Ethylene Glycol Refining via Esterification of Acid Contaminants

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Solution Overview

Problem

Existing methods for refining crude ethylene glycol streams struggle to efficiently remove acid contaminants like methoxyacetic acid and glycolic acid, which have similar boiling points to desired products, leading to inefficiencies and potential product loss due to the addition of bases or costly distillation processes.

Innovation Solution

A process that reacts acid contaminants with monoethylene glycol and diethylene glycol to form esters, which are easier to separate, using catalysts like silica, resin, or zeolites, and incorporates water removal steps to drive the equilibrium towards complete conversion, avoiding the addition of new components and reducing equipment size.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If distillation is used to remove acid contaminants, then separation is achieved, but equipment complexity and cost increase due to similar boiling points

Engineering Contradiction:
Improveremoval of acid contaminantsVSAvoiddistillation equipment
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The invention changes the chemical state of acid contaminants by converting them into esters with different physical properties (higher boiling points). This parameter change from acid form to ester form enables easier separation through standard distillation equipment without requiring complex multi-column systems, thereby resolving the contradiction between removal effectiveness and equipment complexity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention introduces an esterification reaction as an intermediary step that transforms acid contaminants into esters. This intermediary chemical transformation serves as a bridge between the crude glycol stream and the final purified product, enabling separation through conventional distillation rather than requiring complex specialized equipment

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If base is added to neutralize acid contaminants, then acid removal is improved, but system complexity increases and product loss occurs

Engineering Contradiction:
Improveacid contaminant removalVSAvoidproduct loss
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

Instead of treating acid contaminants as harmful substances to be neutralized and discarded, the invention converts them into beneficial esters that can be separated and potentially reused. The harmful acid components are transformed into useful byproducts, eliminating the need for base addition and associated product losses while maintaining system simplicity

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The invention extracts acid contaminants from the glycol stream through esterification, separating them into a distinct ester phase. This extraction approach removes the harmful acidic components without requiring base neutralization, thereby preventing product loss while achieving the desired purification

Inventive Principle:
Principle #2Taking out (Extraction)

3Manufacturing precision

If extensive distillation is performed to meet specifications, then product purity is improved, but energy consumption increases

Engineering Contradiction:
Improveproduct purityVSAvoiddistillation energy
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

The invention performs preliminary esterification of acid contaminants before the final distillation step. This preliminary chemical treatment converts difficult-to-separate acid components into easily separable esters, reducing the burden on subsequent distillation operations and significantly lowering the energy required to achieve specification-grade purity

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively reduces acid contaminants to meet product specifications with minimal product loss, allows for recycling of esters, and optimizes operating conditions of upstream hydrogenation processes, enhancing catalyst stability and yield.

Implementation Method 1

the at least one reaction zone comprises a catalyst to promote the esterification reaction

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

incorporates water removal steps to drive the equilibrium towards complete conversion

Methodology Applied
Scientific EffectEquilibrium shift through product removal:

Data Source

PatentEP4208435B1Process for refining a crude ethylene glycol stream
Publication Date: 2025.12.10 JOHNSON MATTHEY DAVY TECHNOLOGIES LTD
  • EP4208435B1 patent drawingFigure 1~2
  • EP4208435B1 patent drawingFigure 3~4
  • EP4208435B1 patent drawingFigure 5

AI summary

A process for refining a crude ethylene glycol stream comprising monoethylene glycol and at least one acid contaminant is disclosed. The process comprises reacting the acid contaminant with the monoethylene glycol in at least one reaction zone to form an ester and removing the ester in a separation step.