameters of the etching process by using a fluorinated etchant gas (such as SF6, CF4, or NF3) instead of conventional halogen-based etchants. This parameter change enables the etchant to provide both etching and passivation functions, creating a fluorinated surface layer that reduces recombination while maintaining electrical properties.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If PECVD passivation is applied to sub-micrometer features, then conformality is achieved, but carrier lifetime remains very low

Engineering Contradiction:
ImproveconformalityVSAvoidcarrier lifetime
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the chemical composition and deposition mechanism by using a fluorinated etchant that simultaneously etches and passivates. The fluorinated silicon-oxide layer formed has superior passivation properties compared to conventional PECVD layers, achieving both conformal coverage on sub-micrometer features and high carrier lifetime.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If multiple separate process steps are used for etching and passivation, then each step can be optimized, but the number of manufacturing steps increases

Engineering Contradiction:
Improveprocess optimizationVSAvoidnumber of manufacturing steps
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent merges two separate process steps (etching and passivation) into a single integrated step using a fluorinated etchant gas. This reduces the number of manufacturing steps from two separate tool processes to one unified process, improving productivity while maintaining the ability to optimize both functions simultaneously through parameter control.

Inventive Principle:
Principle #5Merging (Combining)

4Illumination intensity

If sub-micron texture is created for light trapping, then surface reflectivity is reduced, but conventional passivation methods become inefficient

Engineering Contradiction:
Improvesurface reflectivityVSAvoidpassivation efficiency
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent changes the chemical parameters by using a fluorinated etchant that forms a fluorinated silicon-oxide layer. This layer provides superior passivation efficiency on sub-micron textured surfaces compared to conventional PECVD methods, enabling both effective light trapping and high passivation quality on sub-micrometer features.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process enhances passivation quality, reduces the number of manufacturing steps, and improves the overall efficiency of solar cells by creating a stable and efficient light-trapping nano-texture without the need for additional anti-reflective layers, while maintaining the substrate's electrical properties.

Implementation Method 1

etching the surface of the substrate with a fluoride-containing etchant gas inside the chamber

Methodology Applied
Scientific EffectChemical etching: Chemical Bonding

Implementation Method 2

oxidising the textured, fluorinated surface of the substrate without exposing the substrate to air

Methodology Applied
Scientific EffectThermal oxidation: Oxidation

Data Source

PatentEP2904634B1Combined etch and passivation of silicon solar cells
Publication Date: 2020.04.08 ULTRA HIGH VACUUM SOLUTIONS TA NINES ENG
  • EP2904634B1 patent drawingFigure 1~2
  • EP2904634B1 patent drawingFigure 3~4
  • EP2904634B1 patent drawingFigure 5

AI summary

A process for passivating and etching a texture on a surface of a substrate, the process comprising the steps of inserting a substrate in a reactor chamber; heating the reactor chamber and substrate; etching the substrate with an fluoride-containing etchant gas inside the chamber; and oxidising the etched surface of the substrate prior to exposing the fluorinated substrate to air or any other reactive atmosphere; wherein oxidisation of the etched surface of the substrate generates a strongly passivated and stable surface texture.