Graphite Ionizer Tube for Secondary Ion Mass Spectrometer

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Conventional primary ion sources for secondary ion mass spectrometers face challenges in achieving high performance and cost-effectiveness, with issues such as diffuse ion-optical objects, compromised beam focus, and non-reusable designs due to stringent sealing requirements.

Innovation Solution

A primary ion source design featuring a unitary graphite or graphite-containing ionizer tube and reservoir base with a conical or frustoconical aperture, allowing for precise cesium ionization and improved sealing through graphite materials, enabling smaller beam sizes and increased ion current while facilitating reusability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a metal swage-type seal is used to ensure sealing between reservoir portions, then sealing reliability is improved, but the ion source becomes non-reusable and requires precise control of sealing force

Engineering Contradiction:
Improvesealing reliabilityVSAvoidreusability
Core Design Contradiction:
ReliabilityVSAdaptability or versatility

Solution Approach 1:

The patent changes the material parameter from metal to graphite for the ionizer section. Graphite's unique property of becoming pliable at high temperatures allows it to conform to the reservoir cavity shape, creating a reliable seal without requiring precise control of sealing force. This material parameter change enables both reliable sealing and reusability, as the graphite can be reheated and reformed for multiple uses.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs a composite structure where the ionizer section is made of graphite while the reservoir portions remain metal. This combination leverages the thermal stability and structural integrity of metal with the temperature-dependent sealing properties of graphite, achieving both reliable sealing and reusability through the synergistic properties of the composite material system.

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If a unitary graphite ionizer tube and reservoir base are used, then manufacturing complexity is reduced and reusability is enabled, but sealing precision may be compromised

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidsealing precision
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent utilizes the temperature-dependent physical parameter of graphite, which transitions from rigid at room temperature to pliable at high temperatures. This parameter change allows the graphite ionizer section to be easily manufactured and installed, then formed precisely against the reservoir cavity when heated, achieving both manufacturing simplicity and sealing precision through the same material's different states.

Inventive Principle:
Principle #35Parameter changes

3Power

If a larger ionizer aperture is used, then ion current is increased, but beam focus is compromised and beam size increases

Engineering Contradiction:
Improveion currentVSAvoidbeam focus
Core Design Contradiction:
PowerVSManufacturing precision

Solution Approach 1:

The patent employs a composite material approach by coating the inner surface of the graphite ionizer tube with a refractory material. This composite structure allows the aperture to maintain a precise geometric shape defined by the refractory coating, ensuring good beam focus, while the graphite body provides thermal stability and can be heated to high temperatures to increase ion current without compromising the aperture geometry.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The design achieves sharper beam focus, higher ion current, and cost-effective reusability by utilizing graphite's refractory properties and softness for precise sealing, enhancing analytical performance and reducing operational costs.

Implementation Method 1

The reservoir body is heated to cause cesium carbonate vapor to diffuse up the narrow tube and decompose as the vapor reaches the strongly-heated ionizer section

Methodology Applied
Scientific EffectVaporization: Evaporation

Implementation Method 2

The ionizer section is strongly heated (e.g., by a combination of electron bombardment and radiative heating from the electron emitting filament) and cesium atoms that impact the tungsten ionizer plate evaporate almost 100% as positive ions

Methodology Applied
Scientific EffectThermal ionization: Ionisation

Implementation Method 3

The ionizer section is strongly heated (e.g., by a combination of electron bombardment and radiative heating from the electron emitting filament)

Methodology Applied
Scientific EffectThermionic emission: Thermionic Emission

Data Source

PatentEP3207636B1Cesium primary ion source for secondary ion mass spectrometer
Publication Date: 2019.12.04 THE ARIZONA BOARD OF REGENTS ON BEHALF OF THE UNIV OF ARIZONA
  • EP3207636B1 patent drawingFigure 1A~1B
  • EP3207636B1 patent drawingFigure 1C~1D
  • EP3207636B1 patent drawingFigure 2

AI summary

A primary ion source subassembly for use with a secondary ion mass spectrometer may include a unitary graphite ionizer tube and reservoir base. A primary ion source may include a capillary insert defining an ionizer aperture. An ionizer aperture may be centrally arranged in an outwardly protruding conical or frustoconical surface, and may be overlaid with a refractory metal coating or sheath. Parameters including ionizer surface shape, ionizer materials, ionizer temperature, and beam stop plate orifice geometry may be manipulated to eliminate ghost images. A graphite tube gasket with a dual tapered surface may promote sealing of a source material cavity.