High bulk tissue comprising cross-linked fibers

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Solution Overview

Problem

Existing tissue products face a challenge in achieving both increased bulk and tensile strength without compromising softness, as traditional methods often result in reduced fiber-to-fiber bonding and increased knits or knots when cross-linking cellulose fibers.

Innovation Solution

The method involves treating fibers with a caustic solution to reduce hemicellulose content and then cross-linking them at low temperatures using agents like polyamide epichlorohydrin resins, which are incorporated into tissue webs to enhance bulk and strength while minimizing knits and knots.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Volume of stationary object

If cross-linking agents are used to increase sheet bulk, then bulk is improved, but tensile strength and tear strength deteriorate due to reduced fiber to fiber bonding

Engineering Contradiction:
Improvesheet bulkVSAvoidtensile strength
Core Design Contradiction:
Volume of stationary objectVSStrength

Solution Approach 1:

The patent changes the chemical parameters of the cross-linking process by using specific cross-linking agents (melamine-formaldehyde, urea-formaldehyde, or isocyanate compounds) and controlling the molar ratio of cross-linking agent to cellulose hydroxyl groups (0.01:1 to 1:1). This allows optimization of both bulk and tensile strength by adjusting the degree of cross-linking. The patent also controls moisture content (5% to 50%) and temperature (20°C to 100°C) during cross-linking to achieve desired properties.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies cross-linking selectively to portions of the tissue web rather than uniformly throughout. By treating only certain areas or layers with cross-linking agents, the patent creates local regions of increased bulk while preserving fiber-to-fiber bonding in other areas, thus maintaining overall tensile strength. This selective application allows different parts of the tissue product to have different properties optimized for their specific functions.

Inventive Principle:
Principle #3Local quality

2Volume of stationary object

If through-air drying is used to increase sheet bulk, then bulk is improved, but softness deteriorates due to the need for calendering

Engineering Contradiction:
Improvesheet bulkVSAvoidsoftness
Core Design Contradiction:
Volume of stationary objectVSEase of operation

Solution Approach 1:

The patent applies cross-linking treatment before the drying process to stabilize the fiber structure. This preliminary cross-linking prevents fiber collapse during subsequent through-air drying and eliminates the need for calendering to achieve smoothness. The cross-linked fibers maintain their spacing and orientation, preserving softness while achieving high bulk through the drying process alone.

Inventive Principle:
Principle #10Preliminary action

3Volume of stationary object

If cross-linked fibers are used to increase bulk, then bulk is improved, but the number of knits and knots increases

Engineering Contradiction:
Improvesheet bulkVSAvoidknits and knots
Core Design Contradiction:
Volume of stationary objectVSManufacturing precision

Solution Approach 1:

The patent uses partial cross-linking where only a portion of the fibers are cross-linked, or only certain regions of the tissue web are cross-linked. By controlling the amount and distribution of cross-linking agent application, the patent achieves sufficient bulk enhancement without excessive cross-linking that would cause fibers to stick together and form knits and knots. The cross-linking density is optimized to prevent unwanted fiber aggregation.

Inventive Principle:
Principle #16Partial or excessive action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach results in tissue products with improved bulk, strength, and reduced stiffness, maintaining softness and increasing sheet bulk by up to 20% compared to products without cross-linked fibers, while maintaining comparable tensile strength.

Implementation Method 1

treating a plurality of fibers with a caustic solution at a temperature less than about 60° C. to yield a plurality of caustic extracted fibers having a hemicellulose content at least about 50 percent less than the plurality of fibers

Methodology Applied
Scientific EffectChemical extraction: Solvation

Implementation Method 2

treating a plurality of fibers with a caustic solution at a temperature less than about 60° C. to yield a plurality of caustic extracted fibers having a hemicellulose content at least about 50 percent less than the plurality of fibers (b) mixing the caustic extracted fibers with a cross-linking agent to yield a plurality of treated fibers

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Implementation Method 3

drying the treated fibers at a drying temperature less than about 200° C. to yield a plurality of cross-linked fibers

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentUS10458067B2High bulk tissue comprising cross-linked fibers
Publication Date: 2019.10.29 KIMBERLY CLARK WORLDWIDE INC

AI summary

The present application relates to a cross-linked fiber and more specifically to fibers that have been subjected to cold caustic extraction (at less than 60° C.) to reduce the hemicellulose content of the fibers by at least 50% and then cross-linked with a cross-linking agent that is curable at a modest temperature, such as less than 160° C. The treated cross-linked fibers preferably have a hemicellulose content that is less than 5% by weight of the fiber. Preferable cross-linking agents are polyamide-epichlorohydrin (PAE) resins, polyamide-polyamine-epichlorohydrin (PPE) resins, and polydiallylamine-epichlorohydrin resins. The cross-linked fibers are readily dispersible in water even without fiberization and generally form webs and products having relatively few knits or knots. As such, the cross-linked fibers of the present invention are well suited for use in the manufacture of tissue webs and products, particularly wet-laid tissue webs and products.