Graded Absorber Layer for Flexible Thin-Film Photovoltaics

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Solution Overview

Problem

High-temperature deposition processes in thin-film photovoltaic device manufacturing restrict substrate material options, lead to contamination, and increase energy costs, while also limiting the use of flexible substrates and roll-to-roll production due to the need for high substrate temperatures and surface treatments.

Innovation Solution

A method involving a five-stage deposition process at temperatures between 350°C and 550°C, with specific atomic ratio adjustments and material flux rates, to create a graded absorber layer with improved crystalline structure and reduced impurity diffusion, allowing for high-efficiency photovoltaic devices on flexible substrates without the need for barrier layers or extensive surface treatments.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If high-temperature deposition processes are used, then photovoltaic device efficiency is improved, but substrate material options are restricted and energy costs increase

Engineering Contradiction:
Improvephotovoltaic device efficiencyVSAvoidsubstrate temperature
Core Design Contradiction:
Manufacturing precisionVSTemperature

Solution Approach 1:

The patent applies parameter changes by systematically varying deposition parameters including substrate temperature (reducing from conventional high temperatures to 350-550°C), deposition rate, atomic ratio of elements, and multi-stage deposition sequences to achieve high efficiency photovoltaic devices at lower temperatures

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent implements local quality through compositional grading within the absorber layer, creating depth-dependent variations in element distribution (Cu, In, Ga, Se) to optimize local electronic properties and carrier collection efficiency, resulting in high device efficiency without requiring high substrate temperatures

Inventive Principle:
Principle #3Local quality

2Manufacturing precision

If high-temperature deposition processes are used, then photovoltaic device efficiency is improved, but energy costs increase

Engineering Contradiction:
Improvephotovoltaic device efficiencyVSAvoidenergy costs
Core Design Contradiction:
Manufacturing precisionVSUse of energy by stationary object

Solution Approach 1:

The patent reduces energy consumption by changing the temperature parameter from conventional high temperatures to 350-550°C deposition range, while compensating for the reduced thermal energy through optimized deposition rates, atomic ratios, and multi-stage deposition processes that maintain high device efficiency

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If high-temperature deposition processes are used, then photovoltaic device efficiency is improved, but contamination increases

Engineering Contradiction:
Improvephotovoltaic device efficiencyVSAvoidcontamination
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent reduces contamination by lowering the substrate temperature parameter to 350-550°C, which minimizes thermal diffusion and impurity migration. The controlled low-temperature process prevents substrate material diffusion into the absorber layer and reduces oxidation, eliminating the need for barrier layers

Inventive Principle:
Principle #35Parameter changes

4Manufacturing precision

If high-temperature deposition processes are used, then photovoltaic device efficiency is improved, but flexible substrate usage is restricted

Engineering Contradiction:
Improvephotovoltaic device efficiencyVSAvoidsubstrate material options
Core Design Contradiction:
Manufacturing precisionVSAdaptability or versatility

Solution Approach 1:

The patent expands substrate material options by changing the temperature parameter to 350-550°C, which is compatible with flexible substrates such as plastic foils that cannot withstand high temperatures. This enables deposition on diverse substrates including glass, metal foils, and flexible plastics

Inventive Principle:
Principle #35Parameter changes

5Manufacturing precision

If high-temperature deposition processes are used, then photovoltaic device efficiency is improved, but surface treatments are required

Engineering Contradiction:
Improvephotovoltaic device efficiencyVSAvoidsurface treatments
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent eliminates surface treatment requirements by optimizing the deposition parameter of substrate temperature to 350-550°C, which enables direct deposition of high-quality absorber layers without the need for barrier layers or extensive surface treatments, simplifying the manufacturing process

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method enables the production of high-efficiency photovoltaic devices with improved crystalline structure and reduced recombination, achieving efficiencies comparable to silicon wafer-based devices while using flexible substrates and enabling low-cost, low-energy roll-to-roll production.

Implementation Method 1

deposition of semiconductor material as a thin film onto a substrate

Methodology Applied
Scientific EffectVapor deposition: Physical Vapour Deposition

Data Source

PatentEP3454362B1Thin-film photovoltaic device with grading
Publication Date: 2022.06.01 FLISOM AG
  • EP3454362B1 patent drawingFigure 1~2C
  • EP3454362B1 patent drawingFigure 3A~3C
  • EP3454362B1 patent drawingFigure 4A~4B

AI summary

A thin-film photovoltaic device (100) comprising a flexible substrate (110) and an absorber layer (130), wherein said absorber layer (130) is made of an ABC chalcogenide material, including ABC chalcogenide material quaternary, pentanary, or multinary variations, wherein A represents elements in group 11 of the periodic table of chemical elements as defined by the International Union of Pure and Applied Chemistry including Cu and Ag, B represents elements in group 13 of the periodic table including In, Ga and Al, and C represents elements in group 16 of the periodic table including S, Se and Te, wherein said ABC chalcogenide material comprises In and Ga elements, characterized in that a compositional analysis of smoothed Ga / (Ga + In) ratio data across the thickness of said absorber layer forms a Ga / (Ga + In) ratio curve (500) in which, starting from a light-exposed side of said absorber layer, said Ga / (Ga + In) ratio curve (500) comprises at least two regions (501, 502) comprising: a. a front grading region (501) of decreasing Ga / (Ga + In) ratio where a light-exposed side of said front grading region has a Ga / (Ga + In) value that is less than 0.5 and where the amplitude of the Ga / (Ga + In) value in said front grading region is less than 0.25 and greater than 0.1; b. a back grading region (502), adjacent to said front grading region (501) and located between said front grading region (501) and the back side of the absorber layer opposite the light-exposed side, of overall increasing Ga / (Ga + In) ratio where: i. over the light-exposed half side of said back grading region (502) the value of Ga / (Ga + In) increases by less than 0.20.