Heat-shrinkable Polyester Film Thickness Control

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Solution Overview

Problem

Conventional heat-shrinkable polyester-based films either have low heat-resistant properties, high irregularity in thickness, or inadequate shrinkage ratios in specific directions, making them unsuitable for applications requiring high heat-shrinkage ratios and uniform thickness.

Innovation Solution

A heat-shrinkable polyester-based film is developed with a composition of 90 mol% ethylene terephthalate units, processed through a transverse stretching method where preheating is done at (Tg+40° C.) to (Tg+70° C.), followed by transverse stretching at (Tg+5° C.) to (Tg+40° C.), and further stretching at (Tg−10° C.) to (Tg+15° C.), achieving high heat-shrinkage ratios and reduced thickness irregularity in both width and longitudinal directions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Shape

If amorphous polyester raw material is used to increase shrinkage ratio, then the shrinkage ratio increases, but heat resistant property deteriorates and thickness irregularity increases

Engineering Contradiction:
Improveshrinkage ratioVSAvoidheat resistant property
Core Design Contradiction:
ShapeVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters of the polyester resin by limiting amorphous components to 5 mol% or less and setting ethylene terephthalate content to 90-100 mol%, thereby achieving both high heat resistance and controlled shrinkage properties through precise compositional control

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies different stretching ratios in different directions (higher transverse stretching ratio of 3.0-5.0 times versus longitudinal stretching ratio of 1.0-2.0 times) to create directional shrinkage characteristics while maintaining overall thermal stability

Inventive Principle:
Principle #3Local quality

2Shape

If amorphous polyester raw material is used to increase shrinkage ratio, then the shrinkage ratio increases, but thickness uniformity deteriorates

Engineering Contradiction:
Improveshrinkage ratioVSAvoidthickness uniformity
Core Design Contradiction:
ShapeVSManufacturing precision

Solution Approach 1:

The patent modifies the resin composition parameters by using predominantly crystalline polyester (ethylene terephthalate 90-100 mol%) with minimal amorphous content, which provides more uniform molecular structure and predictable shrinkage behavior, thereby improving thickness uniformity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies differential stretching ratios where transverse stretching (3.0-5.0 times) is greater than longitudinal stretching (1.0-2.0 times), creating controlled anisotropic shrinkage that maintains uniform thickness distribution across the film

Inventive Principle:
Principle #3Local quality

3Shape

If transverse stretching is performed at high temperature to achieve high shrinkage ratio, then shrinkage ratio increases, but thickness irregularity increases

Engineering Contradiction:
Improveshrinkage ratioVSAvoidthickness irregularity
Core Design Contradiction:
ShapeVSManufacturing precision

Solution Approach 1:

The patent optimizes the temperature parameter within a controlled range (Tg+40°C to Tg+70°C for preheating, Tg+5°C to Tg+40°C for stretching) to balance molecular mobility for shrinkage expression while preventing excessive thermal expansion that would cause thickness irregularity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent performs preheating at higher temperature (Tg+40°C to Tg+70°C) before the actual stretching operation, which gradually activates the polymer chains and prepares the material for controlled shrinkage, preventing sudden deformation and thickness variation

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The film exhibits a heat-shrinkage ratio of 50% to 75% in the width direction, -6% to 14% in the longitudinal direction, and maximum heat shrinkage stress of 4 MPa to 13 MPa, with a crystallinity degree of 1% to 15%, ensuring effective shrinkage and stability for label applications.

Implementation Method 1

the heat-shrinkage ratio in a width direction measured by shrinking the film for 10 seconds in 90° C. hot water is 50% or more and 75% or less

Methodology Applied
Scientific EffectThermal contraction: Thermal Contraction

Implementation Method 2

the heat-shrinkage ratio in a longitudinal direction measured by shrinking the film for 10 seconds in 90° C. hot water is −6% or more and 14% or less

Methodology Applied
Scientific EffectThermal contraction: Thermal Contraction

Data Source

PatentUS12116480B2Heat-shrinkable polyester-based film
Publication Date: 2024.10.15 TOYOBO CO LTD

AI summary

The invention provides a heat-shrinkable polyester-based film, where the heat-shrinkage ratio in the width direction is high and the irregularity of thickness is small. The heat-shrinkable polyester-based film of the present invention contains 90 mol % or more of ethylene terephthalate unit based on 100 mol % of whole ester unit, wherein, the heat-shrinkable polyester-based film satisfies the requirements: (1) heat-shrinkage ratio in a width direction measured by shrinking the film for 10 seconds in 90° C. hot water is 50%-75%, (2) heat-shrinkage ratio in a longitudinal direction measured by shrinking the film for 10 seconds in 90° C. hot water is −6% or more and 14% or less, (3) heat-shrinkage ratio in the longitudinal direction measured by shrinking the film for 10 seconds in 70° C. hot water is −6% or more and 6% or less, and (4) irregularity of thickness in the width direction is 1%-20%.