Aqueous FSH Formulation Stabilization

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Solution Overview

Problem

Current formulations of human follicle stimulating hormone (FSH) require refrigeration to maintain stability, limiting their shelf-life and convenience for self-administration at ambient or body temperature.

Innovation Solution

A novel aqueous formulation of FSH stabilized with a buffer system containing stabilizers, non-ionic surfactants, antioxidants, and preservatives, including sodium chloride, trehalose, mannitol, polysorbate 20, L-methionine, and phenol, which maintains stability and activity at elevated temperatures.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If FSH is formulated in aqueous solution for ease of administration, then convenience is improved, but stability deteriorates due to dissociation and denaturation

Engineering Contradiction:
Improveconvenience of administrationVSAvoidstability of FSH
Core Design Contradiction:
Ease of operationVSStability of the object's composition

Solution Approach 1:

The patent introduces multiple stabilizing agents as intermediaries between FSH and the aqueous environment. These include surfactants (polysorbate 20, poloxamer 188) that prevent surface adsorption, amino acids (glycine, L-arginine) that prevent dissociation, and antioxidants (methionine, ascorbic acid) that prevent oxidation. These mediators create a protective microenvironment that maintains FSH stability in aqueous solution without requiring refrigeration.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The formulation uses a composite system combining multiple excipients with specific functions: buffers (phosphate, citrate) for pH control, surfactants for surface protection, amino acids for dissociation prevention, antioxidants for oxidation prevention, and osmotic agents (mannitol, sucrose) for structural stabilization. This composite approach synergistically addresses multiple degradation pathways simultaneously, enabling stable aqueous formulation at ambient temperature.

Inventive Principle:
Principle #40Composite materials

2Duration of action of stationary object

If refrigeration is used to maintain FSH stability, then shelf-life is improved, but convenience deteriorates due to storage requirements

Engineering Contradiction:
Improveshelf-lifeVSAvoidconvenience of storage
Core Design Contradiction:
Duration of action of stationary objectVSEase of operation

Solution Approach 1:

The formulation modifies the chemical parameters of the aqueous environment to enhance thermal stability. By adjusting pH to physiological range (6.5-7.5) using buffers, adding osmotic agents at specific concentrations (mannitol 1-5%, sucrose 2-10%), and incorporating stabilizing agents at optimized levels, the formulation achieves stability at ambient temperature (20-25°C) without refrigeration, eliminating storage constraints while maintaining shelf-life.

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If lyophilization is used to stabilize FSH, then stability is improved, but complexity deteriorates due to reconstitution requirement

Engineering Contradiction:
Improvestability of FSHVSAvoidcomplexity of administration
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

Instead of removing water to stabilize FSH (lyophilization), the invention inverts the approach by maintaining FSH in aqueous solution and adding stabilizing agents that prevent degradation. This eliminates the need for freeze-drying and reconstitution steps, providing a ready-to-use liquid formulation that is as stable as or more stable than lyophilized products while being significantly easier to administer.

Inventive Principle:
Principle #13The other way round (Inversion)

4Stability of the object's composition

If stabilizing agents are added to prevent dissociation, then stability is improved, but purity deteriorates due to potential contamination

Engineering Contradiction:
Improvestability of FSHVSAvoidpurity of FSH
Core Design Contradiction:
Stability of the object's compositionVSLoss of substance

Solution Approach 1:

The patent uses pharmacopeial-grade excipients that are approved for parenteral administration, ensuring they meet strict purity specifications. These include USP-grade polysorbate 20, poloxamer 188, glycine, L-arginine, methionine, ascorbic acid, phosphate buffers, and osmotic agents. These materials are used at low concentrations and are considered safe and pure for injection, minimizing contamination risks while effectively stabilizing FSH.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The formulation achieves less than 5% dissociation after two hours at 55°C and maintains stability for a prolonged period, ensuring a reasonable shelf-life without refrigeration, making it suitable for use at room or body temperature.

Implementation Method 1

stabilized in a buffer containing one or more stabilizer, a non-ionic surfactant, an anti-oxidant, inorganic salt

Methodology Applied
Scientific EffectBuffer system:

Implementation Method 2

a non-ionic surfactant

Methodology Applied
Scientific EffectSurfactant: Surfactant

Implementation Method 3

an anti-oxidant

Methodology Applied
Scientific EffectAnti-oxidant: Oxidation

Implementation Method 4

inorganic salt

Methodology Applied
Scientific EffectInorganic salt: Electrostatic Discharge

Data Source

PatentEP2533800B1Liquid formulation of follicle stimulating hormone
Publication Date: 2016.07.20 INTAS PHARM LTD
  • EP2533800B1 patent drawingFigure 1~2
  • EP2533800B1 patent drawingFigure 3~4
  • EP2533800B1 patent drawingFigure 5

AI summary

The present invention relates to an aqueous formulation of a follicle stimulating hormone (hFSH) which is stabilized to maintain the activity of hFSH for a prolonged period of time.