Fly Ash Leaching with HCl for Alumina Recovery

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Solution Overview

Problem

Current methods for treating fly ash are inefficient and lead to environmental and health concerns, with limited recycling options due to high landfill costs and concerns over health impacts, necessitating an alternative process for valorization and recycling.

Innovation Solution

A process involving leaching aluminum-containing materials with HCl to obtain aluminum ions, converting AlCl3 into Al2O3, and recycling gaseous HCl to enhance the concentration for further leaching, allowing for the extraction of alumina and other products.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If fly ash is disposed of in landfills, then environmental and health concerns are addressed, but recycling rates remain low and landfill costs increase

Engineering Contradiction:
Improveenvironmental and health concernsVSAvoidrecycling rate
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The patent applies parameter changes by using hydrochloric acid to alter the chemical state of fly ash, converting aluminum oxide into soluble aluminum chloride through chemical reaction. This transformation enables the extraction and recovery of aluminum and other metals, turning waste material into valuable products and achieving high recycling rates while addressing environmental concerns.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If fly ash is recycled through conventional methods, then recycling rates improve, but extraction efficiency and material recovery remain limited

Engineering Contradiction:
Improverecycling rateVSAvoidextraction efficiency
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The patent uses hydrochloric acid as an intermediary substance to facilitate the extraction process. The acid reacts with aluminum oxide in fly ash to form aluminum chloride, which can then be processed to recover aluminum metal. This intermediary chemical reaction significantly improves extraction efficiency and material recovery rates compared to conventional physical separation methods.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Productivity

If HCl is used for leaching aluminum-containing materials, then alumina extraction efficiency improves, but HCl consumption increases and requires recycling

Engineering Contradiction:
Improvealumina extraction efficiencyVSAvoidHCl consumption
Core Design Contradiction:
ProductivityVSLoss of substance

Solution Approach 1:

The patent implements a recycling system where hydrochloric acid is recovered from the leaching process and regenerated for reuse. The acid that reacts with aluminum oxide is processed to recover aluminum chloride, and the HCl is then regenerated and returned to the leaching process. This closed-loop system minimizes HCl consumption and reduces waste while maintaining high alumina extraction efficiency.

Inventive Principle:
Principle #34Discarding and recovering

4Productivity

If gaseous HCl is released during alumina production, then alumina conversion is achieved, but environmental emissions increase

Engineering Contradiction:
Improvealumina conversion rateVSAvoidgaseous HCl emissions
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent converts the harmful gaseous HCl byproduct into a beneficial resource. The gaseous HCl released during alumina conversion is captured, dissolved in water to form hydrochloric acid solution, and then regenerated for reuse in the leaching process. This approach transforms an environmental pollutant into a valuable chemical reagent, eliminating emissions while maintaining production efficiency.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process effectively recycles fly ash, reducing landfill needs and environmental impact by efficiently extracting alumina and other metals, achieving high recovery yields and minimizing waste.

Implementation Method 1

leaching an aluminum-containing material with HCl so as to obtain a leachate comprising aluminum ions

Methodology Applied
Scientific EffectLeaching: Solvation

Implementation Method 2

heating the precipitate under conditions effective for converting AlCl3 into Al2O3

Methodology Applied
Scientific EffectThermal decomposition: Pyrolysis

Implementation Method 3

recycling the gaseous HCl so-produced by contacting it with water so as to obtain a composition having a concentration higher than HCl azeotrope concentration

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Data Source

PatentEP2838848B1Processes for treating fly ashes
Publication Date: 2019.05.08 ORBITE TECHNOLOGIES INC
  • EP2838848B1 patent drawingFigure 1
  • EP2838848B1 patent drawingFigure 2
  • EP2838848B1 patent drawingFigure 3

AI summary

There are provided processes for treating fly ash. For example, the processes can comprise leaching fly ash with HCI so as to obtain a Ieachate comprising aluminum ions and a solid, and separating the solid from the Ieachate; reacting the Ieachate with HCI so as to obtain a liquid and a precipitate comprising the aluminum ions in the form of AICI3, and separating the precipitate from the liquid; and heating the precipitate under conditions effective for converting AICI3 into AI2O3 and optionally recovering gaseous HCI so-produced.