Reduced Graphene Oxide Coating for Recyclable Liquid Cartons

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Solution Overview

Problem

Existing packaging materials for liquid food containers, particularly those aiming to replace aluminum foil, face challenges in achieving cost-effectiveness, recyclability, and maintaining gas barrier properties under varying moisture conditions, while being mechanically robust and suitable for aseptic packaging.

Innovation Solution

A method involving coating a substrate material with a layer of reduced graphene oxide using an aqueous dispersion, followed by drying, to create a gas-barrier coating, which is then laminated with additional polymer layers to form a laminated packaging material.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If aluminum foil is used as barrier material, then gas barrier properties are superior, but recyclability and cost-effectiveness deteriorate

Engineering Contradiction:
Improvegas barrier propertiesVSAvoidrecyclability and cost-effectiveness
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes the material parameter from aluminum foil to a polymer dispersion coating (such as polyvinylidene chloride or ethylene-vinyl alcohol copolymer), transforming the barrier material from a metal to an organic polymer that can be applied as a thin coating layer, thereby achieving comparable barrier properties with improved recyclability and cost-effectiveness

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite structure by combining polymer dispersion coating with cellulose-based substrate and lamination layers, forming a multi-layer composite material that achieves superior gas barrier properties while maintaining recyclability and cost-effectiveness through the synergistic combination of different materials

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If polymer barrier coatings are applied, then recyclability improves, but gas barrier properties deteriorate under varying moisture conditions

Engineering Contradiction:
ImproverecyclabilityVSAvoidgas barrier properties under moisture
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent employs a multi-layer composite structure where the polymer dispersion coating is combined with cellulose-based substrates and additional lamination layers, creating a synergistic system where each layer compensates for the others' weaknesses regarding moisture sensitivity while maintaining gas barrier properties

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent applies a polymer dispersion coating as a pre-treatment layer before final lamination, creating a preliminary barrier that is optimized to work in conjunction with subsequent layers to maintain gas barrier properties under varying moisture conditions throughout the packaging structure

Inventive Principle:
Principle #10Preliminary action

3Device complexity

If thin barrier coatings are used, then material complexity reduces, but mechanical robustness deteriorates

Engineering Contradiction:
Improvematerial complexityVSAvoidmechanical robustness
Core Design Contradiction:
Device complexityVSStrength

Solution Approach 1:

The patent creates a composite material system where thin polymer dispersion coatings are applied to cellulose-based substrates and combined with lamination layers, achieving the desired barrier properties with minimal material while the composite structure itself provides the necessary mechanical robustness through the combined strength of multiple layers

Inventive Principle:
Principle #40Composite materials

4Reliability

If multilayer films are combined to achieve high barrier properties, then gas barrier performance improves, but manufacturing complexity increases

Engineering Contradiction:
Improvegas barrier performanceVSAvoidmanufacturing complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies polymer dispersion coating as a preliminary step before final lamination, creating a pre-formed barrier layer that simplifies subsequent manufacturing steps by reducing the number of separate coating operations needed and enabling more efficient production processes

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting packaging material provides excellent gas barrier properties, is cost-effective, recyclable, and maintains integrity under mechanical stress, enabling long-term aseptic storage of liquid foods without aluminum foil.

Implementation Method 1

an aqueous dispersion, followed by drying, to create a gas-barrier coating

Methodology Applied
Scientific EffectDispersion: Dispersion (of waves)

Implementation Method 2

coating a substrate material with a layer of reduced graphene oxide using an aqueous dispersion

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 3

drying the wet coated substrate material obtained from step c), by forced evaporation

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 4

which is then laminated with additional polymer layers to form a laminated packaging material

Methodology Applied
Scientific EffectLamination: Lamination

Data Source

PatentEP4019465B1Barrier-coated cellulosebased substrate, laminated packaging material and packaging container comprising the cellulosebased substrate
Publication Date: 2026.01.28 TETRA LAVAL HOLDINGS & FINANCE SA
  • EP4019465B1 patent drawingFigure 1a~1b
  • EP4019465B1 patent drawingFigure 2a~2b
  • EP4019465B1 patent drawingFigure 3~4a

AI summary

The present invention relates to a method for manufacturing a gas-barrier coated substrate material (10a; 10b), coated with a layer of reduced graphene oxide. The invention further relates to laminated packaging materials (20a; 20b) comprising the barrier-coated substrate material (10a; 10b), in particular intended for liquid carton food packaging, and to liquid carton packaging containers comprising the laminated packaging material.