Graphene Oxide Membrane Isotopic Water Separation

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Solution Overview

Problem

Nuclear power plants face challenges in separating and removing tritiated water and heavy water from waste streams, as existing technologies are inefficient in distinguishing and isolating these isotopic forms, which are essential for environmental safety and resource recovery.

Innovation Solution

The use of graphene oxide membranes, with specific thickness and interlayer spacing, to separate isotopic forms of water by exploiting differences in permeability based on chemical and physical properties, implemented in a reflux cascade filtration system to achieve efficient separation of light, heavy, and super heavy water.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional filtration methods are used to separate isotopic forms of water, then the process is simple to implement, but the separation efficiency is insufficient to effectively distinguish and isolate tritiated water and heavy water from light water

Engineering Contradiction:
Improveisotopic separation precisionVSAvoidfiltration system complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent employs graphene oxide membranes with precisely controlled porous structures and interlayer spacings (0.3-1.0 micrometers) to achieve isotopic separation. The porous nature of the membrane allows selective permeation based on molecular size and interaction differences between light water, heavy water, and tritiated water molecules, thereby achieving high separation precision without requiring overly complex system architecture

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The invention utilizes composite membrane structures combining graphene oxide layers with specific interlayer spacing configurations. This composite material approach leverages the unique properties of graphene oxide (high strength, controlled porosity, and selective permeability) to achieve effective isotopic separation while maintaining structural integrity and operational feasibility

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If the graphene oxide membrane thickness is increased to improve separation efficiency, then the separation performance improves, but the water flux and productivity decrease

Engineering Contradiction:
Improveisotopic separation efficiencyVSAvoidwater flux through membrane
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent systematically optimizes the membrane thickness parameter within the range of 0.1-10 micrometers to achieve the optimal balance between separation efficiency and water flux. By controlling this critical parameter, the system attains sufficient isotopic separation performance while maintaining adequate productivity, avoiding both excessive thickness (which would reduce flux) and insufficient thickness (which would reduce separation efficiency)

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If multiple filtration modules are implemented in a reflux cascade system to achieve efficient separation, then the isotopic separation effectiveness is enhanced, but the system complexity and operational difficulty increase

Engineering Contradiction:
Improveisotopic separation effectivenessVSAvoidsystem operational simplicity
Core Design Contradiction:
Manufacturing precisionVSEase of operation

Solution Approach 1:

The patent divides the separation system into multiple filtration modules arranged in a reflux cascade configuration, with each module containing graphene oxide membranes with specific interlayer spacings (0.5-2.0 nanometers). This segmentation allows the system to achieve high separation effectiveness through staged purification, where each module contributes to progressively removing isotopic contaminants, while the modular design enables manageable operation and maintenance

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The system effectively reduces the concentration of heavy and super heavy water, allowing for safe environmental release of light water and potential reuse or storage of heavy water, enhancing nuclear power plant operations and environmental safety.

Implementation Method 1

the graphene oxide membrane(s) can be used to separate the gas into a permeate and a retentate, wherein the permeate comprises an increased concentration of light water relative to the retentate

Methodology Applied
Scientific EffectPermeation: Permeation

Implementation Method 2

separate isotopic forms of water by exploiting differences in permeability based on chemical and physical properties

Methodology Applied
Scientific EffectIsotopic separation based on permeability differences:

Data Source

PatentEP3036197B1Systems and methods for isotopic water separation
Publication Date: 2018.12.19 P&T GLOBAL SOLUTIONS LLC
  • EP3036197B1 patent drawingFigure 1
  • EP3036197B1 patent drawingFigure 2
  • EP3036197B1 patent drawingFigure 3

AI summary

Methods and systems for filtering water according to its isotopic forms. In some embodiments, a stream of water comprising at least two distinct isotopic forms of water may be directed into one or more filtration modules comprising a graphene oxide membrane. The graphene oxide membrane(s) may be used to separate the stream into a permeate and a retentate, wherein the permeate comprises an increased concentration of light water relative to the retentate.