Gas Sensor NOx Sensitivity via NO2 Reduction

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Solution Overview

Problem

The sensitivity of existing NO2 detection in gas sensors is lower than that of NO, primarily due to the slow diffusion of NO2 through the diffusion resistor section, which limits the detection of NOX concentration.

Innovation Solution

A gas sensor design incorporating a reduction section upstream of the diffusion resistor section, where NO2 is reduced to NO, and a second oxygen pump cell downstream to enhance sensitivity, with optional heating and catalysts to facilitate the reduction reaction, and a porous structure with higher porosity than the diffusion resistor section to minimize flow resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If a diffusion resistor section is used to control gas flow into the measurement chamber, then the measurement precision is improved, but the diffusion speed of NO2 is reduced, lowering the sensitivity

Engineering Contradiction:
Improvedetection accuracyVSAvoiddiffusion speed
Core Design Contradiction:
Measurement precisionVSSpeed

Solution Approach 1:

The reduction section is placed upstream of the diffusion resistor section to convert NO2 to NO before the gas enters the measurement chamber. This preliminary conversion action ensures that the gas species with faster diffusion characteristics (NO) passes through the diffusion resistor, thereby maintaining both measurement precision and detection sensitivity.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention changes the chemical parameter of the gas by converting NO2 to NO through the reduction section. This parameter change (chemical composition transformation) allows the gas to have different diffusion properties, resolving the contradiction between measurement precision and diffusion speed.

Inventive Principle:
Principle #35Parameter changes

2Measurement precision

If the sensitivity to NO2 is improved by reducing it to NO before measurement, then the detection accuracy is improved, but the device complexity increases due to additional components

Engineering Contradiction:
ImproveNO2 detection sensitivityVSAvoidsensor structure
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The reduction section is integrated with the existing sensor structure, combining the reduction function with the measurement chamber system. This merging approach improves NO2 detection sensitivity while minimizing the increase in device complexity by utilizing the existing structural framework.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The reduction section serves multiple functions: it converts NO2 to NO for improved detection, and also prepares the gas composition for accurate measurement by the subsequent oxygen pump cell. This multi-functionality justifies the additional component by providing multiple benefits within a single structural addition.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This design enhances the sensitivity of the gas sensor for NOX detection by ensuring NO2 is converted to NO before passing through the diffusion resistor, thereby improving detection speed and accuracy without limiting the flow of NOX.

Implementation Method 1

a reduction section provided upstream of the diffusion resistor section and reducing NO2 contained in the object gas introduced into the first measurement chamber to NO

Methodology Applied
Scientific EffectReduction reaction: Reduction

Implementation Method 2

a diffusion resistor section which limits flow of the object gas therethrough

Methodology Applied
Scientific EffectFlow resistance: Drag

Implementation Method 3

Oxygen contained in the exhaust gas introduced into the first measurement chamber is pumped out to the outside by the cell, whereby the concentration of oxygen remaining in the exhaust gas introduced into the second measurement chamber is adjusted

Methodology Applied
Scientific EffectElectrochemical reaction: Electrolysis

Implementation Method 4

NO is decomposed to nitrogen and oxygen by the catalytic action of an electrode formed of noble metal such as Pt or Rh

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 5

a heater for heating the reduction section may be provided

Methodology Applied
Scientific EffectThermal heating: Heating

Data Source

PatentEP2469274B1Gas sensor
Publication Date: 2018.08.29 NITERRA CO LTD
  • EP2469274B1 patent drawingFigure 1
  • EP2469274B1 patent drawingFigure 2

AI summary

[Objective] To provide a gas sensor which can improve the sensitivity to NO x . [Means for Solution] A reduction section 18 for reducing NO 2 contained in exhaust gas to NO is provided on the upstream side of a first diffusion resistor section 103 provided to limit the flow of the exhaust gas into a first measurement chamber 101. When NO x passes through the first diffusion resistor section 103, NO 2 which is greater in molecular weight than NO is lower in the degree of diffusion than NO. Since NO 2 is reduced to NO at the reduction section 18, the exhaust gas passing through the first diffusion resistor section 103 hardly contains NO 2 . Therefore, the speed of flow of NO x through the first diffusion resistor section 103 is not limited by NO 2 , whereby sensitivity for detection of NO x can be improved.