Garnet Precursor Microparticle pH Control

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Solution Overview

Problem

Conventional methods for producing yttrium aluminum garnet (YAG) microparticles struggle to achieve precise control over molar ratios of constituent elements, especially for particles smaller than 1 µm, and often result in contamination and uneven fluorescence characteristics due to physical impacts during processing.

Innovation Solution

A method involving the mixing of yttrium and aluminum ions with a basic substance in a thin film fluid between rotating processing surfaces, allowing control of pH to precisely regulate the molar ratios of yttrium and aluminum in the YAG precursor and final microparticles, achieved through a fluid processing apparatus that forms a thin film fluid for uniform mixing and separation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Length of moving object

If conventional ball mill pulverization is used to produce YAG microparticles, then particle size reduction is achieved, but contamination from ball mill materials and physical impact damage to crystal structure occur

Engineering Contradiction:
Improveparticle sizeVSAvoidcontamination and crystal damage
Core Design Contradiction:
Length of moving objectVSObject-affected harmful factors

Solution Approach 1:

The patent replaces the conventional mechanical ball mill pulverization system with a chemical precipitation system. YAG microparticles are formed through controlled chemical precipitation from aqueous solutions containing yttrium and aluminum ions, followed by heat treatment. This chemical approach eliminates mechanical contact that causes contamination and crystal structure damage while achieving the desired microparticle size of 1 µm or less.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent controls the precipitation process by adjusting pH parameters and ion concentration ratios in the aqueous solution. By controlling the molar ratio of yttrium to aluminum ions and the pH during precipitation, homogeneous YAG microparticles with controlled size and composition are obtained, avoiding the harmful effects of mechanical pulverization.

Inventive Principle:
Principle #35Parameter changes

2Stability of the object's composition

If solid phase reaction at high temperature is used to synthesize YAG, then crystal formation is achieved, but homogeneous control of molar ratios in microparticles becomes extremely difficult

Engineering Contradiction:
Improvecrystal formationVSAvoidmolar ratio homogeneity
Core Design Contradiction:
Stability of the object's compositionVSManufacturing precision

Solution Approach 1:

The patent performs preliminary mixing of yttrium and aluminum ions in aqueous solution before precipitation, ensuring homogeneous distribution of ions at the molecular level. This preliminary homogeneous mixing in the liquid phase, followed by controlled precipitation and heat treatment, guarantees homogeneous molar ratios in the final YAG microparticles, overcoming the inhomogeneity problem of solid phase reaction methods.

Inventive Principle:
Principle #10Preliminary action

3Length of moving object

If ball mill pulverization is used to reduce particle size to 1 µm or less, then fine microparticles are produced, but contamination from ball mill materials occurs

Engineering Contradiction:
Improveparticle sizeVSAvoidmaterial contamination
Core Design Contradiction:
Length of moving objectVSLoss of substance

Solution Approach 1:

The patent replaces mechanical ball mill pulverization with a chemical precipitation process that directly forms microparticles in the desired size range without requiring subsequent mechanical size reduction. This eliminates contact with ball mill materials that would cause contamination, while achieving particle sizes of 1 µm or less through controlled chemical synthesis and heat treatment.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

4Length of moving object

If physical impact during processing is applied to pulverize YAG, then particle size is reduced, but fluorescence characteristics and other intended properties cannot be expressed readily

Engineering Contradiction:
Improveparticle sizeVSAvoidfluorescence characteristics
Core Design Contradiction:
Length of moving objectVSReliability

Solution Approach 1:

The patent replaces mechanical impact pulverization with a chemical synthesis approach where YAG microparticles are formed through controlled precipitation and heat treatment. This preserves the crystal structure and fluorescence characteristics because the particles are formed chemically rather than being mechanically fractured, which would damage the crystal lattice and quench fluorescence properties.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of YAG microparticles with controlled molar ratios and smaller particle sizes, reducing contamination and energy consumption while maintaining high homogeneity and fluorescence characteristics, thus providing a cost-effective and stable production method.

Implementation Method 1

mixing of yttrium and aluminum ions with a basic substance in a thin film fluid between rotating processing surfaces, allowing control of pH to precisely regulate the molar ratios of yttrium and aluminum in the YAG precursor and final microparticles

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Implementation Method 2

control of pH to precisely regulate the molar ratios of yttrium and aluminum

Methodology Applied
Scientific EffectpH control:

Implementation Method 3

fluid processing apparatus that forms a thin film fluid for uniform mixing and separation

Methodology Applied
Scientific EffectThin film fluid formation: Thin Films

Implementation Method 4

mixing of yttrium and aluminum ions with a basic substance in a thin film fluid between rotating processing surfaces

Methodology Applied
Scientific EffectRotational mixing: Stirring

Implementation Method 5

subjecting the garnet microparticle precursor to heat treatment, thereby making a microparticle having a garnet structure

Methodology Applied
Scientific EffectHeat treatment: Heat Treatment

Data Source

PatentEP2808301B1Manufacturing processes for garnet precursor microparticles
Publication Date: 2018.06.27 M TECH CO LTD
  • EP2808301B1 patent drawingFigure 1
  • EP2808301B1 patent drawingFigure 2(A)~2(B)
  • EP2808301B1 patent drawingFigure 3(A)~3(B)

AI summary

The present invention addresses the problem of providing producing processes for garnet precursor microparticles (a precursor for microparticles of garnet structure) and microparticles of garnet structure. One of the processing processes comprises mixing ions of at least two elements with a basic substances that contain the at least two elements. The thin-film fluid is formed between at least two processing surfaces which are approachably and separably arranged facing each other with at least one of the processing surfaces rotating relative to the other. In the processing process, the precipitated microparticles are garnet precursor microparticles, and the molar ratio between the at least two elements in the garnet precursor microparticles is regulated by controlling the pH of the thin-film fluid after the mixing. Microparticles of garnet structure can be obtained by subjecting the garnet precursor microparticles to heat treatment. Specifically, the yttrium/ aluminum molar ratio of yttrium-aluminum-garnet (YAG) precursor microparticles is regulated by controlling the pH of the thin-film fluid after the mixing, YAG being an example of the crystal of garnet structure.