Potentiometric Gas Sensor Array with Temperature-Controlled Electrodes

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Solution Overview

Problem

Current solid-state potentiometric gas sensors lack selectivity and cross-sensitivity, particularly in distinguishing between NO and NO2 in combustion exhausts, requiring expensive electronics and complex designs, and are limited by the use of pseudo-reference electrodes that do not represent a true reference state.

Innovation Solution

The implementation of a gas sensor array with sensing electrodes maintained at different temperatures, allowing for fine-tuning of sensitivity and species selectivity, and using a mechanism to establish temperature differences between electrodes, including the use of heating and cooling elements to control electrode temperatures and improve signal interference.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If multiple sensing electrodes are used to detect different gas species, then measurement precision is improved, but device complexity increases

Engineering Contradiction:
Improvegas concentration detection accuracyVSAvoidsensor array configuration
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The patent applies parameter changes by maintaining different temperatures at different sensing electrodes to achieve selective detection. By controlling the temperature parameter of each electrode independently, the sensor can selectively determine different gas species (NO and NO2) without requiring multiple complex electrode configurations. This resolves the contradiction by improving measurement precision through temperature parameter control rather than increasing device complexity.

Inventive Principle:
Principle #35Parameter changes

2Adaptability or versatility

If temperature control mechanisms are added to sensing electrodes, then selectivity is improved, but device complexity increases

Engineering Contradiction:
Improvespecies selectivityVSAvoidtemperature control system
Core Design Contradiction:
Adaptability or versatilityVSDevice complexity

Solution Approach 1:

The patent implements local quality by applying temperature control locally to specific sensing electrodes rather than uniformly to the entire sensor. Each electrode can be maintained at a different temperature to optimize its response to particular gas species. This localized approach improves species selectivity while minimizing the overall complexity of the temperature control system.

Inventive Principle:
Principle #3Local quality

3Ease of manufacture

If pseudo-reference electrodes are used, then ease of manufacture is improved, but measurement precision deteriorates

Engineering Contradiction:
Improvesensor fabricationVSAvoidvoltage signal accuracy
Core Design Contradiction:
Ease of manufactureVSMeasurement precision

Solution Approach 1:

The patent extracts the reference electrode from the sensing environment by placing it in a separate chamber isolated from the gas mixture. This allows the use of a simple pseudo-reference electrode for ease of manufacture while maintaining measurement precision, as the reference electrode is not exposed to the varying gas concentrations that would affect its potential.

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances the ability to selectively determine NO and NO2 concentrations, reducing the number of electrodes needed, lowering costs, and improving device performance in harsh environments, while maintaining stability and accuracy in gas mixture analysis.

Implementation Method 1

a mechanism configured to establish a temperature difference between the at least two LCO electrodes

Methodology Applied
Scientific EffectResistive heating: Joule Heating

Implementation Method 2

Potentiometric gas sensors based on measuring the potential difference between a semiconducting metal oxide and a noble metal pseudo-reference electrode

Methodology Applied
Scientific EffectElectrochemical potential generation: Electrochemiluminescence

Data Source

PatentEP2201357B1Multifunctional potentiometric gas sensor array with an integrated temperature control and temperature sensors
Publication Date: 2022.09.21 UNIV OF FLORIDA RESEARCH FOUNDATION INC
  • EP2201357B1 patent drawingFigure 1~2
  • EP2201357B1 patent drawingFigure 3
  • EP2201357B1 patent drawingFigure 4

AI summary

Embodiments of the subject invention relate to a gas sensor and method for sensing one or more gases. An embodiment incorporates an array of sensing electrodes maintained at similar or different temperatures, such that the sensitivity and species selectivity of the device can be fine tuned between different pairs of sensing electrodes. A specific embodiment pertains to a gas sensor array for monitoring combustion exhausts and/or chemical reaction byproducts. An embodiment of the subject device related to this invention operates at high temperatures and can withstand harsh chemical environments. Embodiments of the device are made on a single substrate. The devices can also be made on individual substrates and monitored individually as if they were part of an array on a single substrate. The device can incorporate sensing electrodes in the same environment, which allows the electrodes to be coplanar and, thus, keep manufacturing costs low. Embodiments of the device can provide improvements to sensitivity, selectivity, and signal interference via surface temperature control.