HFC-143 Purification via Solvent-Assisted Extractive Distillation

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Solution Overview

Problem

There is a need for an efficient method to purify 1,1,2-trifluoroethane (HFC-143), which is used as a refrigerant and intermediate for obtaining HFO-1132, but current methods are inadequate in achieving high purity efficiently.

Innovation Solution

The method involves an extractive distillation step where a composition containing 1-chloro-1,1,2-trifluoroethane (HCFC-133b) and/or 1,2-dichloro-1,1,2-trifluoroethane (HCFC-123a) is brought into contact with a solvent such as an amine, halogen compound, or toluene to reduce the amount of HCFC-133b and/or HCFC-123a, followed by a distillation step to separate the components.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional distillation methods are used to purify HFC-143, then the purification process is simple, but the purification efficiency is insufficient and cannot achieve high purity effectively

Engineering Contradiction:
Improvepurity of HFC-143VSAvoidpurification efficiency
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The patent introduces a solvent as an intermediary substance to facilitate the separation of HFC-143 from impurities. The solvent selectively interacts with impurity components (such as HCFC-133b and HCFC-123a) through extraction, enabling more effective purification than direct distillation alone. This mediator approach resolves the contradiction by achieving both high purity and improved purification efficiency through the solvent-assisted extractive distillation process

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the operational parameters of the distillation process by introducing a solvent that modifies the relative volatility between HFC-143 and impurity components. By changing the chemical environment through solvent addition, the separation efficiency is enhanced, allowing simultaneous achievement of high purity and efficient purification through the modified distillation conditions

Inventive Principle:
Principle #35Parameter changes

2Productivity

If multiple purification steps are added to achieve high purity HFC-143, then the purification efficiency improves, but the process complexity increases

Engineering Contradiction:
Improvepurification efficiencyVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent merges the extraction function and distillation function into a single integrated extractive distillation process. By combining these two separation mechanisms in one operational unit, the process achieves high purification efficiency without requiring separate extraction and distillation equipment, thus avoiding increased process complexity while maintaining improved productivity

Inventive Principle:
Principle #5Merging (Combining)

3Manufacturing precision

If extractive distillation with solvent is used to purify HFC-143, then the purity of HFC-143 increases, but the process requires additional solvent recovery steps

Engineering Contradiction:
Improvepurity of HFC-143VSAvoidprocess steps
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent implements a solvent recovery system that captures and recycles the solvent from the distillation bottom product. This recovery mechanism eliminates the need for continuous solvent addition, reduces process waste, and maintains high HFC-143 purity while making the additional solvent handling steps self-sustaining rather than net additions to process complexity

Inventive Principle:
Principle #34Discarding and recovering

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method effectively purifies HFC-143 by reducing the content of HCFC-133b and/or HCFC-123a to less than 1 mass%, achieving a high purity of HFC-143, which is suitable for use as a refrigerant.

Implementation Method 1

an extractive distillation step of bringing a composition comprising 1-chloro-1,1,2-trifluoroethane (HCFC-133b) and/or 1,2-dichloro-1,1,2-trifluoroethane (HCFC-123a), and HFC-143 into contact with a solvent A to obtain a composition having a reduced amount of HCFC-133b and/or HCFC-123a

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 2

a distillation step of subjecting a composition comprising HCFC-133b and/or HCFC-123a, and the solvent A obtained from the bottom of an extractive distillation column through the extractive distillation step (1) to distillation to separate the composition into HCFC-133b and/or HCFC-123a, and the solvent A

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP4545510A1Method for producing purified 1,1,2-trifluoroethane (HFC-143), and composition containing HFC-143
Publication Date: 2025.04.30 DAIKIN INDUSTRIES LTD
  • EP4545510A1 patent drawingFigure 1
  • EP4545510A1 patent drawingFigure 2
  • EP4545510A1 patent drawingFigure 3

AI summary

An object of the present disclosure is to provide a method for efficiently purifying HFC-143, and a composition comprising HFC-143. A method for producing purified HFC-143.