Conductive Interference Pigments via Graphene Coating

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Solution Overview

Problem

Existing electrically conductive pigments either have good color properties with indeterminate electrical properties or satisfactory conductivity with achromatic coloration, failing to achieve both high electrical conductivity and attractive coloration necessary for reliable shielding or antistatic applications, and often require additional colorants that increase electrical resistance.

Innovation Solution

Development of electrically conductive, colored interference pigments with a platelet-shaped carrier coated by an outermost layer consisting of at least 95% crystalline carbon in the form of graphite and/or graphene, which enhances electrical conductivity and provides high hiding power without the need for additional colorants.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If carbon black or graphite is used as conductive filler, then electrical conductivity is improved, but the materials darken which is perceived as a disadvantage

Engineering Contradiction:
Improveelectrical conductivityVSAvoiddarkening of materials
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent uses a composite structure with a transparent substrate (mica or silica) coated with a thin layer of crystalline carbon (graphite or graphene). This composite approach combines the transparency of the substrate with the conductivity of the carbon layer, achieving both optical clarity and electrical functionality without the severe darkening effect of bulk carbon black.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

Instead of using carbon throughout the entire pigment volume, the patent applies carbon only as a thin outermost layer (a few nanometers to micrometers thick) on the surface of transparent substrate particles. This localized application provides sufficient conductivity at the surface while maintaining the transparency of the bulk material.

Inventive Principle:
Principle #3Local quality

2Illumination intensity

If transparent substrates with conductive coatings are used, then transparency and light color are improved, but inherent color is achromatic or light gray requiring additional colorants

Engineering Contradiction:
Improvetransparency and light colorVSAvoidneed for additional colorants
Core Design Contradiction:
Illumination intensityVSDevice complexity

Solution Approach 1:

The patent utilizes interference effects through precise control of layer thicknesses in the multilayer coating structure. By adjusting the optical thickness of dielectric layers and the carbon layer, specific wavelengths of light are enhanced or suppressed, producing vibrant interference colors without requiring organic colorants. This optical interference mechanism generates color directly from the structural properties of the coating.

Inventive Principle:
Principle #32Color changes

3Ease of manufacture

If colorants are added to achieve colorful conductive media, then color properties are improved, but electrical resistance increases significantly

Engineering Contradiction:
Improvecolor propertiesVSAvoidelectrical resistance
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent replaces organic colorants with optical interference effects generated by the multilayer coating structure. The interference colors arise from the constructive and destructive interference of light waves reflected from different interfaces within the coating, providing vibrant colors that do not interfere with electrical conductivity since no additional non-conductive colorant materials are introduced.

Inventive Principle:
Principle #32Color changes

Solution Approach 2:

The multilayer composite structure (substrate + dielectric layers + carbon layer) generates color optically rather than through pigment absorption. This allows the conductive carbon component to remain the primary coloring agent, maintaining conductivity while achieving colorful appearance through the optical properties of the layered structure.

Inventive Principle:
Principle #40Composite materials

4Quantity of substance

If pigment concentration is increased to compensate for reduced conductivity, then color intensity is improved, but processing problems occur due to technical limits

Engineering Contradiction:
Improvepigment concentrationVSAvoidprocessing problems
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent changes the fundamental parameters of the conductive component by using crystalline carbon (graphite or graphene) with superior electrical properties compared to amorphous carbon black. This parameter change in carbon structure allows achieving the same or better conductivity at lower pigment concentrations, avoiding processing issues associated with high pigment loading while maintaining or enhancing color intensity.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The pigments achieve specific powder resistances of no more than 1x10^6 ohm*cm, enabling reliable electrical properties while displaying attractive colors, and can be used to create coatings with high gloss, chroma, and hiding power on both white and black substrates.

Implementation Method 1

electrically conductive pigments which have an outermost layer containing crystalline carbon in the form of graphite and/or graphene

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Implementation Method 2

colored interference pigments... optically variable behavior... high gloss, chroma, and hiding power

Methodology Applied
Scientific EffectOptical interference: Interference

Implementation Method 3

by pyrolytic decomposition of the carbon-containing compound

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Data Source

PatentEP3230385B1Electrically conductive, colored interference pigments
Publication Date: 2020.04.15 MERCK PATENT GMBH
  • EP3230385B1 patent drawingFigure 1
  • EP3230385B1 patent drawingFigure 2
  • EP3230385B1 patent drawingFigure 3

AI summary

The present invention relates to electrically conductive, colored interference pigments, in particular platelet-type interference pigments, which have an outermost layer that contains crystalline carbon in the form of graphite and/or graphene. The invention also relates to a method for producing such pigments and the use of the thus produced pigments.