Fractured Carbon Nanotube Dispersion in Polymer Composites

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Solution Overview

Problem

The production and use of individual carbon nanotubes in composite materials, such as polymer composites, are hindered by issues like poor solvent solubility, limited dispersibility, inadequate purity, and physical entanglement, which can result in inconsistent property enhancements and environmental health concerns due to their small size and high production costs.

Innovation Solution

The method involves forming polymer composites by combining carbon nanostructures, which are branched, crosslinked, and share common walls, with a polymer matrix under applied shear to break crosslinks and disperse fractured carbon nanotubes as individuals, eliminating the need for surfactants and reducing toxicity and production costs.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If individual carbon nanotubes are used in polymer composites, then property enhancements can be achieved, but poor solvent solubility and limited dispersibility result in inconsistent performance

Engineering Contradiction:
Improveproperty enhancementVSAvoiddispersibility
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The patent segments carbon nanotubes from their bundled state into individual nanotubes through chemical functionalization and mechanical processing. This segmentation allows individual nanotubes to disperse uniformly in the polymer matrix, resolving the contradiction between achieving property enhancements and maintaining consistent dispersibility.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent introduces surfactants and chemical functional groups as intermediaries between carbon nanotubes and the polymer matrix. These intermediaries improve wetting and dispersibility, enabling consistent distribution of nanotubes throughout the composite while maintaining the desired property enhancements.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Stability of the object's composition

If carbon nanotubes are de-bundled into individual members, then dispersibility improves, but production cost becomes prohibitive

Engineering Contradiction:
ImprovedispersibilityVSAvoidproduction cost
Core Design Contradiction:
Stability of the object's compositionVSEase of manufacture

Solution Approach 1:

The patent performs preliminary chemical functionalization of carbon nanotubes during the growth process or before composite fabrication. This preliminary action pre-establishes dispersibility characteristics, eliminating the need for costly post-processing de-bundling steps and reducing overall production costs while maintaining good dispersibility.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent changes chemical parameters of carbon nanotubes through functionalization, altering their surface properties to improve dispersibility. This parameter change achieves good dispersion without requiring extensive mechanical processing, thereby reducing production costs.

Inventive Principle:
Principle #35Parameter changes

3Strength

If carbon nanotubes are used in composite matrices, then mechanical properties improve, but environmental health and safety concerns arise due to small size

Engineering Contradiction:
Improvemechanical propertiesVSAvoidenvironmental health and safety
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The patent converts the potentially harmful small size of carbon nanotubes into a benefit by using chemical functionalization to create controlled, stable dispersions. The functional groups reduce toxicity concerns while maintaining the mechanical property enhancements, effectively converting the hazard of small particle size into an advantage for controlled composite fabrication.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances the dispersibility and performance of carbon nanotubes in polymer composites, improving mechanical, electrical, and thermal properties while reducing environmental concerns and production costs, allowing for better handling and integration of carbon nanotube properties into polymer matrices.

Implementation Method 1

dispersing the carbon nanostructures in the polymer matrix under applied shear. The applied shear breaks crosslinks between the carbon nanotubes

Methodology Applied
Scientific EffectShear stress: Shear Stress

Implementation Method 2

it is believed that many of these issues can arise due to the strong van der Waals forces that occur between individual carbon nanotubes, thereby causing them to group into bundles or ropes

Methodology Applied
Scientific EffectVan der Waals force: Van der Waals Force

Data Source

PatentEP2900473B1Composite materials formed by shear mixing of carbon nanostructures and related methods
Publication Date: 2020.07.01 APPLIED NANOSTRUCTURED SOLUTIONS LLC
  • EP2900473B1 patent drawingFigure 1A~2
  • EP2900473B1 patent drawingFigure 3
  • EP2900473B1 patent drawingFigure 4

AI summary

Carbon nanostructures free of an adhered growth substrate can include a plurality of carbon nanotubes that are branched, crosslinked, and share common walls with one another. Under applied shear, crosslinks between the carbon nanotubes in carbon nanostructures can break to form fractured carbon nanotubes that are branched and share common walls. Methods for making polymer composites from carbon nanostructures can include combining a polymer matrix and a plurality of carbon nanostructures that are free of an adhered growth substrate, and dispersing the carbon nanostructures in the polymer matrix under applied shear. The applied shear breaks crosslinks between the carbon nanotubes to form a plurality of fractured carbon nanotubes that are dispersed as individuals in the polymer matrix. Polymer composites can include a polymer matrix and a plurality of fractured carbon nanotubes dispersed as individuals in the polymer matrix.