Fuel Cell Separator Stainless Steel With Low Contact Resistance

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Solution Overview

Problem

Stainless steel separators for polymer fuel cells face challenges with high interfacial contact resistance due to oxide films formed during bright annealing, requiring additional costly coating processes to improve conductivity.

Innovation Solution

An austenitic stainless steel composition with specific alloying elements and a manufacturing method involving bright annealing followed by alternating current electrolysis in a sulfuric acid solution to reduce interfacial contact resistance without additional surface treatments.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If stainless steel is bright-annealed in a reducing atmosphere to prevent surface defects and control tension, then surface quality and mechanical properties are improved, but an oxide film with high resistance is formed on the surface

Engineering Contradiction:
Improvesurface qualityVSAvoidinterfacial contact resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent applies alternating current electrolysis to change the chemical state of the oxide film on the stainless steel surface. By controlling the electrolysis parameters (current density, time, electrolyte composition), the high-resistance oxide film is converted into a low-resistance conductive layer, resolving the contradiction between maintaining surface quality from bright annealing and reducing interfacial contact resistance.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If a coating process is applied to reduce interfacial contact resistance, then electrical conductivity is improved, but manufacturing cost and manufacturing time increase

Engineering Contradiction:
Improveinterfacial contact resistanceVSAvoidmanufacturing time
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent uses alternating current electrolysis to enable the stainless steel surface to self-modify its properties. The electrolysis process directly transforms the oxide film into a conductive state without requiring external coating materials or additional coating equipment, thereby reducing manufacturing steps and costs while achieving the desired low contact resistance.

Inventive Principle:
Principle #25Self-service

3Reliability

If a coating process is applied to reduce interfacial contact resistance, then electrical conductivity is improved, but manufacturing cost increases

Engineering Contradiction:
Improveinterfacial contact resistanceVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces expensive noble metal coatings (such as gold or platinum) with an inexpensive alternating current electrolysis treatment. The electrolysis uses common electrolytes and requires no precious materials, achieving the same functional effect of reducing contact resistance at a fraction of the material cost.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

4Reliability

If additional post-processing steps are applied to improve contact resistance, then interfacial contact resistance is reduced, but device complexity increases

Engineering Contradiction:
Improveinterfacial contact resistanceVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent combines the surface treatment and contact resistance reduction into a single alternating current electrolysis step. This integrated process simultaneously achieves surface cleaning, oxide film modification, and conductivity improvement, eliminating the need for separate coating and treatment steps, thereby simplifying the overall manufacturing process.

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively lowers interfacial contact resistance to 10 mΩ·cm2 or less, improving the electrical conductivity of stainless steel separators for fuel cells without increasing manufacturing costs or time.

Implementation Method 1

bright-annealed in a reducing atmosphere using hydrogen or nitrogen for recrystallization and removal of residual stress

Methodology Applied
Scientific EffectAnnealing: Annealing

Implementation Method 2

an oxide film formed by bright annealing

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 3

performing alternating current electrolysis on the bright-annealed material in a sulfuric acid solution

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Data Source

PatentUS20230420698A1Austenitic stainless steel for polymer fuel cell separator with improved contact resistance and manufacturing method thereof
Publication Date: 2023.12.28 POHANG IRON & STEEL CO LTD

AI summary

Disclosed is an austenitic stainless steel for a fuel cell separator with improved contact resistance. The austenitic stainless steel for a fuel cell separator with improved contact resistance according to an embodiment of the present disclosure includes, in percent by weight (wt %), at most of C (excluding 0), at most 3.0% of Si (excluding 0), at most 3.0% of Mn (excluding 0), 20 to 30% of Cr, 8 to 20% of Ni, at most 0.003% of S, at most 0.03% of P, at most 0.6% of Mo (excluding 0), at most 0.8% of Cu (excluding 0), 0.1 to 0.3% of N, at most 2.0% of W (excluding and the remainder being Fe and other inevitable impurities.