Formula I Metal Complex Hole Injection Layer for OLED Voltage Stability

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Solution Overview

Problem

There is a need to improve the performance of semiconductor materials and electronic devices, particularly in achieving stable operating voltage over time and enhancing the characteristics of hole injection layers in organic light-emitting diodes (OLEDs), with a focus on balancing hole and electron injection and enabling mass production through suitable deposition methods.

Innovation Solution

A compound represented by Formula (I) is introduced, comprising a metal complex with specific ligands and substituents, which forms a non-emissive hole injection layer suitable for vacuum thermal evaporation, optimizing the HOMO level and enabling efficient hole injection while being deposited under conditions suitable for mass production.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional hole injection materials are used, then the device can be manufactured, but the operating voltage stability over time is insufficient

Engineering Contradiction:
Improveoperating voltage stabilityVSAvoiddevice lifetime
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The patent modifies the chemical structure of hole injection materials by introducing specific substituents (e.g., fluorinated alkyl groups, aryl groups) at defined positions of the core molecule. These parameter changes in molecular structure lead to improved HOMO levels and enhanced material stability, directly addressing the operating voltage stability and lifetime issues.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention employs composite hole injection layers comprising multiple materials with complementary properties. The specific compound of Formula (I) is combined with other hole transport materials to create a synergistic system that improves both voltage stability and device lifetime compared to single-material systems.

Inventive Principle:
Principle #40Composite materials

2Reliability

If the HOMO level is optimized for efficient hole injection, then hole injection performance improves, but compatibility with mass production deposition methods becomes difficult

Engineering Contradiction:
Improvehole injection efficiencyVSAvoiddeposition process compatibility
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent achieves the dual goal by carefully adjusting molecular parameters - specifically the substitution patterns and molecular weight - to tune both the HOMO level (for injection efficiency) and the deposition characteristics (for manufacturability). The defined structural parameters in Formula (I) represent an optimized balance between these competing requirements.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If the hole injection layer is designed for high performance, then operating voltage improves, but the ability to inject into layers with HOMO level further from vacuum level is insufficient

Engineering Contradiction:
Improveoperating voltageVSAvoidHOMO level matching range
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent provides a series of compounds with systematically varied substituents that allow tuning of the HOMO level across a broader range. This parameter adjustment capability enables the hole injection layer to effectively interface with adjacent layers having different HOMO levels, improving both operating voltage and adaptability.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The compound improves the stability of operating voltage and lifetime of OLEDs by enhancing hole injection characteristics, allowing for efficient deposition processes compatible with mass production, thereby improving the overall performance of electronic devices.

Implementation Method 1

It is also objective to provide a hole injection layer comprising compounds which may be deposited through vacuum thermal evaporation under conditions suitable for mass production.

Methodology Applied
Scientific EffectVacuum thermal evaporation: Evaporation

Data Source

PatentEP3945125A1Compound of formula (i), a semiconductor material comprising at least one compound of formula (i), an semiconductor layer comprising at least one compound of formula (i) and an electronic device comprising at least one compound of formula (i)
Publication Date: 2022.02.02 NOVALED GMBH
  • EP3945125A1 patent drawingFigure 1~2
  • EP3945125A1 patent drawingFigure 3~4
  • EP3945125A1 patent drawingFigure 5~6

AI summary

The present invention relates to a compound of Formula (I), a semiconductor material comprising at least one compound of Formula (I), an semiconductor layer comprising at least one compound of Formula (I) and an electronic device comprising at least one compound of Formula (I).