Glatiramer Acetate Microparticle Solvent Removal

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Solution Overview

Problem

Existing processes for preparing microparticles containing glatiramer acetate result in high levels of residual organic solvents like dichloromethane, which are toxic and carcinogenic, violating regulatory limits for pharmaceutical compositions.

Innovation Solution

A modified double emulsification process involving the application of vacuum and/or air stream during solvent evaporation in the water-in-oil-in-water double emulsion step to reduce residual organic solvent levels to regulatory-acceptable limits without compromising the microparticles' morphology, binding percentage, or release profile.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If traditional solvent evaporation method is used, then microparticle formation is achieved, but residual organic solvent levels are high (toxic and carcinogenic)

Engineering Contradiction:
Improveresidual organic solvent levelsVSAvoidregulatory compliance
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The patent extracts and removes the harmful organic solvent (dichloromethane) from the microparticle system through enhanced evaporation methods. The process specifically targets and eliminates the residual solvent while preserving the therapeutic microparticle structure, reducing solvent levels from problematic concentrations to below 600 ppm.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the evaporation parameters by applying vacuum conditions and/or air streams during the solvent removal step. This modifies the physical conditions of evaporation to accelerate solvent removal and achieve regulatory compliance levels while maintaining microparticle integrity.

Inventive Principle:
Principle #35Parameter changes

2Object-affected harmful factors

If vacuum and air stream are applied during evaporation, then residual solvent levels are reduced, but process complexity increases

Engineering Contradiction:
Improveresidual organic solvent levelsVSAvoidevaporation process equipment
Core Design Contradiction:
Object-affected harmful factorsVSDevice complexity

Solution Approach 1:

The patent employs pneumatic methods by introducing air streams during the evaporation process to enhance solvent removal. This uses gas flow dynamics to accelerate dichloromethane evaporation and achieve regulatory compliance levels more effectively than passive evaporation alone.

Inventive Principle:
Principle #29Pneumatics and hydraulics

Solution Approach 2:

The patent creates a controlled atmospheric environment during evaporation by applying vacuum and/or introducing air streams. This modified atmosphere facilitates faster and more complete solvent removal while protecting the microparticle formulation from degradation.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

3Object-affected harmful factors

If extended evaporation time is used, then residual solvent levels are reduced, but manufacturing time increases

Engineering Contradiction:
Improveresidual organic solvent levelsVSAvoidmanufacturing cycle time
Core Design Contradiction:
Object-affected harmful factorsVSProductivity

Solution Approach 1:

The patent applies preliminary action by implementing vacuum and air stream conditions during the evaporation phase to accelerate solvent removal. This proactive approach to solvent elimination reduces the time required to achieve regulatory compliance levels compared to traditional extended evaporation methods.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent exploits phase transition dynamics by using vacuum and air streams to enhance the evaporation (liquid to gas) of dichloromethane. This accelerates the phase transition process, rapidly reducing residual solvent levels without requiring extended processing times.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively reduces residual organic solvent levels in microparticles to below 600 ppm, ensuring compliance with regulatory standards while maintaining therapeutic efficacy and reducing side effects, thus providing a safer and more effective long-acting parenteral composition for multiple sclerosis treatment.

Implementation Method 1

The organic solvent is slowly evaporated by stirring the double emulsion in a fume hood

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 2

application of vacuum and/or air stream to the double water-in-oil-in-water double emulsion results in a product having reduced levels of organic solvent

Methodology Applied
Scientific EffectVacuum: Vacuum

Data Source

PatentUS12097292B2Process for preparing microparticles containing glatiramer acetate
Publication Date: 2024.09.24 MAPI PHARMA LTD

AI summary

The present invention provides an improved process for preparing microparticles containing glatiramer acetate having low levels of residual organic solvent(s), in particular dichloromethane. The microparticles are incorporated into long acting parenteral pharmaceutical compositions in depot form that are suitable for subcutaneous or intramuscular implantation or injection, and that may be used to treat multiple sclerosis.