Fluorine Copolymer Paper Coating for Oil Resistance

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Solution Overview

Problem

Existing water and oil resistant agents for paper, particularly those using fluorine-containing copolymers with short chain polyfluoroalkyl groups, fail to provide satisfactory water and oil resistance, as they compromise on performance compared to their long chain counterparts, and there is a need for a solution that addresses environmental concerns associated with long chain Rf groups.

Innovation Solution

A water and oil resistant agent for paper comprising a fluorine-containing copolymer with specific polymer units, including a fluorine-containing monomer, a hydrophilic monomer, and an anion-donating monomer, with a weight average molecular weight of 100,000 or more, which enhances both water and oil resistance while being environmentally friendly.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a fluorine-containing copolymer with a long chain Rf group is used, then water and oil resistance is improved, but environmental harm increases due to PFOA production

Engineering Contradiction:
Improvewater and oil resistanceVSAvoidenvironmental harm from PFOA
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent changes the molecular weight parameter of the fluorine-containing copolymer from conventional low molecular weight to high molecular weight (100,000 or more), while using short chain Rf groups (C1-C6). This parameter change allows achieving both adequate water and oil resistance and environmental compatibility, resolving the contradiction between performance and environmental harm.

Inventive Principle:
Principle #35Parameter changes

2Object-generated harmful factors

If a fluorine-containing copolymer with a short chain Rf group is used, then environmental harm is reduced, but water and oil resistance decreases

Engineering Contradiction:
Improveenvironmental compatibilityVSAvoidwater and oil resistance
Core Design Contradiction:
Object-generated harmful factorsVSReliability

Solution Approach 1:

The patent increases the molecular weight parameter to 100,000 or more while maintaining short chain Rf groups (C1-C6). This parameter adjustment compensates for the reduced hydrophobicity from short Rf chains, restoring adequate water and oil resistance while preserving environmental compatibility.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a composite copolymer structure combining fluorine-containing monomers with specific functional groups (carboxyl, sulfonic acid, phosphonic acid) and hydrophilic monomers. This composite approach balances the hydrophobic effect from fluorine groups with hydrophilic contributions from functional groups, achieving optimal performance with short Rf chains.

Inventive Principle:
Principle #40Composite materials

3Object-generated harmful factors

If the carbon number of the Rf group is decreased, then environmental compatibility is improved, but water and oil resistance deteriorates

Engineering Contradiction:
Improveenvironmental compatibilityVSAvoidwater and oil resistance
Core Design Contradiction:
Object-generated harmful factorsVSReliability

Solution Approach 1:

The patent maintains Rf group carbon number between 1-6 (short chain) while compensating through increased molecular weight (100,000 or more) and specific copolymer composition. This parameter strategy preserves environmental compatibility while achieving satisfactory water and oil resistance through the combined effect of high molecular weight and functional group interactions.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The described agent provides superior water and oil resistance to paper, maintaining performance comparable to long chain Rf group-based agents while being environmentally safer, as evidenced by improved resistance test results and stability.

Implementation Method 1

a fluorine-containing copolymer having a short chain Rf, specified polymer units and a high molecular weight can exhibit a superior water and oil resistance

Methodology Applied
Scientific EffectHydrophobe: Hydrophobe

Data Source

PatentUS9249540B2Water and oil resistant agent for paper, treatment process and paper
Publication Date: 2016.02.02 DAIKIN INDUSTRIES LTD

AI summary

Disclosed is a water and oil resistant agent comprising a fluorine-containing copolymer obtained by copolymerizing a (meth)acrylate monomer having a polyfluoroalkyl group having 1-6 carbon atoms, hydrophilic monomer, and monomer having an anion-donating group, which agent affords a superior water and oil resistance to a paper. The invention also discloses a process for treating a paper by the water and oil resistant agent and a treated paper thereby.