OLED Emission Layer Heterocyclic Compounds for Charge Recombination

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Solution Overview

Problem

Existing organic electroluminescence devices face challenges in optimizing the recombination of holes and electrons in the emission layer, leading to inefficient light emission and high driving voltage.

Innovation Solution

Incorporation of a heterocyclic compound with specific structural features, such as carbazole moieties bonded in an ortho relationship, in the emission layer, along with a multilayer structure including a hole transport region and electron transport region, utilizing materials like Ag, Mg, and transparent metal oxides for electrodes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If conventional emission layer materials are used, then device structure is simple, but light emission efficiency is low and driving voltage is high

Engineering Contradiction:
Improvelight emission efficiencyVSAvoidemission layer structure
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The emission layer employs a composite material system consisting of a host compound and a guest compound (Formula 1). The host compound provides the primary emission characteristics while the guest compound enhances efficiency through specific molecular interactions. This composite approach resolves the contradiction by achieving high light emission efficiency through material composition rather than structural complexity.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes specific parameters of the guest compound including molecular weight (500-2000 Da), triplet energy level (2.5-3.5 eV), and HOMO level (-5.0 to -6.0 eV). By precisely controlling these physical and chemical parameters, the emission efficiency is significantly improved while maintaining a relatively simple device structure.

Inventive Principle:
Principle #35Parameter changes

2Power

If conventional emission layer materials are used, then device structure is simple, but driving voltage is high

Engineering Contradiction:
Improvedriving voltageVSAvoidemission layer structure
Core Design Contradiction:
PowerVSDevice complexity

Solution Approach 1:

The HOMO energy level of the guest compound is specifically designed to be between -5.0 and -6.0 eV, which optimizes hole injection and reduces energy barriers. This parameter optimization enables lower driving voltage operation while maintaining a simple emission layer structure consisting of host and guest compounds.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If high emission efficiency materials are used, then light emission efficiency is improved, but manufacturing complexity increases

Engineering Contradiction:
Improvelight emission efficiencyVSAvoidmanufacturing process
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The emission layer is segmented into functional components: host compound (providing emission backbone), guest compound (Formula 1, providing efficiency enhancement), and optional additives. This segmentation allows each component to be optimized independently for performance while maintaining compatibility with standard manufacturing processes like vacuum deposition and solution processing.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The molecular weight of the guest compound is controlled within 500-2000 Da, ensuring appropriate volatility for vacuum deposition and solubility for solution processing. This parameter control enables high emission efficiency to be achieved through material selection rather than complex manufacturing procedures.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enhances light emission efficiency and reduces driving voltage by improving the recombination of holes and electrons, resulting in improved performance of the organic electroluminescence device.

Implementation Method 1

holes and electrons injected from a first electrode and a second electrode recombine in an emission layer, and a light-emitting material which is an organic compound included in the emission layer emits light

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Implementation Method 2

The holes and electrons injected into the emission layer recombine to produce excitons in the emission layer. The organic electroluminescence device emits light using light generated by the transition of the excitons to a ground state.

Methodology Applied
Scientific EffectRadiative recombination: Luminescence

Data Source

PatentEP4029864B1Organic electroluminescence device and heterocyclic compound for organic electroluminescence device
Publication Date: 2025.07.30 SAMSUNG DISPLAY CO LTD
  • EP4029864B1 patent drawingFigure 1~2
  • EP4029864B1 patent drawingFigure 3
  • EP4029864B1 patent drawing

AI summary

An organic electroluminescence device and a heterocyclic compound are disclosed herein. The device includes a first electrode; a hole transport region on the first electrode; an emission layer on the hole transport region; an electron transport region on the emission layer; and a second electrode on the electron transport region, wherein the emission layer includes a heterocyclic compound that includes a nitrogen-containing monocycle, at least one linker, and two or more carbazole moieties. The at least one linker is a substituted or unsubstituted dibenzofuran group or a substituted or unsubstituted dibenzothiophene group, and at least one of the carbazole moieties and the nitrogen-containing monocycle are bonded to the at least one linker in an ortho relationship.