Fluoropolymer Copolymer Composition for Thick Transparent Sheet Extrusion

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Solution Overview

Problem

Existing copolymers with tetrafluoroethylene and perfluoro(alkyl vinyl ether units face challenges in producing thick sheets with uniform thickness and high transparency, while maintaining high tensile strength, low permeability, and resistance to deformation and chemical solutions.

Innovation Solution

A copolymer with a specific composition of tetrafluoroethylene and perfluoro(propyl vinyl ether units, with a content of 4.9 to 7.0% by mass and a melt flow rate of 0.5 to 1.5 g/10 min, which minimizes deformation in the molten state and enhances transparency, tensile strength, and resistance to air, chemical, and carbon dioxide permeability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If the copolymer contains perfluoro(alkyl vinyl ether) units to improve processability and transparency, then the melt flow rate increases and transparency improves, but the tensile strength decreases and deformation resistance worsens

Engineering Contradiction:
Improvemelt flow rateVSAvoidtensile strength
Core Design Contradiction:
Ease of manufactureVSStrength

Solution Approach 1:

The patent applies parameter changes by precisely controlling the content of perfluoro(propyl vinyl ether) units within 4.5-6.6% by mass and the number of unstable terminal groups to 20 or less per 1×10^6 carbon atoms. This optimization balances the melt flow rate (0.5-1.5 g/10 min at 372°C) for good processability while maintaining high tensile strength (20-30 MPa) and deformation resistance in the formed articles.

Inventive Principle:
Principle #35Parameter changes

2Illumination intensity

If the copolymer composition is adjusted to improve transparency, then the haze value decreases and clarity improves, but the chemical solution resistance and permeability properties worsen

Engineering Contradiction:
ImprovetransparencyVSAvoidchemical solution resistance
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent achieves optimal transparency with haze values of 10% or less (typically 2-8%) by controlling the perfluoro(propyl vinyl ether) unit content at 4.5-6.6% by mass. Simultaneously, it maintains excellent chemical solution resistance by limiting unstable terminal groups to 20 or less per 1×10^6 carbon atoms, preventing fluorine ion dissolution in chemical solutions while preserving low permeability to gases and liquids.

Inventive Principle:
Principle #35Parameter changes

3Length of stationary object

If the copolymer is used to produce thick sheets by extrusion, then the sheet thickness increases, but the thickness uniformity decreases and deformation increases

Engineering Contradiction:
Improvesheet thicknessVSAvoidthickness uniformity
Core Design Contradiction:
Length of stationary objectVSManufacturing precision

Solution Approach 1:

The patent enables production of thick sheets (5 mm or more, up to 50 mm or more) with excellent thickness uniformity by optimizing the copolymer parameters: perfluoro(propyl vinyl ether) unit content of 4.5-6.6% by mass provides appropriate melt viscosity, while unstable terminal groups of 20 or less per 1×10^6 carbon atoms prevent excessive flow and deformation during extrusion and molding processes.

Inventive Principle:
Principle #35Parameter changes

4Strength

If the copolymer composition is optimized for high tensile strength, then the mechanical strength increases, but the melt flow rate decreases and processability worsens

Engineering Contradiction:
Improvetensile strengthVSAvoidprocessability
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The patent achieves both high tensile strength (20-30 MPa) and good processability by precisely balancing multiple parameters: perfluoro(propyl vinyl ether) units at 4.5-6.6% by mass provide sufficient chain flexibility for melt flow, while unstable terminal groups limited to 20 or less per 1×10^6 carbon atoms maintain chain integrity for high strength. The resulting melt flow rate of 0.5-1.5 g/10 min at 372°C enables easy extrusion and molding while preserving mechanical properties.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentUS20230406976A1Copolymer, molded body, extruded body, and transfer molded body
Publication Date: 2023.12.21 DAIKIN INDUSTRIES LTD

AI summary

There is provided a copolymer containing tetrafluoroethylene unit and perfluoro(propyl vinyl ether) unit, wherein the copolymer has a content of perfluoro(propyl vinyl ether) unit of 4.9 to 7.0% by mass with respect to the whole of the monomer units, a melt flow rate at 372° C. of 0.5 to 1.5 g/10 min, and the number of functional groups of 20 or less per 106 main-chain carbon atoms.